ES2080106T3 - Agente dispersante, su utilizacion y substancias solidas recubiertas con el. - Google Patents

Agente dispersante, su utilizacion y substancias solidas recubiertas con el.

Info

Publication number
ES2080106T3
ES2080106T3 ES90203520T ES90203520T ES2080106T3 ES 2080106 T3 ES2080106 T3 ES 2080106T3 ES 90203520 T ES90203520 T ES 90203520T ES 90203520 T ES90203520 T ES 90203520T ES 2080106 T3 ES2080106 T3 ES 2080106T3
Authority
ES
Spain
Prior art keywords
compounds
dispersing agent
solid substances
dispersants
transformed
Prior art date
Legal status (The legal status is an assumption and is not a legal conclusion. Google has not performed a legal analysis and makes no representation as to the accuracy of the status listed.)
Expired - Lifetime
Application number
ES90203520T
Other languages
English (en)
Inventor
Peter Hermann Quednau
Current Assignee (The listed assignees may be inaccurate. Google has not performed a legal analysis and makes no representation or warranty as to the accuracy of the list.)
Ciba Specialty Chemicals Heerenveen BV
Original Assignee
Efka Chemicals BV
Priority date (The priority date is an assumption and is not a legal conclusion. Google has not performed a legal analysis and makes no representation as to the accuracy of the date listed.)
Filing date
Publication date
Application filed by Efka Chemicals BV filed Critical Efka Chemicals BV
Application granted granted Critical
Publication of ES2080106T3 publication Critical patent/ES2080106T3/es
Anticipated expiration legal-status Critical
Expired - Lifetime legal-status Critical Current

Links

Classifications

    • C—CHEMISTRY; METALLURGY
    • C08—ORGANIC MACROMOLECULAR COMPOUNDS; THEIR PREPARATION OR CHEMICAL WORKING-UP; COMPOSITIONS BASED THEREON
    • C08G—MACROMOLECULAR COMPOUNDS OBTAINED OTHERWISE THAN BY REACTIONS ONLY INVOLVING UNSATURATED CARBON-TO-CARBON BONDS
    • C08G18/00—Polymeric products of isocyanates or isothiocyanates
    • C08G18/06—Polymeric products of isocyanates or isothiocyanates with compounds having active hydrogen
    • C08G18/70—Polymeric products of isocyanates or isothiocyanates with compounds having active hydrogen characterised by the isocyanates or isothiocyanates used
    • C08G18/72—Polyisocyanates or polyisothiocyanates
    • C08G18/77—Polyisocyanates or polyisothiocyanates having heteroatoms in addition to the isocyanate or isothiocyanate nitrogen and oxygen or sulfur
    • C08G18/78—Nitrogen
    • C08G18/79—Nitrogen characterised by the polyisocyanates used, these having groups formed by oligomerisation of isocyanates or isothiocyanates
    • C08G18/791—Nitrogen characterised by the polyisocyanates used, these having groups formed by oligomerisation of isocyanates or isothiocyanates containing isocyanurate groups
    • C08G18/795—Nitrogen characterised by the polyisocyanates used, these having groups formed by oligomerisation of isocyanates or isothiocyanates containing isocyanurate groups formed by oligomerisation of mixtures of aliphatic and/or cycloaliphatic isocyanates or isothiocyanates with aromatic isocyanates or isothiocyanates
    • C—CHEMISTRY; METALLURGY
    • C09—DYES; PAINTS; POLISHES; NATURAL RESINS; ADHESIVES; COMPOSITIONS NOT OTHERWISE PROVIDED FOR; APPLICATIONS OF MATERIALS NOT OTHERWISE PROVIDED FOR
    • C09K—MATERIALS FOR MISCELLANEOUS APPLICATIONS, NOT PROVIDED FOR ELSEWHERE
    • C09K23/00—Use of substances as emulsifying, wetting, dispersing, or foam-producing agents
    • C—CHEMISTRY; METALLURGY
    • C08—ORGANIC MACROMOLECULAR COMPOUNDS; THEIR PREPARATION OR CHEMICAL WORKING-UP; COMPOSITIONS BASED THEREON
    • C08G—MACROMOLECULAR COMPOUNDS OBTAINED OTHERWISE THAN BY REACTIONS ONLY INVOLVING UNSATURATED CARBON-TO-CARBON BONDS
    • C08G18/00—Polymeric products of isocyanates or isothiocyanates
    • C08G18/06—Polymeric products of isocyanates or isothiocyanates with compounds having active hydrogen
    • C08G18/08—Processes
    • C08G18/10—Prepolymer processes involving reaction of isocyanates or isothiocyanates with compounds having active hydrogen in a first reaction step
    • C—CHEMISTRY; METALLURGY
    • C08—ORGANIC MACROMOLECULAR COMPOUNDS; THEIR PREPARATION OR CHEMICAL WORKING-UP; COMPOSITIONS BASED THEREON
    • C08G—MACROMOLECULAR COMPOUNDS OBTAINED OTHERWISE THAN BY REACTIONS ONLY INVOLVING UNSATURATED CARBON-TO-CARBON BONDS
    • C08G18/00—Polymeric products of isocyanates or isothiocyanates
    • C08G18/06—Polymeric products of isocyanates or isothiocyanates with compounds having active hydrogen
    • C08G18/28—Polymeric products of isocyanates or isothiocyanates with compounds having active hydrogen characterised by the compounds used containing active hydrogen
    • C08G18/2805—Compounds having only one group containing active hydrogen
    • C08G18/2815—Monohydroxy compounds
    • C08G18/283—Compounds containing ether groups, e.g. oxyalkylated monohydroxy compounds
    • C—CHEMISTRY; METALLURGY
    • C08—ORGANIC MACROMOLECULAR COMPOUNDS; THEIR PREPARATION OR CHEMICAL WORKING-UP; COMPOSITIONS BASED THEREON
    • C08G—MACROMOLECULAR COMPOUNDS OBTAINED OTHERWISE THAN BY REACTIONS ONLY INVOLVING UNSATURATED CARBON-TO-CARBON BONDS
    • C08G18/00—Polymeric products of isocyanates or isothiocyanates
    • C08G18/06—Polymeric products of isocyanates or isothiocyanates with compounds having active hydrogen
    • C08G18/28—Polymeric products of isocyanates or isothiocyanates with compounds having active hydrogen characterised by the compounds used containing active hydrogen
    • C08G18/2805—Compounds having only one group containing active hydrogen
    • C08G18/2815—Monohydroxy compounds
    • C08G18/284—Compounds containing ester groups, e.g. oxyalkylated monocarboxylic acids
    • C—CHEMISTRY; METALLURGY
    • C08—ORGANIC MACROMOLECULAR COMPOUNDS; THEIR PREPARATION OR CHEMICAL WORKING-UP; COMPOSITIONS BASED THEREON
    • C08G—MACROMOLECULAR COMPOUNDS OBTAINED OTHERWISE THAN BY REACTIONS ONLY INVOLVING UNSATURATED CARBON-TO-CARBON BONDS
    • C08G18/00—Polymeric products of isocyanates or isothiocyanates
    • C08G18/06—Polymeric products of isocyanates or isothiocyanates with compounds having active hydrogen
    • C08G18/28—Polymeric products of isocyanates or isothiocyanates with compounds having active hydrogen characterised by the compounds used containing active hydrogen
    • C08G18/30—Low-molecular-weight compounds
    • C08G18/38—Low-molecular-weight compounds having heteroatoms other than oxygen
    • C08G18/3819—Low-molecular-weight compounds having heteroatoms other than oxygen having nitrogen
    • C08G18/3821—Carboxylic acids; Esters thereof with monohydroxyl compounds
    • C—CHEMISTRY; METALLURGY
    • C08—ORGANIC MACROMOLECULAR COMPOUNDS; THEIR PREPARATION OR CHEMICAL WORKING-UP; COMPOSITIONS BASED THEREON
    • C08G—MACROMOLECULAR COMPOUNDS OBTAINED OTHERWISE THAN BY REACTIONS ONLY INVOLVING UNSATURATED CARBON-TO-CARBON BONDS
    • C08G18/00—Polymeric products of isocyanates or isothiocyanates
    • C08G18/06—Polymeric products of isocyanates or isothiocyanates with compounds having active hydrogen
    • C08G18/28—Polymeric products of isocyanates or isothiocyanates with compounds having active hydrogen characterised by the compounds used containing active hydrogen
    • C08G18/40—High-molecular-weight compounds
    • C08G18/42—Polycondensates having carboxylic or carbonic ester groups in the main chain
    • C08G18/4263—Polycondensates having carboxylic or carbonic ester groups in the main chain containing carboxylic acid groups
    • C—CHEMISTRY; METALLURGY
    • C08—ORGANIC MACROMOLECULAR COMPOUNDS; THEIR PREPARATION OR CHEMICAL WORKING-UP; COMPOSITIONS BASED THEREON
    • C08G—MACROMOLECULAR COMPOUNDS OBTAINED OTHERWISE THAN BY REACTIONS ONLY INVOLVING UNSATURATED CARBON-TO-CARBON BONDS
    • C08G18/00—Polymeric products of isocyanates or isothiocyanates
    • C08G18/06—Polymeric products of isocyanates or isothiocyanates with compounds having active hydrogen
    • C08G18/28—Polymeric products of isocyanates or isothiocyanates with compounds having active hydrogen characterised by the compounds used containing active hydrogen
    • C08G18/40—High-molecular-weight compounds
    • C08G18/48—Polyethers
    • C08G18/4887—Polyethers containing carboxylic ester groups derived from carboxylic acids other than acids of higher fatty oils or other than resin acids
    • C—CHEMISTRY; METALLURGY
    • C08—ORGANIC MACROMOLECULAR COMPOUNDS; THEIR PREPARATION OR CHEMICAL WORKING-UP; COMPOSITIONS BASED THEREON
    • C08G—MACROMOLECULAR COMPOUNDS OBTAINED OTHERWISE THAN BY REACTIONS ONLY INVOLVING UNSATURATED CARBON-TO-CARBON BONDS
    • C08G18/00—Polymeric products of isocyanates or isothiocyanates
    • C08G18/06—Polymeric products of isocyanates or isothiocyanates with compounds having active hydrogen
    • C08G18/70—Polymeric products of isocyanates or isothiocyanates with compounds having active hydrogen characterised by the isocyanates or isothiocyanates used
    • C08G18/72—Polyisocyanates or polyisothiocyanates
    • C08G18/77—Polyisocyanates or polyisothiocyanates having heteroatoms in addition to the isocyanate or isothiocyanate nitrogen and oxygen or sulfur
    • C08G18/78—Nitrogen
    • C08G18/79—Nitrogen characterised by the polyisocyanates used, these having groups formed by oligomerisation of isocyanates or isothiocyanates
    • C08G18/791—Nitrogen characterised by the polyisocyanates used, these having groups formed by oligomerisation of isocyanates or isothiocyanates containing isocyanurate groups
    • C—CHEMISTRY; METALLURGY
    • C09—DYES; PAINTS; POLISHES; NATURAL RESINS; ADHESIVES; COMPOSITIONS NOT OTHERWISE PROVIDED FOR; APPLICATIONS OF MATERIALS NOT OTHERWISE PROVIDED FOR
    • C09K—MATERIALS FOR MISCELLANEOUS APPLICATIONS, NOT PROVIDED FOR ELSEWHERE
    • C09K23/00—Use of substances as emulsifying, wetting, dispersing, or foam-producing agents
    • C09K23/16—Amines or polyamines
    • Y—GENERAL TAGGING OF NEW TECHNOLOGICAL DEVELOPMENTS; GENERAL TAGGING OF CROSS-SECTIONAL TECHNOLOGIES SPANNING OVER SEVERAL SECTIONS OF THE IPC; TECHNICAL SUBJECTS COVERED BY FORMER USPC CROSS-REFERENCE ART COLLECTIONS [XRACs] AND DIGESTS
    • Y10—TECHNICAL SUBJECTS COVERED BY FORMER USPC
    • Y10S—TECHNICAL SUBJECTS COVERED BY FORMER USPC CROSS-REFERENCE ART COLLECTIONS [XRACs] AND DIGESTS
    • Y10S516/00—Colloid systems and wetting agents; subcombinations thereof; processes of
    • Y10S516/01—Wetting, emulsifying, dispersing, or stabilizing agents

Landscapes

  • Chemical & Material Sciences (AREA)
  • Organic Chemistry (AREA)
  • Medicinal Chemistry (AREA)
  • Health & Medical Sciences (AREA)
  • Chemical Kinetics & Catalysis (AREA)
  • Polymers & Plastics (AREA)
  • Materials Engineering (AREA)
  • Engineering & Computer Science (AREA)
  • Emulsifying, Dispersing, Foam-Producing Or Wetting Agents (AREA)
  • Polyurethanes Or Polyureas (AREA)
  • Solid-Sorbent Or Filter-Aiding Compositions (AREA)
  • Agricultural Chemicals And Associated Chemicals (AREA)
  • Processing Of Solid Wastes (AREA)
  • Detergent Compositions (AREA)

Abstract

LA INVENCION SE REFIERE A DISPERSANTES O SUS SALES, QUE COMPRENDEN: A EL PRODUCTO DE REACCION DE UNO O VARIOS POLIISOCIANATOS CON UNA FUNCIONALIDAD MEDIA DE 2,0 A 5, CON B UNA MEZCLA DE B SUB 1 COMPUESTOS DE MONOHIDROXI, Y B SUB 2 COMPUESTOS DE MONOHIDROXI, COMPUESTOS DE ACIDO MONOCARBOXILICO O COMPUESTOS DE MONOAMINO, COMPUESTOS DEL ACIDO AMONOCARBOXILICO Y C UN COMPUESTO QUE CONTIENE AL MENOS UN NITROGENO ANULAR BASICO ASI COMO UN GRUPO REACTIVO CON ISOCIANATO, TRANSFORMANDOSE DE LOS GRUPOS ISOCIANATOS APROXIMADAMENTE 30-70% CON B Y APROXIMADAMENTE 30-70% CON C, ASI COMO A LA FABRICACION DE TALES DISPERSANTES.
ES90203520T 1989-12-29 1990-12-28 Agente dispersante, su utilizacion y substancias solidas recubiertas con el. Expired - Lifetime ES2080106T3 (es)

Applications Claiming Priority (1)

Application Number Priority Date Filing Date Title
EP89203342 1989-12-29

Publications (1)

Publication Number Publication Date
ES2080106T3 true ES2080106T3 (es) 1996-02-01

Family

ID=8202541

Family Applications (1)

Application Number Title Priority Date Filing Date
ES90203520T Expired - Lifetime ES2080106T3 (es) 1989-12-29 1990-12-28 Agente dispersante, su utilizacion y substancias solidas recubiertas con el.

Country Status (11)

Country Link
US (1) US5399294A (es)
EP (1) EP0438836B1 (es)
JP (1) JP3101824B2 (es)
KR (1) KR0185379B1 (es)
AT (1) ATE128155T1 (es)
CA (1) CA2032992C (es)
DE (1) DE59009688D1 (es)
DK (1) DK0438836T3 (es)
ES (1) ES2080106T3 (es)
GR (1) GR3017463T3 (es)
NL (1) NL188095C (es)

Families Citing this family (51)

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US5425900A (en) * 1990-12-27 1995-06-20 Efka-Chemicals B.V. Dispersing agents, their use and solids coated therewith
ES2095389T3 (es) * 1991-06-26 1997-02-16 Efka Chemicals Bv Agentes dispersantes, su utilizacion y solidos recubiertos con estos.
DE19732251B4 (de) * 1997-07-26 2004-07-29 Byk-Chemie Gmbh Versalzungsprodukte von Polyaminen und deren Einsatz als Dispergiermittel für Pigmente und Füllstoffe
DE19810660A1 (de) 1998-03-12 1999-09-16 Bayer Ag Wäßrige Polyisocyanatvernetzer mit Hydroxypivalinsäure und Dimethylpyrazol-Blockierung
GB9809257D0 (en) † 1998-04-30 1998-07-01 Zeneca Ltd Polyurethane dispersants
DE19919482C2 (de) * 1999-04-29 2001-04-26 Byk Chemie Gmbh Verfahren zur Herstellung eines Thixotropie-Mittels und dessen Verwendung
US6506899B1 (en) 1999-08-09 2003-01-14 E. I. Du Pont De Nemours And Company Pigment dispersants formed by reacting an isocyanate with a poly (ethylene glycol) alkyl ether, a polyester or polyester or polyacrylate and a diamine
DE10003749A1 (de) * 2000-01-28 2001-08-02 Cognis Deutschland Gmbh Verfahren zur Herstellung radikalisch nachvernetzter Polymere
DE10003940A1 (de) * 2000-01-29 2001-08-02 Cognis Deutschland Gmbh Verfahren zur Herstellung radikalisch nachverentzter Polymere unter Einsatz von Aufbaukomponenten
DE10003938A1 (de) * 2000-01-29 2001-08-02 Cognis Deutschland Gmbh Verfahren zur Herstellung radikalisch nachvernetzter Polymere unter Einsatz von Diallylphthalaten
DE10003939A1 (de) * 2000-01-29 2001-08-02 Cognis Deutschland Gmbh Verfahren zur Herstellung radikalisch nachvernetzter Polymere unter Einsatz von reaktiven Anhydriden
JP2005504140A (ja) * 2001-09-25 2005-02-10 スリーエム イノベイティブ プロパティズ カンパニー 硬化性分散剤
US7276555B2 (en) * 2002-05-21 2007-10-02 Hexion Specialty Chemicals, Inc. Amide-modified resin or hydrocarbyl moiety for dispersing a pigment
DE10302743A1 (de) 2003-01-24 2004-07-29 Goldschmidt Ag Verwendung von Siliconharzen als Dispergiermittel
DE102004022753B3 (de) * 2004-05-07 2006-02-16 Byk-Chemie Gmbh Als Dispergiermittel und Dispersionsstabilisatoren geeignete Additionsverbindungen
MX2007007445A (es) 2004-12-20 2007-11-08 Performance Indicator Llc Formulaciones y objetos con fotoluminiscencia persistente, de alta densidad, y metodos para crearlos.
US7910022B2 (en) 2006-09-15 2011-03-22 Performance Indicator, Llc Phosphorescent compositions for identification
DE102005005846A1 (de) 2005-02-08 2006-08-17 Basf Ag Feste Pigmentzubereitungen, enthaltend wasserlösliche oberflächenaktive Additive auf Polyurethanbasis
JP5175098B2 (ja) 2005-08-03 2013-04-03 株式会社Ｄｎｐファインケミカル 重合体組成物の製造方法および重合体組成物
WO2007057326A1 (en) * 2005-11-17 2007-05-24 Ciba Holding Inc. Process for the preparation of a dry powder of a polymeric additive
JP5042241B2 (ja) * 2006-02-24 2012-10-03 チバ ホールディング インコーポレーテッド 新規なポリウレタン分散剤
DE102006012999A1 (de) * 2006-03-22 2007-09-27 Byk-Chemie Gmbh Additionsverbindungen als Dispergiermittel und Dispersionsstabilisatoren
US7547894B2 (en) 2006-09-15 2009-06-16 Performance Indicator, L.L.C. Phosphorescent compositions and methods for identification using the same
JP4893206B2 (ja) * 2006-09-29 2012-03-07 Ｄｉｃ株式会社 顔料分散剤、顔料ペースト、及び印刷インキ組成物
DE102006062441A1 (de) 2006-12-27 2008-07-03 Byk-Chemie Gmbh Modifizierte Kammcopolymere
JP5123539B2 (ja) * 2007-03-06 2013-01-23 大日精化工業株式会社 共重合体およびその使用
US8039193B2 (en) 2007-09-13 2011-10-18 Performance Indicator Llc Tissue markings and methods for reversibly marking tissue employing the same
US7842128B2 (en) 2007-09-13 2010-11-30 Performance Indicatior LLC Tissue marking compositions
DE102008010687B4 (de) 2008-02-22 2014-05-15 Byk-Chemie Gmbh Netz- und Dispergiermittel, deren Herstellung und Verwendung
DE102008045296A1 (de) 2008-09-02 2010-03-04 Byk-Chemie Gmbh Monocarbonsäureester enthaltendes Dispergiermedium für Feststoffpräparationen
JP5317908B2 (ja) * 2008-09-30 2013-10-16 サカタインクス株式会社 カラーフィルター用顔料分散物およびそれを含有するカラーフィルター用顔料分散レジスト組成物
IT1404805B1 (it) 2011-02-10 2013-11-29 Lamberti Spa Disperdenti
DE102012000414B4 (de) 2012-01-12 2014-03-20 Thyssenkrupp Rasselstein Gmbh Verfahren zur Passivierung von Weißblech, sowie verzinntes Stahlband oder -blech
CN102658057B (zh) * 2012-04-16 2014-09-10 王志军 一种新型聚氨酯分散剂及其制备方法
WO2014030310A1 (ja) 2012-08-23 2014-02-27 バンドー化学株式会社 導電性ペースト
WO2015065829A1 (en) 2013-11-01 2015-05-07 Lubrizol Advanced Materials, Inc. Dispersants with multiple aromatic imide anchor groups
PL3131962T3 (pl) 2014-04-15 2018-09-28 Byk-Chemie Gmbh Kompozycja do regulowania właściwości reologicznych
WO2015197648A1 (de) 2014-06-24 2015-12-30 Byk-Chemie Gmbh Acrylat-systeme mit latenter verdickungsneigung
WO2015197647A1 (de) 2014-06-24 2015-12-30 Byk-Chemie Gmbh Epoxidharz-epoxidhärter-systeme mit latenter verdickungsneigung
US10392494B2 (en) 2014-06-24 2019-08-27 Byk-Chemie Gmbh Latent thickeners, rheology control kit and multi-component systems
KR20170026511A (ko) 2014-06-24 2017-03-08 비와이케이-케미 게엠베하 잠복성 증점 경향이 있는 폴리우레탄 이성분 또는 다성분 시스템
WO2015197646A1 (de) 2014-06-24 2015-12-30 Byk-Chemie Gmbh Ungesättigte polyesterharz-systeme mit latenter verdickungsneigung
CN105170019B (zh) * 2015-07-31 2018-03-23 泰山玻璃纤维有限公司 一种阳离子型聚氨酯大分子多子表面活性剂的制备方法
JP7090399B2 (ja) 2017-02-21 2022-06-24 日本ペイント・オートモーティブコーティングス株式会社 水性塗料組成物および複層塗膜
EP3938454A4 (en) 2019-03-12 2022-11-16 Huntsman Petrochemical LLC ISOCYANATES AND AMINES DISPERSING AGENTS
CN114127150A (zh) * 2019-07-18 2022-03-01 巴斯夫欧洲公司 脲基甲酸酯基分散剂
EP4296056A1 (en) 2021-02-22 2023-12-27 Nippon Paint Automotive Coatings Co., Ltd. Multi-layer coating film
JP7340306B1 (ja) 2023-03-28 2023-09-07 サカタインクス株式会社 光硬化型インクジェット印刷用インク組成物
JP2025025656A (ja) 2023-08-10 2025-02-21 サカタインクス株式会社 光硬化型インクジェット印刷用インク組成物
JP2025025657A (ja) 2023-08-10 2025-02-21 サカタインクス株式会社 光硬化型インクジェット印刷用インク組成物
EP4692250A1 (en) 2024-08-05 2026-02-11 Sakata INX Corporation Active-energy-ray-curable inkjet ink composition

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US3684771A (en) * 1971-03-03 1972-08-15 Du Pont Polyesters with substituted amine end groups
US3817944A (en) * 1972-04-05 1974-06-18 Du Pont Polyesters with acid end groups
US4032698A (en) * 1973-02-02 1977-06-28 E. I. Du Pont De Nemours And Company Polymeric materials with substituted urea end groups
US4070388A (en) * 1975-10-14 1978-01-24 E. I. Du Pont De Nemours And Company Polymeric materials with acid end groups
EP0154678B2 (de) * 1984-01-27 1998-12-09 Byk-Chemie GmbH Als Dispergiermittel geeignete Additionsverbindungen, Verfahren zu ihrer Herstellung, ihre Verwendung und damit beschichtete Feststoffe
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EP0535224A1 (en) * 1987-06-26 1993-04-07 Nippon Oil And Fats Company, Limited Pigment dispersant
US4942213A (en) * 1987-12-04 1990-07-17 Byk-Chemie Gmbh Addition compounds useful as dispersing agents and dispersion stabilizers, process for producing them, their use and solids coated therewith

Also Published As

Publication number Publication date
KR0185379B1 (ko) 1999-04-15
KR910011332A (ko) 1991-08-07
US5399294A (en) 1995-03-21
JP3101824B2 (ja) 2000-10-23
DK0438836T3 (da) 1996-02-05
EP0438836B1 (de) 1995-09-20
EP0438836A1 (de) 1991-07-31
NL188095C (nl) 1992-04-01
GR3017463T3 (en) 1995-12-31
CA2032992A1 (en) 1991-06-30
NL9002892A (nl) 1991-07-16
DE59009688D1 (de) 1995-10-26
NL188095B (nl) 1991-11-01
JPH04210220A (ja) 1992-07-31
CA2032992C (en) 2001-04-10
ATE128155T1 (de) 1995-10-15

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