CN111808415A - Polyurethane film for protective clothing and preparation method thereof - Google Patents

Polyurethane film for protective clothing and preparation method thereof Download PDF

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Publication number
CN111808415A
CN111808415A CN202010679617.6A CN202010679617A CN111808415A CN 111808415 A CN111808415 A CN 111808415A CN 202010679617 A CN202010679617 A CN 202010679617A CN 111808415 A CN111808415 A CN 111808415A
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CN
China
Prior art keywords
parts
flame retardant
polyurethane
protective clothing
polyurethane film
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Pending
Application number
CN202010679617.6A
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Chinese (zh)
Inventor
吴明辉
林一速
汤国开
Current Assignee (The listed assignees may be inaccurate. Google has not performed a legal analysis and makes no representation or warranty as to the accuracy of the list.)
Fujian Hengan Hygiene Material Co ltd
Hengan Jinjiang Household Products Co ltd
Hengan Fujian Holding Group Co Ltd
Original Assignee
Fujian Hengan Hygiene Material Co ltd
Hengan Jinjiang Household Products Co ltd
Hengan Fujian Holding Group Co Ltd
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Application filed by Fujian Hengan Hygiene Material Co ltd, Hengan Jinjiang Household Products Co ltd, Hengan Fujian Holding Group Co Ltd filed Critical Fujian Hengan Hygiene Material Co ltd
Priority to CN202010679617.6A priority Critical patent/CN111808415A/en
Publication of CN111808415A publication Critical patent/CN111808415A/en
Pending legal-status Critical Current

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    • CCHEMISTRY; METALLURGY
    • C08ORGANIC MACROMOLECULAR COMPOUNDS; THEIR PREPARATION OR CHEMICAL WORKING-UP; COMPOSITIONS BASED THEREON
    • C08JWORKING-UP; GENERAL PROCESSES OF COMPOUNDING; AFTER-TREATMENT NOT COVERED BY SUBCLASSES C08B, C08C, C08F, C08G or C08H
    • C08J5/00Manufacture of articles or shaped materials containing macromolecular substances
    • C08J5/18Manufacture of films or sheets
    • AHUMAN NECESSITIES
    • A41WEARING APPAREL
    • A41DOUTERWEAR; PROTECTIVE GARMENTS; ACCESSORIES
    • A41D31/00Materials specially adapted for outerwear
    • A41D31/04Materials specially adapted for outerwear characterised by special function or use
    • AHUMAN NECESSITIES
    • A41WEARING APPAREL
    • A41DOUTERWEAR; PROTECTIVE GARMENTS; ACCESSORIES
    • A41D31/00Materials specially adapted for outerwear
    • A41D31/04Materials specially adapted for outerwear characterised by special function or use
    • A41D31/08Heat resistant; Fire retardant
    • AHUMAN NECESSITIES
    • A41WEARING APPAREL
    • A41DOUTERWEAR; PROTECTIVE GARMENTS; ACCESSORIES
    • A41D31/00Materials specially adapted for outerwear
    • A41D31/04Materials specially adapted for outerwear characterised by special function or use
    • A41D31/10Impermeable to liquids, e.g. waterproof; Liquid-repellent
    • CCHEMISTRY; METALLURGY
    • C08ORGANIC MACROMOLECULAR COMPOUNDS; THEIR PREPARATION OR CHEMICAL WORKING-UP; COMPOSITIONS BASED THEREON
    • C08JWORKING-UP; GENERAL PROCESSES OF COMPOUNDING; AFTER-TREATMENT NOT COVERED BY SUBCLASSES C08B, C08C, C08F, C08G or C08H
    • C08J2375/00Characterised by the use of polyureas or polyurethanes; Derivatives of such polymers
    • C08J2375/04Polyurethanes
    • CCHEMISTRY; METALLURGY
    • C08ORGANIC MACROMOLECULAR COMPOUNDS; THEIR PREPARATION OR CHEMICAL WORKING-UP; COMPOSITIONS BASED THEREON
    • C08JWORKING-UP; GENERAL PROCESSES OF COMPOUNDING; AFTER-TREATMENT NOT COVERED BY SUBCLASSES C08B, C08C, C08F, C08G or C08H
    • C08J2425/00Characterised by the use of homopolymers or copolymers of compounds having one or more unsaturated aliphatic radicals, each having only one carbon-to-carbon double bond, and at least one being terminated by an aromatic carbocyclic ring; Derivatives of such polymers
    • C08J2425/02Homopolymers or copolymers of hydrocarbons
    • C08J2425/04Homopolymers or copolymers of styrene
    • C08J2425/06Polystyrene
    • CCHEMISTRY; METALLURGY
    • C08ORGANIC MACROMOLECULAR COMPOUNDS; THEIR PREPARATION OR CHEMICAL WORKING-UP; COMPOSITIONS BASED THEREON
    • C08KUse of inorganic or non-macromolecular organic substances as compounding ingredients
    • C08K13/00Use of mixtures of ingredients not covered by one single of the preceding main groups, each of these compounds being essential
    • C08K13/02Organic and inorganic ingredients
    • CCHEMISTRY; METALLURGY
    • C08ORGANIC MACROMOLECULAR COMPOUNDS; THEIR PREPARATION OR CHEMICAL WORKING-UP; COMPOSITIONS BASED THEREON
    • C08KUse of inorganic or non-macromolecular organic substances as compounding ingredients
    • C08K3/00Use of inorganic substances as compounding ingredients
    • C08K3/18Oxygen-containing compounds, e.g. metal carbonyls
    • C08K3/20Oxides; Hydroxides
    • C08K3/22Oxides; Hydroxides of metals
    • C08K2003/2217Oxides; Hydroxides of metals of magnesium
    • C08K2003/2224Magnesium hydroxide
    • CCHEMISTRY; METALLURGY
    • C08ORGANIC MACROMOLECULAR COMPOUNDS; THEIR PREPARATION OR CHEMICAL WORKING-UP; COMPOSITIONS BASED THEREON
    • C08KUse of inorganic or non-macromolecular organic substances as compounding ingredients
    • C08K2201/00Specific properties of additives
    • C08K2201/011Nanostructured additives
    • CCHEMISTRY; METALLURGY
    • C08ORGANIC MACROMOLECULAR COMPOUNDS; THEIR PREPARATION OR CHEMICAL WORKING-UP; COMPOSITIONS BASED THEREON
    • C08KUse of inorganic or non-macromolecular organic substances as compounding ingredients
    • C08K3/00Use of inorganic substances as compounding ingredients
    • C08K3/34Silicon-containing compounds
    • C08K3/36Silica
    • CCHEMISTRY; METALLURGY
    • C08ORGANIC MACROMOLECULAR COMPOUNDS; THEIR PREPARATION OR CHEMICAL WORKING-UP; COMPOSITIONS BASED THEREON
    • C08KUse of inorganic or non-macromolecular organic substances as compounding ingredients
    • C08K5/00Use of organic ingredients
    • C08K5/02Halogenated hydrocarbons
    • C08K5/03Halogenated hydrocarbons aromatic, e.g. C6H5-CH2-Cl
    • CCHEMISTRY; METALLURGY
    • C08ORGANIC MACROMOLECULAR COMPOUNDS; THEIR PREPARATION OR CHEMICAL WORKING-UP; COMPOSITIONS BASED THEREON
    • C08KUse of inorganic or non-macromolecular organic substances as compounding ingredients
    • C08K5/00Use of organic ingredients
    • C08K5/49Phosphorus-containing compounds
    • C08K5/51Phosphorus bound to oxygen
    • C08K5/52Phosphorus bound to oxygen only
    • C08K5/521Esters of phosphoric acids, e.g. of H3PO4
    • CCHEMISTRY; METALLURGY
    • C08ORGANIC MACROMOLECULAR COMPOUNDS; THEIR PREPARATION OR CHEMICAL WORKING-UP; COMPOSITIONS BASED THEREON
    • C08KUse of inorganic or non-macromolecular organic substances as compounding ingredients
    • C08K5/00Use of organic ingredients
    • C08K5/49Phosphorus-containing compounds
    • C08K5/51Phosphorus bound to oxygen
    • C08K5/52Phosphorus bound to oxygen only
    • C08K5/521Esters of phosphoric acids, e.g. of H3PO4
    • C08K5/523Esters of phosphoric acids, e.g. of H3PO4 with hydroxyaryl compounds

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  • Engineering & Computer Science (AREA)
  • Textile Engineering (AREA)
  • Chemical & Material Sciences (AREA)
  • Manufacturing & Machinery (AREA)
  • Materials Engineering (AREA)
  • Health & Medical Sciences (AREA)
  • Chemical Kinetics & Catalysis (AREA)
  • Medicinal Chemistry (AREA)
  • Polymers & Plastics (AREA)
  • Organic Chemistry (AREA)
  • Compositions Of Macromolecular Compounds (AREA)
  • Treatments For Attaching Organic Compounds To Fibrous Goods (AREA)

Abstract

The invention relates to a polyurethane film for protective clothing and a preparation method thereof, wherein the polyurethane film comprises the following components: 15-35 parts of waterborne polyurethane, 5-10 parts of brominated flame retardant, 2-5 parts of phosphorus flame retardant, 15-25 parts of coupling agent, 5-10 parts of lubricant, 4-6 parts of flatting agent, 10-15 parts of filler and 3-4 parts of stripping aid. According to the preparation method of the polyurethane film for the protective clothing, the waterborne polyurethane, the brominated flame retardant and the phosphorus flame retardant are mixed and stirred, the waterproof performance of the protective clothing is improved by utilizing the waterborne polyurethane, the flame retardance of the protective clothing can be better improved by adding the brominated flame retardant and the phosphorus flame retardant, in addition, the filler is nano alumina, the hardness is high, the size stability is good, or the nano silica can improve the ageing resistance, the strength and the chemical resistance of other materials, and the wear resistance and the flame retardance of the polyurethane film can be further improved.

Description

Polyurethane film for protective clothing and preparation method thereof
Technical Field
The invention relates to the technical field of polyurethane film preparation, in particular to a preparation method of a polyurethane film for protective clothing.
Background
The protective clothing types include fire-fighting protective clothing, industrial protective clothing, medical protective clothing, military protective clothing and protective clothing used by special people. The protective clothing is mainly applied to the industries and departments of fire fighting, military industry, ships, petroleum, chemical industry, paint spraying, cleaning and disinfection, laboratories and the like.
Polyurethane appears in the 30 s of the 20 th century, and through the technical development of nearly eighty years, the material is widely applied to the fields of home furnishing, buildings, daily necessities, traffic, household appliances and the like. The polyurethane can play a role in protection, wherein the three-proofing means moisture resistance, corrosion resistance and salt mist resistance.
The invention discloses an outer-layer fabric of a thermal insulation protective suit for a fireman and a manufacturing method thereof, wherein the outer-layer fabric of the thermal insulation protective suit for the fireman is formed by sequentially coating an aluminum adhesive A and an aluminum adhesive B on the outer surface of aramid fiber 1313, wherein the application number of the outer-layer fabric is 201310438014.7, and the outer-layer fabric of the thermal insulation protective suit for the fireman is as follows: the aluminum adhesive A comprises the following raw materials in parts by mass: 100 parts of oil-based polyurethane, 5-10 parts of an adhesive, 20-30 parts of a cyclized phosphate flame retardant, 15-20 parts of butanone and 4-8 parts of aluminum powder, wherein the aluminum adhesive B comprises the following raw materials in parts by weight: 100 parts of oil-based polyurethane, 5-10 parts of adhesive, 20-30 parts of cyclized phosphate flame retardant, 20-30 parts of butanone and 7-10 parts of aluminum powder. The fabric can effectively reflect high-temperature heat radiation heat, has good moisture permeability, and has excellent flame retardance. However, the firefighter uniform disclosed by the patent is poor in waterproof performance.
The polyurethane film is mostly used when the protective clothing on the market is produced, and as for taking the fire-fighting protective clothing, the polyurethane film on the existing fire-fighting protective clothing can not be better flame-retardant, waterproof and wear-resistant when in use.
Disclosure of Invention
The invention aims to provide a polyurethane film for protective clothing and a preparation method thereof, and aims to solve the problems in the background art.
In order to achieve the purpose, the invention provides the following technical scheme: a preparation method of a polyurethane film for protective clothing comprises the following components: 15-35 parts of waterborne polyurethane, 5-10 parts of brominated flame retardant, 2-5 parts of phosphorus flame retardant, 15-25 parts of coupling agent, 5-10 parts of lubricant, 4-6 parts of flatting agent, 10-15 parts of filler and 3-4 parts of stripping aid.
Preferably, the water-based polyurethane comprises 15 parts of water-based polyurethane, 5 parts of brominated flame retardant, 2 parts of phosphorus flame retardant, 15 parts of coupling agent, 5 parts of lubricant, 4 parts of leveling agent, 10 parts of filler and 3 parts of stripping aid.
Preferably, the water-based polyurethane comprises 25 parts of water-based polyurethane, 7 parts of brominated flame retardant, 4 parts of phosphorus flame retardant, 20 parts of coupling agent, 8 parts of lubricant, 5 parts of leveling agent, 12 parts of filler and 5 parts of stripping aid.
Preferably, the water-based polyurethane comprises 35 parts of water-based polyurethane, 10 parts of brominated flame retardant, 5 parts of phosphorus flame retardant, 25 parts of coupling agent, 10 parts of lubricant, 6 parts of leveling agent, 15 parts of filler and 4 parts of stripping aid.
Preferably, the bromine-based flame retardant is decabromodiphenylethane 8010 or brominated polystyrene; the phosphorus flame retardant is one or two of diphenyl phosphate, trimethyl phosphate, tricresyl phosphate and triisobutyl phosphate.
Preferably, the filler is nano-alumina or nano-silica.
A preparation method of a polyurethane film for protective clothing comprises the following steps:
s1: the materials are weighed and proportioned, then the waterborne polyurethane, the brominated flame retardant and the phosphorus flame retardant are mixed and stirred, then the coupling agent, the lubricating agent, the leveling agent, the filling agent and the stripping aid are sequentially added and mixed, and the polyurethane particles are obtained after the polyurethane particles pass through an extruder after the polyurethane particles are completely reacted;
s2: and (4) putting the polyurethane particles obtained in the step S1 into a calender, then leading out the polyurethane particles through a leading-out roller, and cooling and winding the polyurethane particles to obtain the polyurethane film.
Compared with the prior art, the invention has the beneficial effects that: according to the preparation method of the polyurethane film for the protective clothing, the waterborne polyurethane, the brominated flame retardant and the phosphorus flame retardant are mixed and stirred, the waterproof performance of the protective clothing is improved by utilizing the waterborne polyurethane, the flame retardance of the protective clothing can be better improved by adding the brominated flame retardant and the phosphorus flame retardant, in addition, the filler is nano alumina, the hardness is high, the size stability is good, or the nano silica can improve the ageing resistance, the strength and the chemical resistance of other materials, and the wear resistance and the flame retardance of the polyurethane film can be further improved.
Detailed Description
The technical solutions in the embodiments of the present invention are clearly and completely described, and it is obvious that the described embodiments are only a part of the embodiments of the present invention, and not all embodiments. All other embodiments, which can be derived by a person skilled in the art from the embodiments given herein without making any creative effort, shall fall within the protection scope of the present invention.
Example 1
A polyurethane film for protective clothing comprises the following components: 15 parts of waterborne polyurethane, 5 parts of brominated flame retardant, 2 parts of phosphorus flame retardant, 15 parts of coupling agent, 5 parts of lubricant, 4 parts of leveling agent, 10 parts of filler and 3 parts of stripping aid.
Wherein the bromine flame retardant is decabromodiphenylethane 8010 or brominated polystyrene; the phosphorus flame retardant is one or two of diphenyl phosphate, trimethyl phosphate, tricresyl phosphate and triisobutyl phosphate, and the filler is nano-alumina or nano-silica.
The preparation method of the polyurethane film for the protective clothing comprises the following steps:
s1: the materials are weighed and proportioned, then the waterborne polyurethane, the brominated flame retardant and the phosphorus flame retardant are mixed and stirred, then the coupling agent, the lubricating agent, the leveling agent, the filling agent and the stripping aid are sequentially added and mixed, and the polyurethane particles are obtained after the polyurethane particles pass through an extruder after the polyurethane particles are completely reacted;
s2: and (4) putting the polyurethane particles obtained in the step S1 into a calender, then leading out the polyurethane particles through a leading-out roller, and cooling and winding the polyurethane particles to obtain the polyurethane film.
Example 2
A polyurethane film for protective clothing comprises the following components: 25 parts of waterborne polyurethane, 7 parts of brominated flame retardant, 4 parts of phosphorus flame retardant, 20 parts of coupling agent, 8 parts of lubricant, 5 parts of flatting agent, 12 parts of filler and 5 parts of stripping aid.
Wherein the bromine flame retardant is decabromodiphenylethane 8010 or brominated polystyrene; the phosphorus flame retardant is one or two of diphenyl phosphate, trimethyl phosphate, tricresyl phosphate and triisobutyl phosphate, and the filler is nano-alumina or nano-silica.
The preparation method of the polyurethane film for the protective clothing comprises the following steps:
s1: the materials are weighed and proportioned, then the waterborne polyurethane, the brominated flame retardant and the phosphorus flame retardant are mixed and stirred, then the coupling agent, the lubricating agent, the leveling agent, the filling agent and the stripping aid are sequentially added and mixed, and the polyurethane particles are obtained after the polyurethane particles pass through an extruder after the polyurethane particles are completely reacted;
s2: and (4) putting the polyurethane particles obtained in the step S1 into a calender, then leading out the polyurethane particles through a leading-out roller, and cooling and winding the polyurethane particles to obtain the polyurethane film.
Example 3
A polyurethane film for protective clothing comprises the following components: 35 parts of waterborne polyurethane, 10 parts of brominated flame retardant, 5 parts of phosphorus flame retardant, 25 parts of coupling agent, 10 parts of lubricant, 6 parts of flatting agent, 15 parts of filler and 4 parts of stripping aid.
Wherein the bromine flame retardant is decabromodiphenylethane 8010 or brominated polystyrene; the phosphorus flame retardant is one or two of diphenyl phosphate, trimethyl phosphate, tricresyl phosphate and triisobutyl phosphate, and the filler is nano-alumina or nano-silica.
The preparation method of the polyurethane film for the protective clothing comprises the following steps:
s1: the materials are weighed and proportioned, then the waterborne polyurethane, the brominated flame retardant and the phosphorus flame retardant are mixed and stirred, then the coupling agent, the lubricating agent, the leveling agent, the filling agent and the stripping aid are sequentially added and mixed, and the polyurethane particles are obtained after the polyurethane particles pass through an extruder after the polyurethane particles are completely reacted;
s2: and (4) putting the polyurethane particles obtained in the step S1 into a calender, then leading out the polyurethane particles through a leading-out roller, and cooling and winding the polyurethane particles to obtain the polyurethane film.
Although the present invention has been described in detail with reference to the foregoing embodiments, it will be apparent to those skilled in the art that various changes in the embodiments and/or modifications of the invention can be made, and equivalents and modifications of some features of the invention can be made without departing from the spirit and scope of the invention.

Claims (7)

1. A polyurethane film for protective clothing, comprising: comprises the following components: 15-35 parts of waterborne polyurethane, 5-10 parts of brominated flame retardant, 2-5 parts of phosphorus flame retardant, 15-25 parts of coupling agent, 5-10 parts of lubricant, 4-6 parts of flatting agent, 10-15 parts of filler and 3-4 parts of stripping aid.
2. The polyurethane film for protective clothing according to claim 1, wherein: 15 parts of waterborne polyurethane, 5 parts of brominated flame retardant, 2 parts of phosphorus flame retardant, 15 parts of coupling agent, 5 parts of lubricant, 4 parts of leveling agent, 10 parts of filler and 3 parts of stripping aid.
3. The polyurethane film for protective clothing according to claim 1, wherein: 25 parts of waterborne polyurethane, 7 parts of brominated flame retardant, 4 parts of phosphorus flame retardant, 20 parts of coupling agent, 8 parts of lubricant, 5 parts of flatting agent, 12 parts of filler and 5 parts of stripping aid.
4. The polyurethane film for protective clothing according to claim 1, wherein: 35 parts of waterborne polyurethane, 10 parts of brominated flame retardant, 5 parts of phosphorus flame retardant, 25 parts of coupling agent, 10 parts of lubricant, 6 parts of flatting agent, 15 parts of filler and 4 parts of stripping aid.
5. The polyurethane film for protective clothing according to claim 1, wherein: the brominated flame retardant is decabromodiphenylethane 8010 or brominated polystyrene; the phosphorus flame retardant is one or two of diphenyl phosphate, trimethyl phosphate, tricresyl phosphate and triisobutyl phosphate.
6. The polyurethane film for protective clothing according to claim 1, wherein: the filler is nano-alumina or nano-silica.
7. A method for producing the polyurethane film for protective clothing according to any one of claims 1 to 6, characterized in that: the method comprises the following steps:
s1: the materials are weighed and proportioned, then the waterborne polyurethane, the brominated flame retardant and the phosphorus flame retardant are mixed and stirred, then the coupling agent, the lubricating agent, the leveling agent, the filling agent and the stripping aid are sequentially added and mixed, and the polyurethane particles are obtained after the polyurethane particles pass through an extruder after the polyurethane particles are completely reacted;
s2: and (4) putting the polyurethane particles obtained in the step S1 into a calender, then leading out the polyurethane particles through a leading-out roller, and cooling and winding the polyurethane particles to obtain the polyurethane film.
CN202010679617.6A 2020-07-15 2020-07-15 Polyurethane film for protective clothing and preparation method thereof Pending CN111808415A (en)

Priority Applications (1)

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Cited By (2)

* Cited by examiner, † Cited by third party
Publication number Priority date Publication date Assignee Title
CN113072805A (en) * 2021-03-16 2021-07-06 浙江洛克新材料股份有限公司 TPU film for protective clothing
CN116253984A (en) * 2022-09-09 2023-06-13 深圳市金露兴科技有限公司 Sealing strip and production process thereof

Citations (4)

* Cited by examiner, † Cited by third party
Publication number Priority date Publication date Assignee Title
CN103556470A (en) * 2013-09-24 2014-02-05 江苏南纬悦达纺织研究院有限公司 External layer fabric of heat insulation protective clothing for firefighter and manufacturing method thereof
CN103865250A (en) * 2014-04-03 2014-06-18 昆山金有利新材料科技有限公司 Fireproof polyurethane film and preparation method thereof
CN103881362A (en) * 2014-04-03 2014-06-25 昆山金有利新材料科技有限公司 Waterproof breathable polyurethane film and preparation method thereof
US20160245451A1 (en) * 2014-02-27 2016-08-25 Sekisui Chemical Co., Ltd. Fire-resistant heat-insulating coating material for piping or equipment

Patent Citations (4)

* Cited by examiner, † Cited by third party
Publication number Priority date Publication date Assignee Title
CN103556470A (en) * 2013-09-24 2014-02-05 江苏南纬悦达纺织研究院有限公司 External layer fabric of heat insulation protective clothing for firefighter and manufacturing method thereof
US20160245451A1 (en) * 2014-02-27 2016-08-25 Sekisui Chemical Co., Ltd. Fire-resistant heat-insulating coating material for piping or equipment
CN103865250A (en) * 2014-04-03 2014-06-18 昆山金有利新材料科技有限公司 Fireproof polyurethane film and preparation method thereof
CN103881362A (en) * 2014-04-03 2014-06-25 昆山金有利新材料科技有限公司 Waterproof breathable polyurethane film and preparation method thereof

Cited By (2)

* Cited by examiner, † Cited by third party
Publication number Priority date Publication date Assignee Title
CN113072805A (en) * 2021-03-16 2021-07-06 浙江洛克新材料股份有限公司 TPU film for protective clothing
CN116253984A (en) * 2022-09-09 2023-06-13 深圳市金露兴科技有限公司 Sealing strip and production process thereof

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Application publication date: 20201023

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