CH328659A - Process for the preparation of a disazo dye - Google Patents

Process for the preparation of a disazo dye

Info

Publication number
CH328659A
CH328659A CH328659DA CH328659A CH 328659 A CH328659 A CH 328659A CH 328659D A CH328659D A CH 328659DA CH 328659 A CH328659 A CH 328659A
Authority
CH
Switzerland
Prior art keywords
parts
disazo dye
methyl
preparation
amino
Prior art date
Application number
Other languages
German (de)
Inventor
Hans Dr Ischer
Lukas Dr Schneider
Original Assignee
Sandoz Ag
Priority date (The priority date is an assumption and is not a legal conclusion. Google has not performed a legal analysis and makes no representation as to the accuracy of the date listed.)
Filing date
Publication date
Application filed by Sandoz Ag filed Critical Sandoz Ag
Publication of CH328659A publication Critical patent/CH328659A/en

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Classifications

    • CCHEMISTRY; METALLURGY
    • C09DYES; PAINTS; POLISHES; NATURAL RESINS; ADHESIVES; COMPOSITIONS NOT OTHERWISE PROVIDED FOR; APPLICATIONS OF MATERIALS NOT OTHERWISE PROVIDED FOR
    • C09BORGANIC DYES OR CLOSELY-RELATED COMPOUNDS FOR PRODUCING DYES, e.g. PIGMENTS; MORDANTS; LAKES
    • C09B45/00Complex metal compounds of azo dyes
    • C09B45/02Preparation from dyes containing in o-position a hydroxy group and in o'-position hydroxy, alkoxy, carboxyl, amino or keto groups
    • C09B45/24Disazo or polyazo compounds
    • C09B45/28Disazo or polyazo compounds containing copper
    • CCHEMISTRY; METALLURGY
    • C09DYES; PAINTS; POLISHES; NATURAL RESINS; ADHESIVES; COMPOSITIONS NOT OTHERWISE PROVIDED FOR; APPLICATIONS OF MATERIALS NOT OTHERWISE PROVIDED FOR
    • C09BORGANIC DYES OR CLOSELY-RELATED COMPOUNDS FOR PRODUCING DYES, e.g. PIGMENTS; MORDANTS; LAKES
    • C09B35/00Disazo and polyazo dyes of the type A<-D->B prepared by diazotising and coupling
    • C09B35/02Disazo dyes
    • C09B35/039Disazo dyes characterised by the tetrazo component
    • C09B35/28Disazo dyes characterised by the tetrazo component the tetrazo component containing two aryl nuclei linked by at least one of the groups —CON<, —SO2N<, —SO2—, or —SO2—O—

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  • Chemical & Material Sciences (AREA)
  • Organic Chemistry (AREA)
  • Organic Low-Molecular-Weight Compounds And Preparation Thereof (AREA)

Description

  

      Verfahren        zur        Herstellung    eines     Disazofarbstoffes       Gegenstand der vorliegenden Erfindung  ist ein Verfahren zur     Herstellung    eines     Dis-          azofarbstoffes,    -welches darin besteht, dass man  1     Mol    der durch Kuppeln von     tetrazotierter          1-(4'-Amino-3'-methyl)-benzoylamino-4-amino-          benzol-3-carbonsäure    mit     5-Oxy-7-sulfo-          naphthyl    (2)     -carbaminsäure-    (4' -     acetylamino)

          -          phenylamid    erhältlichen     Diazomonoazoverbin-          dung    mit 1     Mo11-Phenyl-3-methyl-5-pyrazolon-          3'-sulfonsäüre        kuppelt.    ,  Im Beispiel bedeuten die Teile Gewichts  teile.  



       Beispiel     Eine     neutralgestellte,        8-10     kalte Suspen  sion der durch Kuppeln von 28,5 -Teilen     tetra-          zotierter        1-(4'-Amino-3'-methyl)-benzoylamino-          4-aminobenzol-3-carbonsäure    mit 41,5 Teilen       5--Oxy-7-sulfonaphthyl(2)        -carbaminsäure-        (4'-          acetyiamino)

  -phenyla.mid    erhältlichen     Diazo-          monoazozwischenverbindung    wird innerhalb  von einer Stunde in eine 30  warme Lösung  aus 28 Teilen     1-Phenyl-3-methyl-5-pyrazolon-          3'-sulfonsäure,    12 Teilen     Natriumcarbonat,     300 Teilen     Pyridin    und 500 Teilen Wasser  gegeben.

   Der gebildete     Disazofarbstoff    wird  nach zweistündigem Rühren mittels Zusatz  von     Natriumchlorid    abgeschieden, anschlie  ssend filtriert und     getrocknet.    Er färbt     Baum-          wolle    und     Fasern    aus regenerierter     Cellulose     im     Naehkupferungsverfahren    in scharlach  roten Tönen von guter Licht- und Waschecht  heit.  



  Die oben genannte Suspension der     Diazo-          monoazozwischenverbindiing    erhält man, wenn  man 28,5 Teile 1-(4'-Amino-3'-methyl)-benzoyl-         amino-4-aminobenzol-3-carbonsäure    in 800 Tei  len Eiswasser anrührt und die     Aufschläm-          mung    mit 50 Teilen     30o/oiger    Salzsäure und       hieraiü        bei        0         mit        46        Teilen        30%iger        Natrium-          nitritlösung    versetzt.

   Der     Tetrazolösung    lässt  man     eine    Lösung von 41,5 Teilen     5-0xy-7-          suHonaphthyl    (2) -     carbaminsäure    - (4' -     acetyl-          amino)-phenylamid        und    10 Teilen Natrium  carbonat in 400 Teilen Wasser zulaufen, stellt  die Temperatur der Kupplungsmasse auf  8-10  und gibt ihr innerhalb von einer  Stunde     portionenweise        ungefähr    20 Teile     Na-          triumbicarbonat    zu.

   Nachdem die Masse neu  tralgestellt     worden:    ist, rührt man sie noch  2 Stunden lang bei 8-10  weiter. Dabei kup  pelt nur die am     Benzoylrest    sitzende     Diazo-          gruppe.    Die entstandene     Diazomonoazozwi-          schenverbindung    scheidet sich in orangeroten  Kristallen aus.



      Process for the preparation of a disazo dye The present invention relates to a process for the preparation of a disazo dye, which consists in that 1 mol of 1- (4'-amino-3'-methyl) -benzoylamino-4-benzoylamino-4 -amino- benzene-3-carboxylic acid with 5-oxy-7-sulfonaphthyl (2) -carbamic acid- (4 '- acetylamino)

          - Phenylamide available diazomonoazo compound with 1 Mo11-phenyl-3-methyl-5-pyrazolone-3'-sulfonic acid. , In the example, the parts mean parts by weight.



       Example A neutralized, 8-10 cold suspension of the 1- (4'-amino-3'-methyl) -benzoylamino-4-aminobenzene-3-carboxylic acid tetrazotized by coupling 28.5 parts with 41.5 parts 5 - Oxy-7-sulfonaphthyl (2) -carbamic acid- (4'-acetyiamino)

  -phenyla.mid available diazo monoazo intermediate compound is added within one hour to a warm solution of 28 parts of 1-phenyl-3-methyl-5-pyrazolone-3'-sulfonic acid, 12 parts of sodium carbonate, 300 parts of pyridine and 500 parts of water .

   After stirring for two hours, the disazo dye formed is precipitated by adding sodium chloride, then filtered and dried. It dyes cotton and fibers from regenerated cellulose in the sewing process in scarlet red shades of good lightfastness and washfastness.



  The above-mentioned suspension of the diazo monoazo intermediate compound is obtained if 28.5 parts of 1- (4'-amino-3'-methyl) -benzoylamino-4-aminobenzene-3-carboxylic acid are stirred in 800 parts of ice water and the 50 parts of 30% strength hydrochloric acid were added to the suspension, followed by 46 parts of 30% strength sodium nitrite solution at 0.

   The tetrazo solution is allowed to run a solution of 41.5 parts of 5-0xy-7-suHonaphthyl (2) -carbamic acid - (4 '- acetyl-amino) -phenylamide and 10 parts of sodium carbonate in 400 parts of water, and the temperature of the coupling compound is set to 8-10 and add about 20 parts of sodium bicarbonate in portions within an hour.

   After the mass has been neutralized, it is stirred for a further 2 hours at 8-10. Only the diazo group on the benzoyl radical couples. The resulting diazomonoazo intermediate compound precipitates in orange-red crystals.

 

Claims (1)

PATENTANSPRUCH Verfahren zur Herstellung eines Disazo- farbstoffes, dadurch gekennzeichnet, däss man 1 Mol der durch Kuppeln von tetrazotierter 1-(4'-Ainino-3'-methyl)-benzoylamino-4-amino- benzol-3-carbonsäure mit 5-Oxy-7-sulfonaph thyl(2)-carbaminsäure-(4'-acetylamino) PATENT CLAIM A process for the preparation of a disazo dye, characterized in that 1 mol of the 1- (4'-amino-3'-methyl) -benzoylamino-4-aminobenzene-3-carboxylic acid obtained by coupling with 5-oxy -7-sulfonaphthyl (2) -carbamic acid- (4'-acetylamino) -phenyl- amid erhältlichen Diazomonoazoverbindung mit 1 Mol 1-Pheny 1-3-methyl-5-pyrazolon-3'- sulfonsäure kuppelt. Der neue Disazofarbstoff färbt Baumwolle und Fasern aus regenerierter Cellulose im Nachkupferungsverfahren in scharlachroten Tönen von guter Licht- und Waschechtheit. -phenyl amide available diazomonoazo compound with 1 mol of 1-pheny 1-3-methyl-5-pyrazolone-3'-sulfonic acid. The new disazo dye dyes cotton and fibers made from regenerated cellulose in the copper-plating process in scarlet shades of good lightfastness and washfastness.
CH328659D 1954-05-11 1954-05-11 Process for the preparation of a disazo dye CH328659A (en)

Applications Claiming Priority (2)

Application Number Priority Date Filing Date Title
CH328659T 1954-05-11
CH310831T 1954-05-11

Publications (1)

Publication Number Publication Date
CH328659A true CH328659A (en) 1958-03-15

Family

ID=25735781

Family Applications (1)

Application Number Title Priority Date Filing Date
CH328659D CH328659A (en) 1954-05-11 1954-05-11 Process for the preparation of a disazo dye

Country Status (1)

Country Link
CH (1) CH328659A (en)

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