CH90882A - Process for the preparation of p-arseno-di- (1-phenyl-2,3-dimethyl-4-amino-5-pyrazolone) -monomethylene sulfoxylic acid. - Google Patents

Process for the preparation of p-arseno-di- (1-phenyl-2,3-dimethyl-4-amino-5-pyrazolone) -monomethylene sulfoxylic acid.

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Publication number
CH90882A
CH90882A CH90882DA CH90882A CH 90882 A CH90882 A CH 90882A CH 90882D A CH90882D A CH 90882DA CH 90882 A CH90882 A CH 90882A
Authority
CH
Switzerland
Prior art keywords
dimethyl
amino
phenyl
pyrazolone
monomethylene
Prior art date
Application number
Other languages
German (de)
Inventor
Farbwerke Vorm Meiste Bruening
Original Assignee
Hoechst Ag
Priority date (The priority date is an assumption and is not a legal conclusion. Google has not performed a legal analysis and makes no representation as to the accuracy of the date listed.)
Filing date
Publication date
Application filed by Hoechst Ag filed Critical Hoechst Ag
Publication of CH90882A publication Critical patent/CH90882A/en

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Description

  

      Verfahren    zur Darstellung von     p-Arseno-di-(1-phenyl-2.3-dimethyl-4-amino-ö-pyi#azolon)-          monomethylensulfoxylsäure.       Durch Einführung der     Methylensulfoxyl-          gruppe    in das     p-Arseno-di-(1-phenyl-2.3-          dimethyl-4-amino-5-pyrazolon)    gewinnt man  nach dem Hauptpatent, indem man es mit       Formaldehydsulfosäure    .behandelt, die     p-          Arseno-di-(1-phenyl-2    .

       3-dimethyl-4-amino-5-          pyrazolon)-monomethylensLilfoxylsäure     Es     wurde    gefunden, dass man dieselbe  Verbindung erhält, indem man die Darstel  lung der erstgenannten     Aminoverbindung          mit    der Einführung der     Methylensulfoxyl-          gruppe    in einer Operation vereinigt in der  Weise,     dass    man das     1-.(Phenyl-p=arsinsäure)-          2.3-climethyl-5-pyrazolon        nitrosiert    und die       entstehende        Nitrosoverbindung    mit Formal  dehydsulfoxylat behandelt.

    



       Beispiel:     <B>15,6</B> g     1-(Phenyl-p-arsinsäure)        9-    .     3-di-          methyl-5-pyräzolon    werden mit 50 cm'     nor-          mäler    Natronlauge. gelöst und mit 3,5 g       Natriumnitrit    in 10     cm3    Wasser versetzt.  Hierauf gibt man 50 cm'
EMI0001.0033  
       -Salzsäure    zu,    Sobald die     Nitroso-Verbindung    vollkommen  auskristallisiert ist, fügt man 80 g     Formal-          dehydsulfoxylat    in 150 cm' Wasser gelöst  zu.

   Es entsteht eine klare gelbe Lösung; die  nach Zugabe von 25     cm3   
EMI0001.0039  
   -Salzsäure auf  dem     Wasserbad    kurze Zeit erwärmt wird.  Sodann wird gefällt, sofort Eis Hinzugege  ben und die abgeschiedene     Sulfoxylsäüre-          abgesaugt    und gut gewaschen.



      Process for the preparation of p-arseno-di- (1-phenyl-2,3-dimethyl-4-amino-ö-pyi # azolon) - monomethylene sulfoxylic acid. By introducing the methylene sulfoxyl group into the p-arseno-di- (1-phenyl-2,3-dimethyl-4-amino-5-pyrazolone), according to the main patent, by treating it with formaldehyde sulfonic acid, the p-arsenic acid di- (1-phenyl-2.

       3-dimethyl-4-amino-5-pyrazolon) monomethylene lilfoxylic acid It has been found that the same compound is obtained by combining the representation of the first-mentioned amino compound with the introduction of the methylene sulfoxyl group in one operation in such a way that the 1 -. (Phenyl-p = arsinic acid) - 2.3-climethyl-5-pyrazolone nitrosated and the nitroso compound formed is treated with formaldehyde sulfoxylate.

    



       Example: <B> 15.6 </B> g 1- (phenyl-p-arsic acid) 9-. 3-dimethyl-5-pyrazolone are mixed with 50 cm 'normal sodium hydroxide solution. dissolved and mixed with 3.5 g sodium nitrite in 10 cm3 water. Then give 50 cm '
EMI0001.0033
       Hydrochloric acid. As soon as the nitroso compound has completely crystallized out, 80 g of formaldehyde sulfoxylate dissolved in 150 cm of water are added.

   A clear yellow solution results; after adding 25 cm3
EMI0001.0039
   - Hydrochloric acid is heated briefly on a water bath. Then it is precipitated, ice is added immediately and the sulfoxylic acid which has separated out is filtered off with suction and washed thoroughly.

 

Claims (1)

PATENTANSPRUCH: Verfabren zur Darstellung von p-Arseno- d i-(1-ph en5T1-2 . 3-climethyl-jt-amino-5-pyräzo= Ion)-monomethylensulfoxylsäure, .dadurch gekennzeichnet, dass man das 1.-(Plienyl=p- arsinsä.ure)-2 - 3-dimethyl-5-pyräzolon nitro- siert und die entstehende Nitrosoverbindung mit Formaldeliydsulfoxylat behandelt. PATENT CLAIM: Method for the preparation of p-arsenod i- (1-ph en5T1-2. 3-climethyl-jt-amino-5-pyrazo = ion) -monomethylene sulfoxylic acid, characterized in that the 1 .- (plienyl = p-arsinic acid) -2-3-dimethyl-5-pyrazolone nitro- sated and the resulting nitroso compound treated with formaldehyde sulfoxylate.
CH90882D 1917-12-15 1918-12-27 Process for the preparation of p-arseno-di- (1-phenyl-2,3-dimethyl-4-amino-5-pyrazolone) -monomethylene sulfoxylic acid. CH90882A (en)

Applications Claiming Priority (2)

Application Number Priority Date Filing Date Title
DE90882X 1917-12-15
CH90186T 1918-12-27

Publications (1)

Publication Number Publication Date
CH90882A true CH90882A (en) 1921-10-01

Family

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Family Applications (1)

Application Number Title Priority Date Filing Date
CH90882D CH90882A (en) 1917-12-15 1918-12-27 Process for the preparation of p-arseno-di- (1-phenyl-2,3-dimethyl-4-amino-5-pyrazolone) -monomethylene sulfoxylic acid.

Country Status (1)

Country Link
CH (1) CH90882A (en)

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