DK2473584T3 - Fraktioneringsfri fremgangsmåde til fremstilling af brændstof med lavt kogepunkt fra råolie eller fraktioner deraf - Google Patents

Fraktioneringsfri fremgangsmåde til fremstilling af brændstof med lavt kogepunkt fra råolie eller fraktioner deraf Download PDF

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DK2473584T3
DK2473584T3 DK10812466.0T DK10812466T DK2473584T3 DK 2473584 T3 DK2473584 T3 DK 2473584T3 DK 10812466 T DK10812466 T DK 10812466T DK 2473584 T3 DK2473584 T3 DK 2473584T3
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gas
crude oil
liquid
approx
reaction vessel
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DK10812466.0T
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Rudolf W Gunnerman
Peter W Gunnerman
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Rudolf W Gunnerman
Peter W Gunnerman
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Priority claimed from US12/551,264 external-priority patent/US7806947B2/en
Priority claimed from US12/651,592 external-priority patent/US8226817B2/en
Application filed by Rudolf W Gunnerman, Peter W Gunnerman filed Critical Rudolf W Gunnerman
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Publication of DK2473584T3 publication Critical patent/DK2473584T3/da

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    • C—CHEMISTRY; METALLURGY
    • C10—PETROLEUM, GAS OR COKE INDUSTRIES; TECHNICAL GASES CONTAINING CARBON MONOXIDE; FUELS; LUBRICANTS; PEAT
    • C10L—FUELS NOT OTHERWISE PROVIDED FOR; NATURAL GAS; SYNTHETIC NATURAL GAS OBTAINED BY PROCESSES NOT COVERED BY SUBCLASSES C10G OR C10K; LIQUIFIED PETROLEUM GAS; USE OF ADDITIVES TO FUELS OR FIRES; FIRE-LIGHTERS
    • C10L1/00—Liquid carbonaceous fuels
    • C10L1/04—Liquid carbonaceous fuels essentially based on blends of hydrocarbons
    • B—PERFORMING OPERATIONS; TRANSPORTING
    • B01—PHYSICAL OR CHEMICAL PROCESSES OR APPARATUS IN GENERAL
    • B01J—CHEMICAL OR PHYSICAL PROCESSES, e.g. CATALYSIS OR COLLOID CHEMISTRY; THEIR RELEVANT APPARATUS
    • B01J23/00—Catalysts comprising metals or metal oxides or hydroxides, not provided for in group B01J21/00
    • B01J23/70—Catalysts comprising metals or metal oxides or hydroxides, not provided for in group B01J21/00 of the iron group metals or copper
    • B01J23/76—Catalysts comprising metals or metal oxides or hydroxides, not provided for in group B01J21/00 of the iron group metals or copper combined with metals, oxides or hydroxides provided for in groups B01J23/02 - B01J23/36
    • B01J23/84—Catalysts comprising metals or metal oxides or hydroxides, not provided for in group B01J21/00 of the iron group metals or copper combined with metals, oxides or hydroxides provided for in groups B01J23/02 - B01J23/36 with arsenic, antimony, bismuth, vanadium, niobium, tantalum, polonium, chromium, molybdenum, tungsten, manganese, technetium or rhenium
    • B01J23/889—Manganese, technetium or rhenium
    • B01J23/8892—Manganese
    • C—CHEMISTRY; METALLURGY
    • C10—PETROLEUM, GAS OR COKE INDUSTRIES; TECHNICAL GASES CONTAINING CARBON MONOXIDE; FUELS; LUBRICANTS; PEAT
    • C10G—CRACKING HYDROCARBON OILS; PRODUCTION OF LIQUID HYDROCARBON MIXTURES, e.g. BY DESTRUCTIVE HYDROGENATION, OLIGOMERISATION, POLYMERISATION; RECOVERY OF HYDROCARBON OILS FROM OIL-SHALE, OIL-SAND, OR GASES; REFINING MIXTURES MAINLY CONSISTING OF HYDROCARBONS; REFORMING OF NAPHTHA; MINERAL WAXES
    • C10G11/00—Catalytic cracking, in the absence of hydrogen, of hydrocarbon oils
    • C—CHEMISTRY; METALLURGY
    • C10—PETROLEUM, GAS OR COKE INDUSTRIES; TECHNICAL GASES CONTAINING CARBON MONOXIDE; FUELS; LUBRICANTS; PEAT
    • C10G—CRACKING HYDROCARBON OILS; PRODUCTION OF LIQUID HYDROCARBON MIXTURES, e.g. BY DESTRUCTIVE HYDROGENATION, OLIGOMERISATION, POLYMERISATION; RECOVERY OF HYDROCARBON OILS FROM OIL-SHALE, OIL-SAND, OR GASES; REFINING MIXTURES MAINLY CONSISTING OF HYDROCARBONS; REFORMING OF NAPHTHA; MINERAL WAXES
    • C10G11/00—Catalytic cracking, in the absence of hydrogen, of hydrocarbon oils
    • C10G11/10—Catalytic cracking, in the absence of hydrogen, of hydrocarbon oils with stationary catalyst bed
    • C—CHEMISTRY; METALLURGY
    • C10—PETROLEUM, GAS OR COKE INDUSTRIES; TECHNICAL GASES CONTAINING CARBON MONOXIDE; FUELS; LUBRICANTS; PEAT
    • C10G—CRACKING HYDROCARBON OILS; PRODUCTION OF LIQUID HYDROCARBON MIXTURES, e.g. BY DESTRUCTIVE HYDROGENATION, OLIGOMERISATION, POLYMERISATION; RECOVERY OF HYDROCARBON OILS FROM OIL-SHALE, OIL-SAND, OR GASES; REFINING MIXTURES MAINLY CONSISTING OF HYDROCARBONS; REFORMING OF NAPHTHA; MINERAL WAXES
    • C10G15/00—Cracking of hydrocarbon oils by electric means, electromagnetic or mechanical vibrations, by particle radiation or with gases superheated in electric arcs
    • C10G15/08—Cracking of hydrocarbon oils by electric means, electromagnetic or mechanical vibrations, by particle radiation or with gases superheated in electric arcs by electric means or by electromagnetic or mechanical vibrations
    • C—CHEMISTRY; METALLURGY
    • C10—PETROLEUM, GAS OR COKE INDUSTRIES; TECHNICAL GASES CONTAINING CARBON MONOXIDE; FUELS; LUBRICANTS; PEAT
    • C10G—CRACKING HYDROCARBON OILS; PRODUCTION OF LIQUID HYDROCARBON MIXTURES, e.g. BY DESTRUCTIVE HYDROGENATION, OLIGOMERISATION, POLYMERISATION; RECOVERY OF HYDROCARBON OILS FROM OIL-SHALE, OIL-SAND, OR GASES; REFINING MIXTURES MAINLY CONSISTING OF HYDROCARBONS; REFORMING OF NAPHTHA; MINERAL WAXES
    • C10G29/00—Refining of hydrocarbon oils, in the absence of hydrogen, with other chemicals
    • C10G29/20—Organic compounds not containing metal atoms
    • C10G29/205—Organic compounds not containing metal atoms by reaction with hydrocarbons added to the hydrocarbon oil
    • C—CHEMISTRY; METALLURGY
    • C10—PETROLEUM, GAS OR COKE INDUSTRIES; TECHNICAL GASES CONTAINING CARBON MONOXIDE; FUELS; LUBRICANTS; PEAT
    • C10G—CRACKING HYDROCARBON OILS; PRODUCTION OF LIQUID HYDROCARBON MIXTURES, e.g. BY DESTRUCTIVE HYDROGENATION, OLIGOMERISATION, POLYMERISATION; RECOVERY OF HYDROCARBON OILS FROM OIL-SHALE, OIL-SAND, OR GASES; REFINING MIXTURES MAINLY CONSISTING OF HYDROCARBONS; REFORMING OF NAPHTHA; MINERAL WAXES
    • C10G49/00—Treatment of hydrocarbon oils, in the presence of hydrogen or hydrogen-generating compounds, not provided for in a single one of groups C10G45/02, C10G45/32, C10G45/44, C10G45/58 or C10G47/00
    • C10G49/007—Treatment of hydrocarbon oils, in the presence of hydrogen or hydrogen-generating compounds, not provided for in a single one of groups C10G45/02, C10G45/32, C10G45/44, C10G45/58 or C10G47/00 in the presence of hydrogen from a special source or of a special composition or having been purified by a special treatment
    • C—CHEMISTRY; METALLURGY
    • C10—PETROLEUM, GAS OR COKE INDUSTRIES; TECHNICAL GASES CONTAINING CARBON MONOXIDE; FUELS; LUBRICANTS; PEAT
    • C10G—CRACKING HYDROCARBON OILS; PRODUCTION OF LIQUID HYDROCARBON MIXTURES, e.g. BY DESTRUCTIVE HYDROGENATION, OLIGOMERISATION, POLYMERISATION; RECOVERY OF HYDROCARBON OILS FROM OIL-SHALE, OIL-SAND, OR GASES; REFINING MIXTURES MAINLY CONSISTING OF HYDROCARBONS; REFORMING OF NAPHTHA; MINERAL WAXES
    • C10G49/00—Treatment of hydrocarbon oils, in the presence of hydrogen or hydrogen-generating compounds, not provided for in a single one of groups C10G45/02, C10G45/32, C10G45/44, C10G45/58 or C10G47/00
    • C10G49/02—Treatment of hydrocarbon oils, in the presence of hydrogen or hydrogen-generating compounds, not provided for in a single one of groups C10G45/02, C10G45/32, C10G45/44, C10G45/58 or C10G47/00 characterised by the catalyst used
    • C10G49/04—Treatment of hydrocarbon oils, in the presence of hydrogen or hydrogen-generating compounds, not provided for in a single one of groups C10G45/02, C10G45/32, C10G45/44, C10G45/58 or C10G47/00 characterised by the catalyst used containing nickel, cobalt, chromium, molybdenum, or tungsten metals, or compounds thereof
    • B—PERFORMING OPERATIONS; TRANSPORTING
    • B01—PHYSICAL OR CHEMICAL PROCESSES OR APPARATUS IN GENERAL
    • B01J—CHEMICAL OR PHYSICAL PROCESSES, e.g. CATALYSIS OR COLLOID CHEMISTRY; THEIR RELEVANT APPARATUS
    • B01J35/00—Catalysts, in general, characterised by their form or physical properties
    • B01J35/50—Catalysts, in general, characterised by their form or physical properties characterised by their shape or configuration
    • B01J35/58—Fabrics or filaments
    • C—CHEMISTRY; METALLURGY
    • C10—PETROLEUM, GAS OR COKE INDUSTRIES; TECHNICAL GASES CONTAINING CARBON MONOXIDE; FUELS; LUBRICANTS; PEAT
    • C10G—CRACKING HYDROCARBON OILS; PRODUCTION OF LIQUID HYDROCARBON MIXTURES, e.g. BY DESTRUCTIVE HYDROGENATION, OLIGOMERISATION, POLYMERISATION; RECOVERY OF HYDROCARBON OILS FROM OIL-SHALE, OIL-SAND, OR GASES; REFINING MIXTURES MAINLY CONSISTING OF HYDROCARBONS; REFORMING OF NAPHTHA; MINERAL WAXES
    • C10G2300/00—Aspects relating to hydrocarbon processing covered by groups C10G1/00 - C10G99/00
    • C10G2300/10—Feedstock materials
    • C10G2300/1025—Natural gas
    • C—CHEMISTRY; METALLURGY
    • C10—PETROLEUM, GAS OR COKE INDUSTRIES; TECHNICAL GASES CONTAINING CARBON MONOXIDE; FUELS; LUBRICANTS; PEAT
    • C10G—CRACKING HYDROCARBON OILS; PRODUCTION OF LIQUID HYDROCARBON MIXTURES, e.g. BY DESTRUCTIVE HYDROGENATION, OLIGOMERISATION, POLYMERISATION; RECOVERY OF HYDROCARBON OILS FROM OIL-SHALE, OIL-SAND, OR GASES; REFINING MIXTURES MAINLY CONSISTING OF HYDROCARBONS; REFORMING OF NAPHTHA; MINERAL WAXES
    • C10G2300/00—Aspects relating to hydrocarbon processing covered by groups C10G1/00 - C10G99/00
    • C10G2300/10—Feedstock materials
    • C10G2300/1037—Hydrocarbon fractions
    • C10G2300/104—Light gasoline having a boiling range of about 20 - 100 °C
    • C—CHEMISTRY; METALLURGY
    • C10—PETROLEUM, GAS OR COKE INDUSTRIES; TECHNICAL GASES CONTAINING CARBON MONOXIDE; FUELS; LUBRICANTS; PEAT
    • C10G—CRACKING HYDROCARBON OILS; PRODUCTION OF LIQUID HYDROCARBON MIXTURES, e.g. BY DESTRUCTIVE HYDROGENATION, OLIGOMERISATION, POLYMERISATION; RECOVERY OF HYDROCARBON OILS FROM OIL-SHALE, OIL-SAND, OR GASES; REFINING MIXTURES MAINLY CONSISTING OF HYDROCARBONS; REFORMING OF NAPHTHA; MINERAL WAXES
    • C10G2300/00—Aspects relating to hydrocarbon processing covered by groups C10G1/00 - C10G99/00
    • C10G2300/10—Feedstock materials
    • C10G2300/1037—Hydrocarbon fractions
    • C10G2300/1044—Heavy gasoline or naphtha having a boiling range of about 100 - 180 °C
    • C—CHEMISTRY; METALLURGY
    • C10—PETROLEUM, GAS OR COKE INDUSTRIES; TECHNICAL GASES CONTAINING CARBON MONOXIDE; FUELS; LUBRICANTS; PEAT
    • C10G—CRACKING HYDROCARBON OILS; PRODUCTION OF LIQUID HYDROCARBON MIXTURES, e.g. BY DESTRUCTIVE HYDROGENATION, OLIGOMERISATION, POLYMERISATION; RECOVERY OF HYDROCARBON OILS FROM OIL-SHALE, OIL-SAND, OR GASES; REFINING MIXTURES MAINLY CONSISTING OF HYDROCARBONS; REFORMING OF NAPHTHA; MINERAL WAXES
    • C10G2300/00—Aspects relating to hydrocarbon processing covered by groups C10G1/00 - C10G99/00
    • C10G2300/10—Feedstock materials
    • C10G2300/1037—Hydrocarbon fractions
    • C10G2300/1048—Middle distillates
    • C10G2300/1051—Kerosene having a boiling range of about 180 - 230 °C
    • C—CHEMISTRY; METALLURGY
    • C10—PETROLEUM, GAS OR COKE INDUSTRIES; TECHNICAL GASES CONTAINING CARBON MONOXIDE; FUELS; LUBRICANTS; PEAT
    • C10G—CRACKING HYDROCARBON OILS; PRODUCTION OF LIQUID HYDROCARBON MIXTURES, e.g. BY DESTRUCTIVE HYDROGENATION, OLIGOMERISATION, POLYMERISATION; RECOVERY OF HYDROCARBON OILS FROM OIL-SHALE, OIL-SAND, OR GASES; REFINING MIXTURES MAINLY CONSISTING OF HYDROCARBONS; REFORMING OF NAPHTHA; MINERAL WAXES
    • C10G2300/00—Aspects relating to hydrocarbon processing covered by groups C10G1/00 - C10G99/00
    • C10G2300/10—Feedstock materials
    • C10G2300/1037—Hydrocarbon fractions
    • C10G2300/1048—Middle distillates
    • C10G2300/1055—Diesel having a boiling range of about 230 - 330 °C
    • C—CHEMISTRY; METALLURGY
    • C10—PETROLEUM, GAS OR COKE INDUSTRIES; TECHNICAL GASES CONTAINING CARBON MONOXIDE; FUELS; LUBRICANTS; PEAT
    • C10G—CRACKING HYDROCARBON OILS; PRODUCTION OF LIQUID HYDROCARBON MIXTURES, e.g. BY DESTRUCTIVE HYDROGENATION, OLIGOMERISATION, POLYMERISATION; RECOVERY OF HYDROCARBON OILS FROM OIL-SHALE, OIL-SAND, OR GASES; REFINING MIXTURES MAINLY CONSISTING OF HYDROCARBONS; REFORMING OF NAPHTHA; MINERAL WAXES
    • C10G2300/00—Aspects relating to hydrocarbon processing covered by groups C10G1/00 - C10G99/00
    • C10G2300/10—Feedstock materials
    • C10G2300/1037—Hydrocarbon fractions
    • C10G2300/1048—Middle distillates
    • C10G2300/1059—Gasoil having a boiling range of about 330 - 427 °C
    • C—CHEMISTRY; METALLURGY
    • C10—PETROLEUM, GAS OR COKE INDUSTRIES; TECHNICAL GASES CONTAINING CARBON MONOXIDE; FUELS; LUBRICANTS; PEAT
    • C10G—CRACKING HYDROCARBON OILS; PRODUCTION OF LIQUID HYDROCARBON MIXTURES, e.g. BY DESTRUCTIVE HYDROGENATION, OLIGOMERISATION, POLYMERISATION; RECOVERY OF HYDROCARBON OILS FROM OIL-SHALE, OIL-SAND, OR GASES; REFINING MIXTURES MAINLY CONSISTING OF HYDROCARBONS; REFORMING OF NAPHTHA; MINERAL WAXES
    • C10G2300/00—Aspects relating to hydrocarbon processing covered by groups C10G1/00 - C10G99/00
    • C10G2300/40—Characteristics of the process deviating from typical ways of processing
    • C10G2300/4006—Temperature

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  • Chemical & Material Sciences (AREA)
  • Oil, Petroleum & Natural Gas (AREA)
  • Engineering & Computer Science (AREA)
  • Organic Chemistry (AREA)
  • Chemical Kinetics & Catalysis (AREA)
  • General Chemical & Material Sciences (AREA)
  • Physics & Mathematics (AREA)
  • Electromagnetism (AREA)
  • Materials Engineering (AREA)
  • Mechanical Engineering (AREA)
  • Production Of Liquid Hydrocarbon Mixture For Refining Petroleum (AREA)
  • Catalysts (AREA)
  • Fats And Perfumes (AREA)

Claims (13)

1. Fremgangsmåde til fremstilling af et flydende brændstof fra en gas, der indeholder mindst ca. 50 vol.-% methan, hvilken fremgangsmåde omfatter: (a) at bringe gassen i kontakt med (i) et flydende råmateriale, der består af råolie eller en flydende petroleumsfraktion og (ii) et metallisk katalysatorgitter, hvilke flydende råmateriale og metalliske katalysatorgitter er indeholdt i en reaktionsbeholder ved en temperatur på ca. 80 °C eller derover, men under kogepunktet for råolien, hvilket metalliske katalysatorgitter omfatter vindinger af et overgangsmetal, der er understøttet på en jernramme; (b) at udvinde et gasformigt reaktionsprodukt der er dannet i reaktionsbeholderen; og (c) at kondensere det gasformige reaktionsprodukt til det flydende brændsel.
2. Fremgangsmåden ifølge krav 1, hvor gassen er naturgas
3. Fremgangsmåden ifølge krav 1, hvor gassen er naturgas, og det flydende råmateriale er råolie eller dieselolie.
4. Fremgangsmåden ifølge krav 1, hvor det flydende råmaterialet optager en del af reaktionsbeholderen og derved danner et væskeniveau i reaktionsbeholderen og et hovedrum over væskeniveauet, hvor det metalliske katalysatorgitter befinder sig i hovedrummet, trin (a) omfatter tilførsel af gassen til reaktionsbeholder under væskeniveauet, og trin (b) omfatter genvinding af det gasformige reaktionsprodukt fra hovedrummet.
5. Fremgangsmåden ifølge krav 1, hvor trin (a) udføres ved en temperatur på fra ca. 150 °C til ca. 200 °C og et tryk på fra ca. 1 atmosfære til ca. 1,5 atmosfærer.
6. Fremgangsmåden ifølge krav 1, hvor rammen er cirkulær i yderdiameter med forstærkningsstænger eller stænger inden for omkredsen, og vindingerne konvergerer i midten af rammen.
7. Fremgangsmåden ifølge krav 1, hvor vindingerne er af flere overgangsmetaller, herunder cobalt, nikkel, wolfram, chrom og aluminium på en jernramme.
8. Fremgangsmåden ifølge krav 1, hvor gassen defineres som en første gas, hvilket gasformigt reaktionsprodukt defineres som et første gasformigt reaktionsprodukt, og det flydende brændsel defineres som et første kondensat; hvilken fremgangsmåde yderligere omfatter: (b) at føre en anden gas der indeholder mindst ca. 50 vol.-% methan gennem det første kondensat og et metallisk katalysatorgitter, hvilke første kondensat og metalliske katalysatorgitter er indeholdt i en anden reaktionsbeholder med det første kondensat ved en temperatur på ca. 80 °C eller derover, men under kogetemperaturen af det første kondensat, hvilket metalliske katalysatorgitter omfatter vindinger af et overgangsmetal, der er understøttet på en jernramme; (c) at udvinde et andet gasformigt reaktionsprodukt fra den anden reaktionsbeholder; (d) at kondensere det andet gasformige reaktionsprodukt for at danne det flydende brændsel.
9. Fremgangsmåden ifølge krav 8, hvor det flydende råmaterialet er råolie, og den første gas og den anden gas begge er naturgas.
10. Fremgangsmåde til transport af råolie gennem en rørledning, hvilken fremgangsmåde omfatter: (a) at kontakte en gas der indeholder mindst ca. 50 vol.-% methan med (i) et flydende råmateriale, der består af råolie eller en flydende petroleumsfraktion og (ii) et metallisk katalysatorgitter, hvilke flydende råmateriale og metalliske katalysatorgitter er indeholdt i en reaktionsbeholder ved en temperatur på ca. 80 °C eller derover, men under kogepunktet for råolien, hvilket metalkatalysatorgitter omfatter vindinger af et overgangsmetal, der er understøttet på en jernramme; (b) at udvinde et gasformigt reaktionsprodukt der er dannet i reaktionsbeholderen; og (c) at kondensere det gasformige reaktionsprodukt til det flydende brændsel; (d) at blande råolien med det resulterende flydende brændsel for at danne en blanding og (e) at pumpe blandingen gennem rørledningen.
11. Fremgangsmåden ifølge krav 10, hvor det flydende råmateriale er råolie, og gassen er naturgas.
12. Fremgangsmåden ifølge krav 10, hvor trin (d) udføres ved en temperatur på fra ca. 150 °C til ca. 200 °C og et tryk på fra ca. 1 atmosfære til ca. 1,5 atmosfærer.
13. Fremgangsmåden ifølge krav 10, hvor katalysatoren omfatter vindinger af cobalt, nikkel, wolfram, chrom og aluminium på en jernramme.
DK10812466.0T 2009-08-31 2010-07-27 Fraktioneringsfri fremgangsmåde til fremstilling af brændstof med lavt kogepunkt fra råolie eller fraktioner deraf DK2473584T3 (da)

Applications Claiming Priority (3)

Application Number Priority Date Filing Date Title
US12/551,264 US7806947B2 (en) 2009-08-31 2009-08-31 Liquid hydrocarbon fuel from methane assisted by spontaneously generated voltage
US12/651,592 US8226817B2 (en) 2010-01-04 2010-01-04 Non-fractionation process for production of low-boiling fuel from crude oil
PCT/US2010/043351 WO2011025613A1 (en) 2009-08-31 2010-07-27 Non-fractionation process for production of low-boiling fuel from crude oil or fractions thereof

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DK2473584T3 true DK2473584T3 (da) 2019-03-11

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EP (1) EP2473584B1 (da)
JP (1) JP2013503239A (da)
CN (1) CN102597184A (da)
AR (1) AR077989A1 (da)
AU (1) AU2010286906A1 (da)
BR (1) BR112012004429A2 (da)
CA (1) CA2771576C (da)
CO (1) CO6440517A2 (da)
DK (1) DK2473584T3 (da)
ES (1) ES2710849T3 (da)
HR (1) HRP20190276T1 (da)
HU (1) HUE042729T2 (da)
MX (1) MX2012002487A (da)
PL (1) PL2473584T3 (da)
PT (1) PT2473584T (da)
RU (1) RU2012112065A (da)
SI (1) SI2473584T1 (da)
TR (1) TR201902099T4 (da)
WO (1) WO2011025613A1 (da)

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US8226817B2 (en) 2010-01-04 2012-07-24 Gunnerman Rudolf W Non-fractionation process for production of low-boiling fuel from crude oil
CA2995805A1 (en) 2014-08-20 2016-02-25 Nexcrude Technologies, Inc. Methods for separating light fractions from hydrocarbon feedstock
DE102020114494A1 (de) 2020-05-29 2021-12-02 Vng Ag Kraftstoffmischung mit verbesserter CO2- Bilanz
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CA2771576C (en) 2019-09-17
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