CH90883A - Process for the preparation of p-arseno-di- (1-phenyl-2,3-dimethyl-4-amino-5-pyrazolone) -monoacetic acid. - Google Patents

Process for the preparation of p-arseno-di- (1-phenyl-2,3-dimethyl-4-amino-5-pyrazolone) -monoacetic acid.

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Publication number
CH90883A
CH90883A CH90883DA CH90883A CH 90883 A CH90883 A CH 90883A CH 90883D A CH90883D A CH 90883DA CH 90883 A CH90883 A CH 90883A
Authority
CH
Switzerland
Prior art keywords
dimethyl
amino
pyrazolone
phenyl
acid
Prior art date
Application number
Other languages
German (de)
Inventor
Farbwerke Vorm Meiste Bruening
Original Assignee
Hoechst Ag
Priority date (The priority date is an assumption and is not a legal conclusion. Google has not performed a legal analysis and makes no representation as to the accuracy of the date listed.)
Filing date
Publication date
Application filed by Hoechst Ag filed Critical Hoechst Ag
Publication of CH90883A publication Critical patent/CH90883A/en

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Description

  

  Verfahren zur Darstellung der     p-Arseno-di-(1-phenyl-2.3-diiimethy1-4-amino-5-pyrilzolon)-          monoessigsiinre.       Im Hauptpatent wurde ein Verfahren zur  Darstellung von     p-Arseno-di-(1-phenyl-2-3-          dimethyl-4-amino-5-pyrazolon)    -     monomethy-          lensulfoxylsäure    beschrieben, das darauf  ruht, dass man p-Asseno-di-(i-phenyl-2 ³     3-di-          methyl-4i-amino-5-pyrazolon)    mit     Fornial-          dehydsulfoxylat    behandelt, wodurch die  saure Atomgruppe -CH2-O-SOH eingeführt  wird.

   Durch diese Einführung gewinnt man  eine für medizinische Zwecke wertvolle  Verbindung.  



  Es wurde gefunden dass man durch Ein  führung des Essigsäurerestes -CH2-COOH an  Stelle des Methylensulfoxylrestes eine Ver  bindung mit ähnlicher Wirkungsweise ge  winnt. Um dieselbe herzustellen, lässt man  auf p-Arseno-di-(i-Phenyl-2 ³     3-dimethyl-4-          amiho-5-pyrazolon)    Halogenessigsäure, z. B.  Bromessigsäure, einwirken. Die neue Ver  bindung ist in Wasser schwer löslich, in  Alkohol unlöslich, in Mineralsäuren und     Al-          kalier    löst sie sich, mit den letzteren bildet  sie gelbliche, leicht lösliche Salze.

      Beispiel:  12,54 g salzsaures     p-Arseno-cli-(1-plienyl-          2    ³3-dimethyl-4-amino-5-pyrazolon) werden  in 100 cm' Wasser gelöst, mit 15%iger Na  tronlauge neutralisiert und 14 g Bromessig  säure, gelöst in 30 g Wasser, hinzugegeben.  Man erhitzt kurze Zeit auf etwa 60 , ver  dünnt dann mit Wasser und fügt Soda  lösung hinzu. Von dem Ungelösten wird  nun abfiltriert und die     Glycinarsenoverbin-          dung    aus d er Lösung mit Essigsäure ge  fällt.  



  Verwendet man in diesem Beispiel einen  grösseren Überschuss an Bromessigsäure, so  erhält man das dem Monoglygin ähnliche  Diglycin.



  Process for the preparation of the p-arseno-di- (1-phenyl-2,3-diimethy1-4-amino-5-pyrilzolone) monoacetic acids. In the main patent, a process for the preparation of p-arseno-di- (1-phenyl-2-3-dimethyl-4-amino-5-pyrazolone) - monomethylene sulfoxylic acid was described, which is based on the fact that one p-Asseno-di - (i-phenyl-2 ³ 3-dimethyl-4i-amino-5-pyrazolone) treated with formaldehyde sulfoxylate, whereby the acidic atomic group -CH2-O-SOH is introduced.

   This introduction creates a connection that is valuable for medical purposes.



  It has been found that by introducing the acetic acid residue -CH2-COOH instead of the methylene sulfoxyl residue, a connection with a similar mode of action is won. To prepare the same, p-arseno-di- (i-phenyl-23 3-dimethyl-4-amiho-5-pyrazolone) haloacetic acid, e.g. B. bromoacetic acid act. The new compound is sparingly soluble in water, insoluble in alcohol, it dissolves in mineral acids and alkalis, with the latter it forms yellowish, easily soluble salts.

      Example: 12.54 g of hydrochloric acid p-arseno-cli- (1-plienyl- 2 ³3-dimethyl-4-amino-5-pyrazolone) are dissolved in 100 cm 'of water, neutralized with 15% sodium hydroxide solution and 14 g of bromoacetic acid acid, dissolved in 30 g of water, was added. It is heated to about 60 for a short time, then diluted with water and soda solution is added. The undissolved material is then filtered off and the glycine arsenic compound is precipitated from the solution with acetic acid.



  If a larger excess of bromoacetic acid is used in this example, diglycine, which is similar to monoglygin, is obtained.

 

Claims (1)

PATENTANSPRUCH: Verfahren zur Herstellung von p-Arseno- di- (1-Plienyl-2 ³ 3-dimethyl- 4-amino-5-pyrazo- Ion,)-l'n.onoes,sigsäure, dadurch gekennzeich- ,net, -dass man Halogenessigsäure auf p-Ar- send-di-(1-phenyl-2³3-dimethyl-4-amino-5-py- razolon) einWirkenl lässt; die Säure, ist ein gelblidbös, in Wasser schwer lösliches, 'in Alkohol unlösliches Pulver, in Salzsäure ist sie löslich. Mit Alkalien und Alkalikarbo- naten bildet sie gelbel leicht lösliche Salze. PATENT CLAIM: Process for the production of p-arsenodi (1-plienyl-2 ³ 3-dimethyl- 4-amino-5-pyrazo-ion,) - l'n.onoes, acetic acid, thereby marked-, net, - that haloacetic acid is allowed to act on p-arsenic-di- (1-phenyl-233-dimethyl-4-amino-5-pyrazolone); the acid, is a yellowish powder, hardly soluble in water, insoluble in alcohol, it is soluble in hydrochloric acid. With alkalis and alkali carbonates, it forms yellow, easily soluble salts.
CH90883D 1917-12-15 1918-12-27 Process for the preparation of p-arseno-di- (1-phenyl-2,3-dimethyl-4-amino-5-pyrazolone) -monoacetic acid. CH90883A (en)

Applications Claiming Priority (2)

Application Number Priority Date Filing Date Title
DE90883X 1917-12-15
CH90186T 1918-12-27

Publications (1)

Publication Number Publication Date
CH90883A true CH90883A (en) 1921-10-01

Family

ID=25704132

Family Applications (1)

Application Number Title Priority Date Filing Date
CH90883D CH90883A (en) 1917-12-15 1918-12-27 Process for the preparation of p-arseno-di- (1-phenyl-2,3-dimethyl-4-amino-5-pyrazolone) -monoacetic acid.

Country Status (1)

Country Link
CH (1) CH90883A (en)

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