CN102732205A - High temperature resistant polyurethane complex adhesive - Google Patents

High temperature resistant polyurethane complex adhesive Download PDF

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Publication number
CN102732205A
CN102732205A CN2012102287651A CN201210228765A CN102732205A CN 102732205 A CN102732205 A CN 102732205A CN 2012102287651 A CN2012102287651 A CN 2012102287651A CN 201210228765 A CN201210228765 A CN 201210228765A CN 102732205 A CN102732205 A CN 102732205A
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parts
high temperature
temperature resistant
resistant polyurethane
dioctyl phthalate
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CN2012102287651A
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CN102732205B (en
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吴朋钱
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ZHEJIANG DUOBANG CHEMICAL CO Ltd
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ZHEJIANG DUOBANG CHEMICAL CO Ltd
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    • YGENERAL TAGGING OF NEW TECHNOLOGICAL DEVELOPMENTS; GENERAL TAGGING OF CROSS-SECTIONAL TECHNOLOGIES SPANNING OVER SEVERAL SECTIONS OF THE IPC; TECHNICAL SUBJECTS COVERED BY FORMER USPC CROSS-REFERENCE ART COLLECTIONS [XRACs] AND DIGESTS
    • Y02TECHNOLOGIES OR APPLICATIONS FOR MITIGATION OR ADAPTATION AGAINST CLIMATE CHANGE
    • Y02WCLIMATE CHANGE MITIGATION TECHNOLOGIES RELATED TO WASTEWATER TREATMENT OR WASTE MANAGEMENT
    • Y02W30/00Technologies for solid waste management
    • Y02W30/50Reuse, recycling or recovery technologies
    • Y02W30/62Plastics recycling; Rubber recycling

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  • Compositions Of Macromolecular Compounds (AREA)
  • Adhesives Or Adhesive Processes (AREA)

Abstract

The invention discloses a high temperature resistant polyurethane complex adhesive, which belongs to the technical field of complex adhesives. The high temperature resistant polyurethane complex adhesive comprises the following substances by weight: 160 parts of methylbenzene, 150 parts of dimethyl carbonate, 587.5 parts of aromatic polyester polyol, 30 parts of polyphthalate polyol ester, 1.63 parts of trimethylolpropane, 65 parts of methylbenzene-2,4-diisocyanate, 1.5 parts of catalyst CAT S102, 1.2 parts of 1,4-butanediol, 1.2 parts of 1,3-butanediol, 0.15 part of antioxidant and 3.02 parts of organic bismuth. The complex adhesive, provided by the invention, has the advantages of large binding strength, strong high temperature resistance, short curing time of chemical curing, and capability of saving energy, optimizing environment and reaching standards of export products of European Union.

Description

A kind of high temperature resistant polyurethane composite gel
Technical field
The invention belongs to the composite gum technical field, be specifically related to a kind of high temperature resistant polyurethane composite gel.
Background technology
At present, the solvent borne polyurethane composite gum that market is supplied, the compound textiles slurry point displacement generation foaming will occur as carrying out the stamp processing again, causes waste product to increase.
Going up goods to the bed of European Union's area outlet will can not blistered standard-required through 90 ℃ of 60 washings, and commercially available product does not all reach this requirement at present.
Summary of the invention
For addressing the above problem, the object of the present invention is to provide a kind of high temperature resistant polyurethane composite gel.
A kind of high temperature resistant polyurethane composite gel; Material by following parts by weight is formed: 160 parts of toluene, 3.02 parts of 150 parts of methylcarbonates, 587.5 parts of benzoic anhydride polyester polyols, 30 parts of polyphenyl dioctyl phthalate polyol esters, 1.63 parts of TriMethylolPropane(TMP)s, 65 parts of Toluene-2,4-diisocyanate .4-vulcabond, 1.5 parts of catalyzer CAT S102,1.2 parts of 1.4-butyleneglycols, 1.2 parts of 1.3-butyleneglycols, 0.15 part in oxidation inhibitor and organo-bismuths.
Said benzoic anhydride polyester polyol is polymerized by phthalic anhydride, hexanodioic acid and Diethylene Glycol.
Said polyphenyl dioctyl phthalate polyol ester is a kind of in polyphenyl dioctyl phthalate propylene glycol ester, polyphenyl dioctyl phthalate 1.3-butanediol ester, polyphenyl dioctyl phthalate 1.4-butanediol ester, the polyphenyl dioctyl phthalate pinakon ester and more than one.
Said oxidation inhibitor is antioxidant 1010.
Said organo-bismuth is an organo-bismuth 8108.
Said catalyzer CAT S102 (CAT S102 Catalyst) is organic two rings and organic acid mixture.
Said organic two rings can be two ethylenimine, and said organic acid can be Hydrocerol A.
Product type called after DB-2797 of the present invention.
Beneficial effect of the present invention: the present invention adopts phthalic acid synthetic benzoic anhydride polyester polyol to make urethane compound, produces big bond strength.Improve high-temperature resistance, and adopt catalyzer CAT S102, promote set time; This can replace using electrothermal solidifying, saves the energy and has optimized environment again, can reach outlet European Union product standard again; Improved textiles compound yield rate again, reduced production costs greatly.
Embodiment
Below in conjunction with specific embodiment the present invention is further specified.
Used antioxidant 1010 is available from Beijing Jiyi Chemicals Co., Ltd. in following examples; Organo-bismuth 8108 is available from the lucky chemical industry of last seamount ltd; Catalyzer CAT S102 is available from new allusion quotation chemical material (Shanghai) Co., Ltd..
Embodiment 1
A kind of high temperature resistant polyurethane composite gel, he is made up of the material of following parts by weight: 8,108 3.02 parts of 160 parts of toluene, 150 parts of methylcarbonates, 587.5 parts of benzoic anhydride polyester polyols, 30 parts of polyphenyl dioctyl phthalate propylene glycol esters, 1.63 parts of TriMethylolPropane(TMP)s, 65 parts of Toluene-2,4-diisocyanate .4-vulcabond, 1.2 parts of 1.4-butyleneglycols, 1.2 parts of 1.3-butyleneglycols, 0.15 part of antioxidant 1010 and organo-bismuths.
The preparation method of above-mentioned high temperature resistant polyurethane composite gel is following: get 160 parts of toluene, 587.5 parts of benzoic anhydride polyester polyols, 30 parts of polyphenyl dioctyl phthalate propylene glycol esters, 1.63 parts of TriMethylolPropane(TMP)s, 65 parts of Toluene-2,4-diisocyanate .4-vulcabond, 1.2 parts of 1.4-butyleneglycols, 0.15 part of antioxidant 1010 and 8,108 3.02 parts of thorough mixing of organo-bismuth, heat to 75-80 ℃, kept this temperature 15 minutes; Add 1.2 parts of 1.3-butyleneglycols; Mixing is cooled to normal temperature, adds 150 parts of methylcarbonates then; Mixing; After test solid content, viscosity is qualified, metering packing, warehouse-in.
Embodiment 2
A kind of high temperature resistant polyurethane composite gel, he is made up of the material of following parts by weight: 8,108 3.02 parts of 160 parts of toluene, 150 parts of methylcarbonates, 587.5 parts of benzoic anhydride polyester polyols, 30 parts of polyphenyl dioctyl phthalate 1.3-butanediol esters, 1.63 parts of TriMethylolPropane(TMP)s, 65 parts of Toluene-2,4-diisocyanate .4-vulcabond, 1.2 parts of 1.3-butyleneglycols, 1.2 parts of 1.4-butyleneglycols, 0.15 part of antioxidant 1010 and organo-bismuths.
The preparation method of above-mentioned high temperature resistant polyurethane composite gel is following: get 160 parts of toluene, 587.5 parts of benzoic anhydride polyester polyols, 30 parts of polyphenyl dioctyl phthalate 1.3-butanediol esters, 1.63 parts of TriMethylolPropane(TMP)s, 1.2 parts of 1.4-butyleneglycols, 65 parts of Toluene-2,4-diisocyanate .4-vulcabond, 0.15 part of antioxidant 1010 and 8,108 3.02 parts of thorough mixing of organo-bismuth, heat to 75-80 ℃, kept this temperature 15 minutes; Add 1.2 parts of 1.3-butyleneglycols; Mixing is cooled to normal temperature, adds 150 parts of methylcarbonates then; Mixing; After test solid content, viscosity is qualified, metering packing, warehouse-in.
Embodiment 3
A kind of high temperature resistant polyurethane composite gel, he is made up of the material of following parts by weight: 8,108 3.02 parts of 160 parts of toluene, 150 parts of methylcarbonates, 587.5 parts of benzoic anhydride polyester polyols, 30 parts of polyphenyl dioctyl phthalate 1.3-butanediol esters, 1.63 parts of TriMethylolPropane(TMP)s, 65 parts of Toluene-2,4-diisocyanate .4-vulcabond, 1.2 parts of 1.3-butyleneglycols, 1.2 parts of 1.4-butyleneglycols, 0.15 part of antioxidant 1010,1.5 parts of catalyzer CAT S102 and organo-bismuths.
The preparation method of above-mentioned high temperature resistant polyurethane composite gel is following: get 160 parts of toluene, 587.5 parts of benzoic anhydride polyester polyols, 30 parts of polyphenyl dioctyl phthalate 1.3-butanediol esters, 1.2 parts of 1.4-butyleneglycols, 1.63 parts of TriMethylolPropane(TMP)s, 65 parts of Toluene-2,4-diisocyanate .4-vulcabond, 0.15 part of antioxidant 1010,1.5 parts of catalyzer CAT S102 and 8,108 3.02 parts of thorough mixing of organo-bismuth, heat to 75-80 ℃, kept this temperature 15 minutes; Add 1.2 parts of 1.3-butyleneglycols; Mixing is cooled to normal temperature, adds 150 parts of methylcarbonates then; Mixing; After test solid content, viscosity is qualified, metering packing, warehouse-in.
Embodiment 4
A kind of high temperature resistant polyurethane composite gel, he is made up of the material of following parts by weight: 8,108 3.02 parts of 160 parts of toluene, 150 parts of methylcarbonates, 587.5 parts of benzoic anhydride polyester polyols, polyphenyl dioctyl phthalate 1.4-butanediol ester, 30 parts, 1.63 parts of TriMethylolPropane(TMP)s, 65 parts of Toluene-2,4-diisocyanate .4-vulcabond, 1.2 parts of 1.3-butyleneglycols, 1.2 parts of 1.4-butyleneglycols, 0.15 part of antioxidant 1010,1.5 parts of catalyzer CAT S102 and organo-bismuths.
The preparation method of above-mentioned high temperature resistant polyurethane composite gel is following: get 160 parts of toluene, 587.5 parts of benzoic anhydride polyester polyols, polyphenyl dioctyl phthalate 1.4-butanediol ester, 30 parts, 1.63 parts of TriMethylolPropane(TMP)s, 65 parts of Toluene-2,4-diisocyanate .4-vulcabond, 0.15 part of antioxidant 1010,1.2 parts of 1.4-butyleneglycols, 1.5 parts of catalyzer CAT S102 and 8,108 3.02 parts of thorough mixing of organo-bismuth, heat to 75-80 ℃, kept this temperature 15 minutes; Add 1.2 parts of 1.3-butyleneglycols; Mixing is cooled to normal temperature, adds 150 parts of methylcarbonates then; Mixing; After test solid content, viscosity is qualified, metering packing, warehouse-in.
Embodiment 5
A kind of high temperature resistant polyurethane composite gel, he is made up of the material of following parts by weight: 8,108 3.02 parts of 160 parts of toluene, 150 parts of methylcarbonates, 587.5 parts of benzoic anhydride polyester polyols, 30 parts of polyphenyl dioctyl phthalate pinakon esters, 1.63 parts of TriMethylolPropane(TMP)s, 65 parts of Toluene-2,4-diisocyanate .4-vulcabond, 1.2 parts of 1.3-butyleneglycols, 1.2 parts of 1.4-butyleneglycols, 0.15 part of antioxidant 1010,1.5 parts of catalyzer CAT S102 and organo-bismuths.
The preparation method of above-mentioned high temperature resistant polyurethane composite gel is following: get 160 parts of toluene, 587.5 parts of benzoic anhydride polyester polyols, 30 parts of polyphenyl dioctyl phthalate pinakon esters, 1.63 parts of TriMethylolPropane(TMP)s, 65 parts of Toluene-2,4-diisocyanate .4-two isocyanide esters, 0.15 part of antioxidant 1010,1.2 parts of 1.4-butyleneglycols, 1.5 parts of catalyzer CAT S102 and 8,108 3.02 parts of thorough mixing of organo-bismuth, heat to 75-80 ℃, kept this temperature 15 minutes; Add 1.2 parts of 1.3-butyleneglycols; Mixing is cooled to normal temperature, adds 150 parts of methylcarbonates then; Mixing; After test solid content, viscosity is qualified, metering packing, warehouse-in.

Claims (5)

1. high temperature resistant polyurethane composite gel; It is characterized in that; Material by following parts by weight is formed: 160 parts of toluene, 3.02 parts of 150 parts of methylcarbonates, 587.5 parts of benzoic anhydride polyester polyols, 30 parts of polyphenyl dioctyl phthalate polyol esters, 1.63 parts of TriMethylolPropane(TMP)s, 65 parts of Toluene-2,4-diisocyanate .4-vulcabond, catalyzer CAT S1021.5 part, 1.2 parts of 1.4-butyleneglycols, 1.2 parts of 1.3-butyleneglycols, 0.15 part in oxidation inhibitor and organo-bismuths.
2. according to the said a kind of high temperature resistant polyurethane composite gel of claim 1, it is characterized in that said benzoic anhydride polyester polyol is polymerized by phthalic anhydride, hexanodioic acid and Diethylene Glycol.
3. according to according to the said a kind of high temperature resistant polyurethane binder of claim 1; It is characterized in that said polyphenyl dioctyl phthalate polyol ester is a kind of in polyphenyl dioctyl phthalate propylene glycol ester, polyphenyl dioctyl phthalate 1.3-butanediol ester, polyphenyl dioctyl phthalate 1.4-butanediol ester, the polyphenyl dioctyl phthalate pinakon ester and more than one.
4. according to the said a kind of high temperature resistant polyurethane binder of claim 1, it is characterized in that said oxidation inhibitor is antioxidant 1010.
5. according to the said a kind of high temperature resistant polyurethane binder of claim 1, it is characterized in that said organo-bismuth is an organo-bismuth 8108.
CN2012102287651A 2012-07-04 2012-07-04 High temperature resistant polyurethane complex adhesive Active CN102732205B (en)

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Cited By (3)

* Cited by examiner, † Cited by third party
Publication number Priority date Publication date Assignee Title
CN103865465A (en) * 2012-12-14 2014-06-18 江苏天顺新材料有限公司 Moisture-curing polyurethane hot melt adhesive for automobile lamp and its preparation method
CN106367016A (en) * 2016-08-29 2017-02-01 无锡万能胶粘剂有限公司 Arogel slurry
CN111394044A (en) * 2020-04-16 2020-07-10 上海炼升化工股份有限公司 Fast-curing high-temperature-resistant adhesive and preparation method thereof

Citations (4)

* Cited by examiner, † Cited by third party
Publication number Priority date Publication date Assignee Title
CN1624067A (en) * 2004-10-29 2005-06-08 东华大学 Dry type compound polyurethane adhesive and its preparation method
US20100273008A1 (en) * 2007-11-21 2010-10-28 Sika Technology Ag Polyurethane polymer for reversible adhesive bonds
CN101880516A (en) * 2010-07-05 2010-11-10 广东多正化工科技有限公司 Low free MDI monomer two-component solvent-free polyurethane adhesive
CN102311716A (en) * 2010-07-09 2012-01-11 吴江市亚太高分子化工有限公司 Composite glue and preparation process thereof

Patent Citations (4)

* Cited by examiner, † Cited by third party
Publication number Priority date Publication date Assignee Title
CN1624067A (en) * 2004-10-29 2005-06-08 东华大学 Dry type compound polyurethane adhesive and its preparation method
US20100273008A1 (en) * 2007-11-21 2010-10-28 Sika Technology Ag Polyurethane polymer for reversible adhesive bonds
CN101880516A (en) * 2010-07-05 2010-11-10 广东多正化工科技有限公司 Low free MDI monomer two-component solvent-free polyurethane adhesive
CN102311716A (en) * 2010-07-09 2012-01-11 吴江市亚太高分子化工有限公司 Composite glue and preparation process thereof

Cited By (3)

* Cited by examiner, † Cited by third party
Publication number Priority date Publication date Assignee Title
CN103865465A (en) * 2012-12-14 2014-06-18 江苏天顺新材料有限公司 Moisture-curing polyurethane hot melt adhesive for automobile lamp and its preparation method
CN106367016A (en) * 2016-08-29 2017-02-01 无锡万能胶粘剂有限公司 Arogel slurry
CN111394044A (en) * 2020-04-16 2020-07-10 上海炼升化工股份有限公司 Fast-curing high-temperature-resistant adhesive and preparation method thereof

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