EP2823091A4 - ELECTROLYTIC CELL COMPRISING A THREE-PHASE INTERFACE FOR REACTING CARBON-BASED GASES IN AQUEOUS ELECTROLYTE - Google Patents

ELECTROLYTIC CELL COMPRISING A THREE-PHASE INTERFACE FOR REACTING CARBON-BASED GASES IN AQUEOUS ELECTROLYTE

Info

Publication number
EP2823091A4
EP2823091A4 EP13757822.5A EP13757822A EP2823091A4 EP 2823091 A4 EP2823091 A4 EP 2823091A4 EP 13757822 A EP13757822 A EP 13757822A EP 2823091 A4 EP2823091 A4 EP 2823091A4
Authority
EP
European Patent Office
Prior art keywords
aqueous electrolyte
electrolytic cell
phase interface
reacting carbon
based gases
Prior art date
Legal status (The legal status is an assumption and is not a legal conclusion. Google has not performed a legal analysis and makes no representation as to the accuracy of the status listed.)
Withdrawn
Application number
EP13757822.5A
Other languages
German (de)
French (fr)
Other versions
EP2823091A1 (en
Inventor
Ed Chen
Current Assignee (The listed assignees may be inaccurate. Google has not performed a legal analysis and makes no representation or warranty as to the accuracy of the list.)
VICEROY CHEMICAL Inc
Original Assignee
VICEROY CHEMICAL Inc
Priority date (The priority date is an assumption and is not a legal conclusion. Google has not performed a legal analysis and makes no representation as to the accuracy of the date listed.)
Filing date
Publication date
Application filed by VICEROY CHEMICAL Inc filed Critical VICEROY CHEMICAL Inc
Publication of EP2823091A1 publication Critical patent/EP2823091A1/en
Publication of EP2823091A4 publication Critical patent/EP2823091A4/en
Withdrawn legal-status Critical Current

Links

Classifications

    • C—CHEMISTRY; METALLURGY
    • C25—ELECTROLYTIC OR ELECTROPHORETIC PROCESSES; APPARATUS THEREFOR
    • C25B—ELECTROLYTIC OR ELECTROPHORETIC PROCESSES FOR THE PRODUCTION OF COMPOUNDS OR NON-METALS; APPARATUS THEREFOR
    • C25B3/00—Electrolytic production of organic compounds
    • C25B3/20—Processes
    • C25B3/25—Reduction
    • C—CHEMISTRY; METALLURGY
    • C25—ELECTROLYTIC OR ELECTROPHORETIC PROCESSES; APPARATUS THEREFOR
    • C25B—ELECTROLYTIC OR ELECTROPHORETIC PROCESSES FOR THE PRODUCTION OF COMPOUNDS OR NON-METALS; APPARATUS THEREFOR
    • C25B11/00—Electrodes; Manufacture thereof not otherwise provided for
    • C25B11/02—Electrodes; Manufacture thereof not otherwise provided for characterised by shape or form
    • C25B11/03—Electrodes; Manufacture thereof not otherwise provided for characterised by shape or form perforated or foraminous
    • C25B11/031—Porous electrodes
    • C—CHEMISTRY; METALLURGY
    • C25—ELECTROLYTIC OR ELECTROPHORETIC PROCESSES; APPARATUS THEREFOR
    • C25B—ELECTROLYTIC OR ELECTROPHORETIC PROCESSES FOR THE PRODUCTION OF COMPOUNDS OR NON-METALS; APPARATUS THEREFOR
    • C25B11/00—Electrodes; Manufacture thereof not otherwise provided for
    • C25B11/02—Electrodes; Manufacture thereof not otherwise provided for characterised by shape or form
    • C25B11/03—Electrodes; Manufacture thereof not otherwise provided for characterised by shape or form perforated or foraminous
    • C25B11/031—Porous electrodes
    • C25B11/032—Gas diffusion electrodes
    • C—CHEMISTRY; METALLURGY
    • C25—ELECTROLYTIC OR ELECTROPHORETIC PROCESSES; APPARATUS THEREFOR
    • C25B—ELECTROLYTIC OR ELECTROPHORETIC PROCESSES FOR THE PRODUCTION OF COMPOUNDS OR NON-METALS; APPARATUS THEREFOR
    • C25B11/00—Electrodes; Manufacture thereof not otherwise provided for
    • C25B11/04—Electrodes; Manufacture thereof not otherwise provided for characterised by the material
    • C25B11/051—Electrodes formed of electrocatalysts on a substrate or carrier
    • C25B11/073—Electrodes formed of electrocatalysts on a substrate or carrier characterised by the electrocatalyst material
    • C25B11/075—Electrodes formed of electrocatalysts on a substrate or carrier characterised by the electrocatalyst material consisting of a single catalytic element or catalytic compound
    • C25B11/081—Electrodes formed of electrocatalysts on a substrate or carrier characterised by the electrocatalyst material consisting of a single catalytic element or catalytic compound the element being a noble metal
    • C—CHEMISTRY; METALLURGY
    • C25—ELECTROLYTIC OR ELECTROPHORETIC PROCESSES; APPARATUS THEREFOR
    • C25B—ELECTROLYTIC OR ELECTROPHORETIC PROCESSES FOR THE PRODUCTION OF COMPOUNDS OR NON-METALS; APPARATUS THEREFOR
    • C25B3/00—Electrolytic production of organic compounds
    • C25B3/01—Products
    • C25B3/03—Acyclic or carbocyclic hydrocarbons
    • C—CHEMISTRY; METALLURGY
    • C25—ELECTROLYTIC OR ELECTROPHORETIC PROCESSES; APPARATUS THEREFOR
    • C25B—ELECTROLYTIC OR ELECTROPHORETIC PROCESSES FOR THE PRODUCTION OF COMPOUNDS OR NON-METALS; APPARATUS THEREFOR
    • C25B3/00—Electrolytic production of organic compounds
    • C25B3/01—Products
    • C25B3/05—Heterocyclic compounds
    • C—CHEMISTRY; METALLURGY
    • C25—ELECTROLYTIC OR ELECTROPHORETIC PROCESSES; APPARATUS THEREFOR
    • C25B—ELECTROLYTIC OR ELECTROPHORETIC PROCESSES FOR THE PRODUCTION OF COMPOUNDS OR NON-METALS; APPARATUS THEREFOR
    • C25B3/00—Electrolytic production of organic compounds
    • C25B3/01—Products
    • C25B3/07—Oxygen containing compounds
    • C—CHEMISTRY; METALLURGY
    • C25—ELECTROLYTIC OR ELECTROPHORETIC PROCESSES; APPARATUS THEREFOR
    • C25B—ELECTROLYTIC OR ELECTROPHORETIC PROCESSES FOR THE PRODUCTION OF COMPOUNDS OR NON-METALS; APPARATUS THEREFOR
    • C25B3/00—Electrolytic production of organic compounds
    • C25B3/20—Processes
    • C25B3/23—Oxidation
    • C—CHEMISTRY; METALLURGY
    • C25—ELECTROLYTIC OR ELECTROPHORETIC PROCESSES; APPARATUS THEREFOR
    • C25B—ELECTROLYTIC OR ELECTROPHORETIC PROCESSES FOR THE PRODUCTION OF COMPOUNDS OR NON-METALS; APPARATUS THEREFOR
    • C25B9/00—Cells or assemblies of cells; Constructional parts of cells; Assemblies of constructional parts, e.g. electrode-diaphragm assemblies; Process-related cell features
    • Y—GENERAL TAGGING OF NEW TECHNOLOGICAL DEVELOPMENTS; GENERAL TAGGING OF CROSS-SECTIONAL TECHNOLOGIES SPANNING OVER SEVERAL SECTIONS OF THE IPC; TECHNICAL SUBJECTS COVERED BY FORMER USPC CROSS-REFERENCE ART COLLECTIONS [XRACs] AND DIGESTS
    • Y10—TECHNICAL SUBJECTS COVERED BY FORMER USPC
    • Y10T—TECHNICAL SUBJECTS COVERED BY FORMER US CLASSIFICATION
    • Y10T156/00—Adhesive bonding and miscellaneous chemical manufacture
    • Y10T156/10—Methods of surface bonding and/or assembly therefor

Landscapes

  • Chemical & Material Sciences (AREA)
  • Organic Chemistry (AREA)
  • Engineering & Computer Science (AREA)
  • Chemical Kinetics & Catalysis (AREA)
  • Electrochemistry (AREA)
  • Materials Engineering (AREA)
  • Metallurgy (AREA)
  • Electrodes For Compound Or Non-Metal Manufacture (AREA)
  • Electrolytic Production Of Non-Metals, Compounds, Apparatuses Therefor (AREA)
  • Catalysts (AREA)
EP13757822.5A 2012-03-03 2013-03-01 ELECTROLYTIC CELL COMPRISING A THREE-PHASE INTERFACE FOR REACTING CARBON-BASED GASES IN AQUEOUS ELECTROLYTE Withdrawn EP2823091A4 (en)

Applications Claiming Priority (5)

Application Number Priority Date Filing Date Title
US201261606398P 2012-03-03 2012-03-03
US201261608583P 2012-03-08 2012-03-08
US201261639544P 2012-04-27 2012-04-27
US201261713487P 2012-10-13 2012-10-13
PCT/US2013/028748 WO2013134078A1 (en) 2012-03-03 2013-03-01 Electrolytic cell including a three-phase interface to react carbon-based gases in an aqueous electrolyte

Publications (2)

Publication Number Publication Date
EP2823091A1 EP2823091A1 (en) 2015-01-14
EP2823091A4 true EP2823091A4 (en) 2016-04-20

Family

ID=49042206

Family Applications (1)

Application Number Title Priority Date Filing Date
EP13757822.5A Withdrawn EP2823091A4 (en) 2012-03-03 2013-03-01 ELECTROLYTIC CELL COMPRISING A THREE-PHASE INTERFACE FOR REACTING CARBON-BASED GASES IN AQUEOUS ELECTROLYTE

Country Status (6)

Country Link
US (1) US20130228470A1 (en)
EP (1) EP2823091A4 (en)
CN (1) CN104428449A (en)
CA (1) CA2866306A1 (en)
RU (1) RU2014139975A (en)
WO (1) WO2013134078A1 (en)

Families Citing this family (19)

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Publication number Priority date Publication date Assignee Title
US10329676B2 (en) * 2012-07-26 2019-06-25 Avantium Knowledge Centre B.V. Method and system for electrochemical reduction of carbon dioxide employing a gas diffusion electrode
US20140275629A1 (en) * 2013-03-14 2014-09-18 Ed Ite Chen Method and Apparatus for the Electrical Activation of a Catalyst
US10161051B2 (en) 2013-10-03 2018-12-25 Brown University Electrochemical reduction of CO2 at copper nanofoams
CN106521544B (en) * 2015-09-15 2018-07-13 中国科学院大连化学物理研究所 Carbon dioxide electrochemical reduction porous electrode complex and its preparation and application
WO2018067632A1 (en) * 2016-10-04 2018-04-12 Johna Leddy Carbon dioxide reduction and carbon compound electrochemistry in the presence of lanthanides
US10675681B2 (en) 2017-02-02 2020-06-09 Honda Motor Co., Ltd. Core shell
DE102017204096A1 (en) 2017-03-13 2018-09-13 Siemens Aktiengesellschaft Production of gas diffusion electrodes with ion transport resins for the electrochemical reduction of CO2 to chemical recyclables
US11613819B2 (en) 2017-06-21 2023-03-28 The Governing Council Of The University Of Toronto Catalysts with sharp reaction interface for electrochemical CO2 reduction with enhanced selectivity
US11299811B2 (en) 2018-01-29 2022-04-12 Board Of Regents, The University Of Texas System Continuous flow reactor and hybrid electro-catalyst for high selectivity production of C2H4 from CO2 and water via electrolysis
DE102018201287A1 (en) * 2018-01-29 2019-08-01 Siemens Aktiengesellschaft Porous electrode for the electrochemical conversion of organic compounds into two immiscible phases in an electrochemical flux reactor
CN109811364B (en) * 2019-01-10 2020-10-27 北京化工大学 A kind of ruthenium/cuprous oxide electrocatalytic material and preparation method thereof
US11686004B2 (en) * 2019-10-22 2023-06-27 University Of Cincinnati Gas diffusion electrodes with segmented catalyst layers for CO2 reduction
IT201900020026A1 (en) * 2019-10-30 2021-04-30 Industrie De Nora Spa ELECTRODE FOR THE ELECTROLYTIC EVOLUTION OF HYDROGEN
WO2021243199A1 (en) * 2020-05-29 2021-12-02 Newchem21 Inc. Process for electrochemical oxidation of hydrocarbons
US12134826B2 (en) 2021-03-04 2024-11-05 Totalenergies Onetech CO2 electroreduction to multi-carbon products in strong acid
CN113151849B (en) * 2021-03-24 2024-01-19 厦门大学 Method for preparing lactic acid by using propane
CN114373940B (en) * 2021-12-16 2025-01-24 清华大学 Gas diffusion electrode and its preparation method and application
CN115161687B (en) * 2022-06-22 2025-06-13 华南理工大学 A biocarbon-based gas diffusion electrode with multiple pores and its preparation method and application
WO2024233449A1 (en) * 2023-05-05 2024-11-14 Rensselaer Polytechnic Institute Systems and methods for converting co2 to one or more multicarbon products

Citations (3)

* Cited by examiner, † Cited by third party
Publication number Priority date Publication date Assignee Title
US4673473A (en) * 1985-06-06 1987-06-16 Peter G. Pa Ang Means and method for reducing carbon dioxide to a product
JPS62297483A (en) * 1986-02-13 1987-12-24 Kotaro Ogura Selective conversion of methane into methanol and chloromethane at ordinary temperature
WO2011150422A1 (en) * 2010-05-28 2011-12-01 The Trustees Of Columbia University In The City Of New York Porous metal dendrites as gas diffusion electrodes for high efficiency aqueous reduction of co2 to hydrocarbons

Family Cites Families (9)

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Publication number Priority date Publication date Assignee Title
JPH0697614B2 (en) * 1988-08-26 1994-11-30 エヌ・イーケムキャット株式会社 Supported platinum alloy electrocatalyst
FR2751564B1 (en) * 1996-07-26 2001-10-12 Inst Francais Du Petrole METHOD AND DEVICE FOR THE OPERATION OF A THREE-PHASE BUBBLE COLUMN WITH FISCHER-TROPSCH SYNTHESIS APPLICATION
US7507687B2 (en) * 2000-03-22 2009-03-24 Cabot Corporation Electrocatalyst powders, methods for producing powder and devices fabricated from same
US7201993B2 (en) * 2000-08-04 2007-04-10 Matsushita Electric Industrial Co., Ltd. Polymer electrolyte fuel cell
JP4923598B2 (en) * 2006-02-02 2012-04-25 トヨタ自動車株式会社 Highly hydrophilic carrier, catalyst carrier, fuel cell electrode, method for producing the same, and polymer electrolyte fuel cell including the same
KR101386162B1 (en) * 2006-07-21 2014-04-18 삼성에스디아이 주식회사 Electrode for fuel cell and fuel cell employing the same
JP5322145B2 (en) * 2007-05-30 2013-10-23 株式会社日立製作所 Composite electrolyte membrane for fuel cell and production method thereof, membrane electrode assembly and fuel cell
US8409419B2 (en) * 2008-05-21 2013-04-02 Paul R. Kruesi Conversion of carbon to hydrocarbons
US9145615B2 (en) * 2010-09-24 2015-09-29 Yumei Zhai Method and apparatus for the electrochemical reduction of carbon dioxide

Patent Citations (3)

* Cited by examiner, † Cited by third party
Publication number Priority date Publication date Assignee Title
US4673473A (en) * 1985-06-06 1987-06-16 Peter G. Pa Ang Means and method for reducing carbon dioxide to a product
JPS62297483A (en) * 1986-02-13 1987-12-24 Kotaro Ogura Selective conversion of methane into methanol and chloromethane at ordinary temperature
WO2011150422A1 (en) * 2010-05-28 2011-12-01 The Trustees Of Columbia University In The City Of New York Porous metal dendrites as gas diffusion electrodes for high efficiency aqueous reduction of co2 to hydrocarbons

Non-Patent Citations (3)

* Cited by examiner, † Cited by third party
Title
JUN YANO ET AL: "Selective ethylene formation by pulse-mode electrochemical reduction of carbon dioxide using copper and copper-oxide electrodes", JOURNAL OF SOLID STATE ELECTROCHEMISTRY ; CURRENT RESEARCH AND DEVELOPMENT IN SCIENCE AND TECHNOLOGY, SPRINGER, BERLIN, DE, vol. 11, no. 4, 29 July 2006 (2006-07-29), pages 554 - 557, XP019462203, ISSN: 1433-0768 *
KOTARO OGURA ET AL: "Direct conversion of methane to methanol, chloromethane and dichloromethane at room temperature'", NATURE, vol. 319, 23 January 1986 (1986-01-23), pages 308, XP055157326 *
See also references of WO2013134078A1 *

Also Published As

Publication number Publication date
WO2013134078A1 (en) 2013-09-12
RU2014139975A (en) 2016-04-20
CN104428449A (en) 2015-03-18
US20130228470A1 (en) 2013-09-05
EP2823091A1 (en) 2015-01-14
CA2866306A1 (en) 2013-09-12

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