EP2583338A4 - Binder für eine sekundärbatterie zur bereitstellung hervorragender zykluseigenschaften - Google Patents

Binder für eine sekundärbatterie zur bereitstellung hervorragender zykluseigenschaften

Info

Publication number
EP2583338A4
EP2583338A4 EP11795923.9A EP11795923A EP2583338A4 EP 2583338 A4 EP2583338 A4 EP 2583338A4 EP 11795923 A EP11795923 A EP 11795923A EP 2583338 A4 EP2583338 A4 EP 2583338A4
Authority
EP
European Patent Office
Prior art keywords
binder
secondary battery
excellent cycle
cycle property
swelling index
Prior art date
Legal status (The legal status is an assumption and is not a legal conclusion. Google has not performed a legal analysis and makes no representation as to the accuracy of the status listed.)
Granted
Application number
EP11795923.9A
Other languages
English (en)
French (fr)
Other versions
EP2583338B1 (de
EP2583338A2 (de
Inventor
Ok Sun Kim
Young-Min Kim
Minah Kang
Current Assignee (The listed assignees may be inaccurate. Google has not performed a legal analysis and makes no representation or warranty as to the accuracy of the list.)
LG Chem Ltd
Original Assignee
LG Chem Ltd
Priority date (The priority date is an assumption and is not a legal conclusion. Google has not performed a legal analysis and makes no representation as to the accuracy of the date listed.)
Filing date
Publication date
Application filed by LG Chem Ltd filed Critical LG Chem Ltd
Priority to PL11795923T priority Critical patent/PL2583338T3/pl
Publication of EP2583338A2 publication Critical patent/EP2583338A2/de
Publication of EP2583338A4 publication Critical patent/EP2583338A4/de
Application granted granted Critical
Publication of EP2583338B1 publication Critical patent/EP2583338B1/de
Active legal-status Critical Current
Anticipated expiration legal-status Critical

Links

Classifications

    • H—ELECTRICITY
    • H01—ELECTRIC ELEMENTS
    • H01M—PROCESSES OR MEANS, e.g. BATTERIES, FOR THE DIRECT CONVERSION OF CHEMICAL ENERGY INTO ELECTRICAL ENERGY
    • H01M4/00—Electrodes
    • H01M4/02—Electrodes composed of, or comprising, active material
    • H01M4/62—Selection of inactive substances as ingredients for active masses, e.g. binders, fillers
    • H01M4/621—Binders
    • H01M4/622—Binders being polymers
    • C—CHEMISTRY; METALLURGY
    • C08—ORGANIC MACROMOLECULAR COMPOUNDS; THEIR PREPARATION OR CHEMICAL WORKING-UP; COMPOSITIONS BASED THEREON
    • C08F—MACROMOLECULAR COMPOUNDS OBTAINED BY REACTIONS ONLY INVOLVING CARBON-TO-CARBON UNSATURATED BONDS
    • C08F212/00—Copolymers of compounds having one or more unsaturated aliphatic radicals, each having only one carbon-to-carbon double bond, and at least one being terminated by an aromatic carbocyclic ring
    • C08F212/02—Monomers containing only one unsaturated aliphatic radical
    • C08F212/04—Monomers containing only one unsaturated aliphatic radical containing one ring
    • C08F212/06—Hydrocarbons
    • C08F212/12—Monomers containing a branched unsaturated aliphatic radical or a ring substituted by an alkyl radical
    • C—CHEMISTRY; METALLURGY
    • C08—ORGANIC MACROMOLECULAR COMPOUNDS; THEIR PREPARATION OR CHEMICAL WORKING-UP; COMPOSITIONS BASED THEREON
    • C08F—MACROMOLECULAR COMPOUNDS OBTAINED BY REACTIONS ONLY INVOLVING CARBON-TO-CARBON UNSATURATED BONDS
    • C08F212/00—Copolymers of compounds having one or more unsaturated aliphatic radicals, each having only one carbon-to-carbon double bond, and at least one being terminated by an aromatic carbocyclic ring
    • C08F212/02—Monomers containing only one unsaturated aliphatic radical
    • C08F212/32—Monomers containing only one unsaturated aliphatic radical containing two or more rings
    • C—CHEMISTRY; METALLURGY
    • C08—ORGANIC MACROMOLECULAR COMPOUNDS; THEIR PREPARATION OR CHEMICAL WORKING-UP; COMPOSITIONS BASED THEREON
    • C08F—MACROMOLECULAR COMPOUNDS OBTAINED BY REACTIONS ONLY INVOLVING CARBON-TO-CARBON UNSATURATED BONDS
    • C08F212/00—Copolymers of compounds having one or more unsaturated aliphatic radicals, each having only one carbon-to-carbon double bond, and at least one being terminated by an aromatic carbocyclic ring
    • C08F212/34—Monomers containing two or more unsaturated aliphatic radicals
    • C08F212/36—Divinylbenzene
    • C—CHEMISTRY; METALLURGY
    • C08—ORGANIC MACROMOLECULAR COMPOUNDS; THEIR PREPARATION OR CHEMICAL WORKING-UP; COMPOSITIONS BASED THEREON
    • C08F—MACROMOLECULAR COMPOUNDS OBTAINED BY REACTIONS ONLY INVOLVING CARBON-TO-CARBON UNSATURATED BONDS
    • C08F220/00—Copolymers of compounds having one or more unsaturated aliphatic radicals, each having only one carbon-to-carbon double bond, and only one being terminated by only one carboxyl radical or a salt, anhydride ester, amide, imide or nitrile thereof
    • C08F220/02—Monocarboxylic acids having less than ten carbon atoms; Derivatives thereof
    • C08F220/10—Esters
    • C08F220/12—Esters of monohydric alcohols or phenols
    • C08F220/16—Esters of monohydric alcohols or phenols of phenols or of alcohols containing two or more carbon atoms
    • C08F220/18—Esters of monohydric alcohols or phenols of phenols or of alcohols containing two or more carbon atoms with acrylic or methacrylic acids
    • C08F220/1804—C4-(meth)acrylate, e.g. butyl (meth)acrylate, isobutyl (meth)acrylate or tert-butyl (meth)acrylate
    • H—ELECTRICITY
    • H01—ELECTRIC ELEMENTS
    • H01M—PROCESSES OR MEANS, e.g. BATTERIES, FOR THE DIRECT CONVERSION OF CHEMICAL ENERGY INTO ELECTRICAL ENERGY
    • H01M10/00—Secondary cells; Manufacture thereof
    • H01M10/05—Accumulators with non-aqueous electrolyte
    • H01M10/052—Li-accumulators
    • H01M10/0525—Rocking-chair batteries, i.e. batteries with lithium insertion or intercalation in both electrodes; Lithium-ion batteries
    • H—ELECTRICITY
    • H01—ELECTRIC ELEMENTS
    • H01M—PROCESSES OR MEANS, e.g. BATTERIES, FOR THE DIRECT CONVERSION OF CHEMICAL ENERGY INTO ELECTRICAL ENERGY
    • H01M4/00—Electrodes
    • H01M4/02—Electrodes composed of, or comprising, active material
    • H01M4/62—Selection of inactive substances as ingredients for active masses, e.g. binders, fillers
    • H01M4/621—Binders
    • C—CHEMISTRY; METALLURGY
    • C08—ORGANIC MACROMOLECULAR COMPOUNDS; THEIR PREPARATION OR CHEMICAL WORKING-UP; COMPOSITIONS BASED THEREON
    • C08F—MACROMOLECULAR COMPOUNDS OBTAINED BY REACTIONS ONLY INVOLVING CARBON-TO-CARBON UNSATURATED BONDS
    • C08F212/00—Copolymers of compounds having one or more unsaturated aliphatic radicals, each having only one carbon-to-carbon double bond, and at least one being terminated by an aromatic carbocyclic ring
    • C08F212/02—Monomers containing only one unsaturated aliphatic radical
    • C08F212/04—Monomers containing only one unsaturated aliphatic radical containing one ring
    • C08F212/06—Hydrocarbons
    • C08F212/08—Styrene
    • C—CHEMISTRY; METALLURGY
    • C08—ORGANIC MACROMOLECULAR COMPOUNDS; THEIR PREPARATION OR CHEMICAL WORKING-UP; COMPOSITIONS BASED THEREON
    • C08F—MACROMOLECULAR COMPOUNDS OBTAINED BY REACTIONS ONLY INVOLVING CARBON-TO-CARBON UNSATURATED BONDS
    • C08F220/00—Copolymers of compounds having one or more unsaturated aliphatic radicals, each having only one carbon-to-carbon double bond, and only one being terminated by only one carboxyl radical or a salt, anhydride ester, amide, imide or nitrile thereof
    • C08F220/02—Monocarboxylic acids having less than ten carbon atoms; Derivatives thereof
    • C08F220/04—Acids; Metal salts or ammonium salts thereof
    • C08F220/06—Acrylic acid; Methacrylic acid; Metal salts or ammonium salts thereof
    • C—CHEMISTRY; METALLURGY
    • C08—ORGANIC MACROMOLECULAR COMPOUNDS; THEIR PREPARATION OR CHEMICAL WORKING-UP; COMPOSITIONS BASED THEREON
    • C08F—MACROMOLECULAR COMPOUNDS OBTAINED BY REACTIONS ONLY INVOLVING CARBON-TO-CARBON UNSATURATED BONDS
    • C08F220/00—Copolymers of compounds having one or more unsaturated aliphatic radicals, each having only one carbon-to-carbon double bond, and only one being terminated by only one carboxyl radical or a salt, anhydride ester, amide, imide or nitrile thereof
    • C08F220/02—Monocarboxylic acids having less than ten carbon atoms; Derivatives thereof
    • C08F220/10—Esters
    • C08F220/12—Esters of monohydric alcohols or phenols
    • C08F220/16—Esters of monohydric alcohols or phenols of phenols or of alcohols containing two or more carbon atoms
    • C08F220/18—Esters of monohydric alcohols or phenols of phenols or of alcohols containing two or more carbon atoms with acrylic or methacrylic acids
    • C08F220/1808—C8-(meth)acrylate, e.g. isooctyl (meth)acrylate or 2-ethylhexyl (meth)acrylate
    • C—CHEMISTRY; METALLURGY
    • C08—ORGANIC MACROMOLECULAR COMPOUNDS; THEIR PREPARATION OR CHEMICAL WORKING-UP; COMPOSITIONS BASED THEREON
    • C08F—MACROMOLECULAR COMPOUNDS OBTAINED BY REACTIONS ONLY INVOLVING CARBON-TO-CARBON UNSATURATED BONDS
    • C08F220/00—Copolymers of compounds having one or more unsaturated aliphatic radicals, each having only one carbon-to-carbon double bond, and only one being terminated by only one carboxyl radical or a salt, anhydride ester, amide, imide or nitrile thereof
    • C08F220/02—Monocarboxylic acids having less than ten carbon atoms; Derivatives thereof
    • C08F220/10—Esters
    • C08F220/40—Esters of unsaturated alcohols, e.g. allyl (meth)acrylate
    • C—CHEMISTRY; METALLURGY
    • C08—ORGANIC MACROMOLECULAR COMPOUNDS; THEIR PREPARATION OR CHEMICAL WORKING-UP; COMPOSITIONS BASED THEREON
    • C08F—MACROMOLECULAR COMPOUNDS OBTAINED BY REACTIONS ONLY INVOLVING CARBON-TO-CARBON UNSATURATED BONDS
    • C08F220/00—Copolymers of compounds having one or more unsaturated aliphatic radicals, each having only one carbon-to-carbon double bond, and only one being terminated by only one carboxyl radical or a salt, anhydride ester, amide, imide or nitrile thereof
    • C08F220/02—Monocarboxylic acids having less than ten carbon atoms; Derivatives thereof
    • C08F220/42—Nitriles
    • C08F220/44—Acrylonitrile
    • H—ELECTRICITY
    • H01—ELECTRIC ELEMENTS
    • H01M—PROCESSES OR MEANS, e.g. BATTERIES, FOR THE DIRECT CONVERSION OF CHEMICAL ENERGY INTO ELECTRICAL ENERGY
    • H01M10/00—Secondary cells; Manufacture thereof
    • H01M10/05—Accumulators with non-aqueous electrolyte
    • H01M10/056—Accumulators with non-aqueous electrolyte characterised by the materials used as electrolytes, e.g. mixed inorganic/organic electrolytes
    • H01M10/0564—Accumulators with non-aqueous electrolyte characterised by the materials used as electrolytes, e.g. mixed inorganic/organic electrolytes the electrolyte being constituted of organic materials only
    • H01M10/0566—Liquid materials
    • H01M10/0567—Liquid materials characterised by the additives
    • H—ELECTRICITY
    • H01—ELECTRIC ELEMENTS
    • H01M—PROCESSES OR MEANS, e.g. BATTERIES, FOR THE DIRECT CONVERSION OF CHEMICAL ENERGY INTO ELECTRICAL ENERGY
    • H01M10/00—Secondary cells; Manufacture thereof
    • H01M10/05—Accumulators with non-aqueous electrolyte
    • H01M10/056—Accumulators with non-aqueous electrolyte characterised by the materials used as electrolytes, e.g. mixed inorganic/organic electrolytes
    • H01M10/0564—Accumulators with non-aqueous electrolyte characterised by the materials used as electrolytes, e.g. mixed inorganic/organic electrolytes the electrolyte being constituted of organic materials only
    • H01M10/0566—Liquid materials
    • H01M10/0569—Liquid materials characterised by the solvents
    • H—ELECTRICITY
    • H01—ELECTRIC ELEMENTS
    • H01M—PROCESSES OR MEANS, e.g. BATTERIES, FOR THE DIRECT CONVERSION OF CHEMICAL ENERGY INTO ELECTRICAL ENERGY
    • H01M4/00—Electrodes
    • H01M4/02—Electrodes composed of, or comprising, active material
    • H01M4/13—Electrodes for accumulators with non-aqueous electrolyte, e.g. for lithium-accumulators; Processes of manufacture thereof
    • H01M4/131—Electrodes based on mixed oxides or hydroxides, or on mixtures of oxides or hydroxides, e.g. LiCoOx
    • H—ELECTRICITY
    • H01—ELECTRIC ELEMENTS
    • H01M—PROCESSES OR MEANS, e.g. BATTERIES, FOR THE DIRECT CONVERSION OF CHEMICAL ENERGY INTO ELECTRICAL ENERGY
    • H01M4/00—Electrodes
    • H01M4/02—Electrodes composed of, or comprising, active material
    • H01M4/13—Electrodes for accumulators with non-aqueous electrolyte, e.g. for lithium-accumulators; Processes of manufacture thereof
    • H01M4/133—Electrodes based on carbonaceous material, e.g. graphite-intercalation compounds or CFx
    • H—ELECTRICITY
    • H01—ELECTRIC ELEMENTS
    • H01M—PROCESSES OR MEANS, e.g. BATTERIES, FOR THE DIRECT CONVERSION OF CHEMICAL ENERGY INTO ELECTRICAL ENERGY
    • H01M4/00—Electrodes
    • H01M4/02—Electrodes composed of, or comprising, active material
    • H01M4/13—Electrodes for accumulators with non-aqueous electrolyte, e.g. for lithium-accumulators; Processes of manufacture thereof
    • H01M4/134—Electrodes based on metals, Si or alloys
    • H—ELECTRICITY
    • H01—ELECTRIC ELEMENTS
    • H01M—PROCESSES OR MEANS, e.g. BATTERIES, FOR THE DIRECT CONVERSION OF CHEMICAL ENERGY INTO ELECTRICAL ENERGY
    • H01M4/00—Electrodes
    • H01M4/02—Electrodes composed of, or comprising, active material
    • H01M4/62—Selection of inactive substances as ingredients for active masses, e.g. binders, fillers
    • H01M4/624—Electric conductive fillers
    • Y—GENERAL TAGGING OF NEW TECHNOLOGICAL DEVELOPMENTS; GENERAL TAGGING OF CROSS-SECTIONAL TECHNOLOGIES SPANNING OVER SEVERAL SECTIONS OF THE IPC; TECHNICAL SUBJECTS COVERED BY FORMER USPC CROSS-REFERENCE ART COLLECTIONS [XRACs] AND DIGESTS
    • Y02—TECHNOLOGIES OR APPLICATIONS FOR MITIGATION OR ADAPTATION AGAINST CLIMATE CHANGE
    • Y02E—REDUCTION OF GREENHOUSE GAS [GHG] EMISSIONS, RELATED TO ENERGY GENERATION, TRANSMISSION OR DISTRIBUTION
    • Y02E60/00—Enabling technologies; Technologies with a potential or indirect contribution to GHG emissions mitigation
    • Y02E60/10—Energy storage using batteries

Landscapes

  • Chemical & Material Sciences (AREA)
  • Chemical Kinetics & Catalysis (AREA)
  • Electrochemistry (AREA)
  • General Chemical & Material Sciences (AREA)
  • Health & Medical Sciences (AREA)
  • Medicinal Chemistry (AREA)
  • Polymers & Plastics (AREA)
  • Organic Chemistry (AREA)
  • Engineering & Computer Science (AREA)
  • Materials Engineering (AREA)
  • Manufacturing & Machinery (AREA)
  • Battery Electrode And Active Subsutance (AREA)
  • Secondary Cells (AREA)
EP11795923.9A 2010-06-16 2011-06-08 Binder für eine sekundärbatterie zur bereitstellung hervorragender zykluseigenschaften Active EP2583338B1 (de)

Priority Applications (1)

Application Number Priority Date Filing Date Title
PL11795923T PL2583338T3 (pl) 2010-06-16 2011-06-08 Środek wiążący do akumulatora, zapewniający doskonale właściwości cyklu

Applications Claiming Priority (2)

Application Number Priority Date Filing Date Title
KR1020100057146A KR101161143B1 (ko) 2010-06-16 2010-06-16 사이클 성능이 우수한 이차전지용 바인더
PCT/KR2011/004180 WO2011159057A2 (en) 2010-06-16 2011-06-08 Binder for secondary battery providing excellent cycle property

Publications (3)

Publication Number Publication Date
EP2583338A2 EP2583338A2 (de) 2013-04-24
EP2583338A4 true EP2583338A4 (de) 2014-01-29
EP2583338B1 EP2583338B1 (de) 2017-03-22

Family

ID=45348715

Family Applications (1)

Application Number Title Priority Date Filing Date
EP11795923.9A Active EP2583338B1 (de) 2010-06-16 2011-06-08 Binder für eine sekundärbatterie zur bereitstellung hervorragender zykluseigenschaften

Country Status (6)

Country Link
US (1) US9543584B2 (de)
EP (1) EP2583338B1 (de)
KR (1) KR101161143B1 (de)
CN (1) CN102939676B (de)
PL (1) PL2583338T3 (de)
WO (1) WO2011159057A2 (de)

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CN104471763B (zh) * 2012-07-11 2017-10-24 株式会社Lg 化学 具有优异胶粘强度和寿命特性的二次电池电极用粘合剂
JP6337554B2 (ja) * 2014-03-24 2018-06-06 日本ゼオン株式会社 非水系二次電池多孔膜用バインダー、非水系二次電池多孔膜用組成物、非水系二次電池用多孔膜および非水系二次電池
PL3136483T3 (pl) * 2014-04-21 2018-12-31 Fujifilm Wako Pure Chemical Corporation Spoiwo dla ogniwa litowego
HUE058910T2 (hu) 2014-06-04 2022-09-28 Zeon Corp Kötõanyag-összetétel lítiumion-akkumulátor elektród-alkalmazáshoz, zagyösszetétel lítiumion-akkumulátor elektród-alkalmazáshoz, elektród lítiumakkumulátor elektród-alkalmazáshoz, és lítiumion-akkumulátor
JP6739350B2 (ja) 2014-07-11 2020-08-12 エルジー・ケム・リミテッド 正極およびその製造方法
CN104362348A (zh) * 2014-11-06 2015-02-18 东莞新能源科技有限公司 一种负极电极膜及应用了该电极膜的锂离子电池
US20180102542A1 (en) * 2015-04-22 2018-04-12 Toagosei Co., Ltd. Binder for nonaqueous electrolyte secondary battery electrode, and use thereof
CN105085777B (zh) * 2015-07-17 2017-12-05 中国石油天然气股份有限公司 一种聚苯乙烯2‑丁烯酸乙酯及其制备方法与应用
WO2017047640A1 (ja) * 2015-09-14 2017-03-23 株式会社大阪ソーダ 非水電解質二次電池用の正極材料
JP6908029B2 (ja) * 2016-04-19 2021-07-21 日本ゼオン株式会社 非水系二次電池機能層用バインダー組成物、非水系二次電池機能層用組成物、非水系二次電池用機能層、非水系二次電池用電池部材および非水系二次電池
CN109565051A (zh) * 2016-07-29 2019-04-02 花王株式会社 蓄电设备电极用树脂组合物
KR102211109B1 (ko) * 2017-09-15 2021-02-02 주식회사 엘지화학 실리콘 전극 바인더
US20190319263A1 (en) * 2018-04-13 2019-10-17 Nanotek Instruments, Inc. Alkali metal-selenium secondary battery containing a cathode of protected selenium
CN112825369B (zh) * 2019-11-20 2022-03-29 珠海冠宇电池股份有限公司 一种高温性能优异的高电压锂离子电池
CN111082062A (zh) * 2019-12-23 2020-04-28 宣城研一新能源科技有限公司 锂离子电池用水溶型粘结剂及其制备方法
KR20220128634A (ko) * 2020-01-10 2022-09-21 솔베이(소시에떼아노님) 적어도 하나의 겔화된 전극을 갖는 전기화학 디바이스
WO2021153376A1 (ja) * 2020-01-31 2021-08-05 日本ゼオン株式会社 全固体電池用バインダー粒子、全固体電池用組成物、全固体電池用機能層、および全固体電池
CN113054193B (zh) * 2021-03-12 2022-05-24 广东工业大学 一种硅基负极自修复聚合物粘结剂及其制备方法和应用
CN119286437B (zh) * 2024-12-11 2025-04-08 深圳好电科技有限公司 一种负极粘结剂、负极片及二次电池

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EP1249882A1 (de) * 1999-09-03 2002-10-16 Zeon Corporation Binder zur verwendung im elektrolyte von lithium-sekundär-zelle und dessen verwendung
WO2006123892A1 (en) * 2005-05-17 2006-11-23 Lg Chem, Ltd. Polymer binder for electrochemcal device comprising multiply stacked electrochemical cells
KR20080062966A (ko) * 2006-12-30 2008-07-03 주식회사 엘지화학 열적 안정성이 우수한 이차전지용 바인더
KR20090017939A (ko) * 2007-08-16 2009-02-19 주식회사 엘지화학 도전성이 우수한 리튬 이온 2차 전지용 바인더 조성물 및이를 포함하는 리튬 이온 2차 전지
WO2011090318A2 (en) * 2010-01-20 2011-07-28 Lg Chem, Ltd. Binder for secondary battery providing excellent adhesion strength and cycle property

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US6756153B1 (en) 1999-01-28 2004-06-29 Zeon Corporation Binder composition for electrode for lithium-ion secondary battery and utilization thereof
JP2000286167A (ja) * 1999-03-29 2000-10-13 Toyota Motor Corp 電池・キャパシタ用電極の製造方法
US6656633B2 (en) * 2000-07-26 2003-12-02 Zeon Corporation Binder for electrode for lithium ion secondary battery, and utilization thereof
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CN101156264B (zh) * 2005-04-07 2011-05-25 Lg化学株式会社 用于锂二次电池的具有优良的倍率特性和长期循环性能的粘合剂
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US8277977B2 (en) * 2007-01-16 2012-10-02 Zeon Corporation Binder composition, slurry for electrodes, electrode and nonaqueous electrolyte secondary battery

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Publication number Priority date Publication date Assignee Title
EP1249882A1 (de) * 1999-09-03 2002-10-16 Zeon Corporation Binder zur verwendung im elektrolyte von lithium-sekundär-zelle und dessen verwendung
WO2006123892A1 (en) * 2005-05-17 2006-11-23 Lg Chem, Ltd. Polymer binder for electrochemcal device comprising multiply stacked electrochemical cells
KR20080062966A (ko) * 2006-12-30 2008-07-03 주식회사 엘지화학 열적 안정성이 우수한 이차전지용 바인더
KR20090017939A (ko) * 2007-08-16 2009-02-19 주식회사 엘지화학 도전성이 우수한 리튬 이온 2차 전지용 바인더 조성물 및이를 포함하는 리튬 이온 2차 전지
WO2011090318A2 (en) * 2010-01-20 2011-07-28 Lg Chem, Ltd. Binder for secondary battery providing excellent adhesion strength and cycle property

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DATABASE WPI Week 200937, Derwent World Patents Index; AN 2009-F82413, XP002717962 *

Also Published As

Publication number Publication date
CN102939676B (zh) 2016-02-10
WO2011159057A2 (en) 2011-12-22
EP2583338B1 (de) 2017-03-22
KR101161143B1 (ko) 2012-06-29
US20130202963A1 (en) 2013-08-08
US9543584B2 (en) 2017-01-10
WO2011159057A3 (en) 2012-04-26
KR20110137109A (ko) 2011-12-22
CN102939676A (zh) 2013-02-20
PL2583338T3 (pl) 2017-08-31
EP2583338A2 (de) 2013-04-24

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