FR3143634B1 - Interconnecteur pour empilement de cellules à oxydes solides de type SOEC/SOFC comportant une couche de contact ajourée - Google Patents

Interconnecteur pour empilement de cellules à oxydes solides de type SOEC/SOFC comportant une couche de contact ajourée

Info

Publication number
FR3143634B1
FR3143634B1 FR2213927A FR2213927A FR3143634B1 FR 3143634 B1 FR3143634 B1 FR 3143634B1 FR 2213927 A FR2213927 A FR 2213927A FR 2213927 A FR2213927 A FR 2213927A FR 3143634 B1 FR3143634 B1 FR 3143634B1
Authority
FR
France
Prior art keywords
soec
interconnector
contact layer
solid oxide
openwork
Prior art date
Legal status (The legal status is an assumption and is not a legal conclusion. Google has not performed a legal analysis and makes no representation as to the accuracy of the status listed.)
Active
Application number
FR2213927A
Other languages
English (en)
Other versions
FR3143634A1 (fr
Inventor
Karl Vulliez
Iorio Stéphane Di
Manon Elie
Géraldine Palcoux
Current Assignee (The listed assignees may be inaccurate. Google has not performed a legal analysis and makes no representation or warranty as to the accuracy of the list.)
Commissariat a lEnergie Atomique et aux Energies Alternatives CEA
Original Assignee
Commissariat a lEnergie Atomique CEA
Commissariat a lEnergie Atomique et aux Energies Alternatives CEA
Priority date (The priority date is an assumption and is not a legal conclusion. Google has not performed a legal analysis and makes no representation as to the accuracy of the date listed.)
Filing date
Publication date
Application filed by Commissariat a lEnergie Atomique CEA, Commissariat a lEnergie Atomique et aux Energies Alternatives CEA filed Critical Commissariat a lEnergie Atomique CEA
Priority to FR2213927A priority Critical patent/FR3143634B1/fr
Priority to PCT/FR2023/052075 priority patent/WO2024134101A1/fr
Priority to JP2025536837A priority patent/JP2026504339A/ja
Priority to EP23841523.6A priority patent/EP4638834A1/fr
Publication of FR3143634A1 publication Critical patent/FR3143634A1/fr
Application granted granted Critical
Publication of FR3143634B1 publication Critical patent/FR3143634B1/fr
Active legal-status Critical Current
Anticipated expiration legal-status Critical

Links

Classifications

    • C—CHEMISTRY; METALLURGY
    • C25—ELECTROLYTIC OR ELECTROPHORETIC PROCESSES; APPARATUS THEREFOR
    • C25B—ELECTROLYTIC OR ELECTROPHORETIC PROCESSES FOR THE PRODUCTION OF COMPOUNDS OR NON-METALS; APPARATUS THEREFOR
    • C25B9/00—Cells or assemblies of cells; Constructional parts of cells; Assemblies of constructional parts, e.g. electrode-diaphragm assemblies; Process-related cell features
    • C25B9/70—Assemblies comprising two or more cells
    • C25B9/73—Assemblies comprising two or more cells of the filter-press type
    • C25B9/75—Assemblies comprising two or more cells of the filter-press type having bipolar electrodes
    • C—CHEMISTRY; METALLURGY
    • C25—ELECTROLYTIC OR ELECTROPHORETIC PROCESSES; APPARATUS THEREFOR
    • C25B—ELECTROLYTIC OR ELECTROPHORETIC PROCESSES FOR THE PRODUCTION OF COMPOUNDS OR NON-METALS; APPARATUS THEREFOR
    • C25B15/00—Operating or servicing cells
    • C25B15/08—Supplying or removing reactants or electrolytes; Regeneration of electrolytes
    • C—CHEMISTRY; METALLURGY
    • C25—ELECTROLYTIC OR ELECTROPHORETIC PROCESSES; APPARATUS THEREFOR
    • C25B—ELECTROLYTIC OR ELECTROPHORETIC PROCESSES FOR THE PRODUCTION OF COMPOUNDS OR NON-METALS; APPARATUS THEREFOR
    • C25B9/00—Cells or assemblies of cells; Constructional parts of cells; Assemblies of constructional parts, e.g. electrode-diaphragm assemblies; Process-related cell features
    • C25B9/60—Constructional parts of cells
    • C25B9/65—Means for supplying current; Electrode connections; Electric inter-cell connections
    • H—ELECTRICITY
    • H01—ELECTRIC ELEMENTS
    • H01M—PROCESSES OR MEANS, e.g. BATTERIES, FOR THE DIRECT CONVERSION OF CHEMICAL ENERGY INTO ELECTRICAL ENERGY
    • H01M4/00—Electrodes
    • H01M4/86—Inert electrodes with catalytic activity, e.g. for fuel cells
    • H01M4/90—Selection of catalytic material
    • H01M4/9016—Oxides, hydroxides or oxygenated metallic salts
    • H01M4/9025—Oxides specially used in fuel cell operating at high temperature, e.g. SOFC
    • H01M4/9033—Complex oxides, optionally doped, of the type M1MeO3, M1 being an alkaline earth metal or a rare earth, Me being a metal, e.g. perovskites
    • H—ELECTRICITY
    • H01—ELECTRIC ELEMENTS
    • H01M—PROCESSES OR MEANS, e.g. BATTERIES, FOR THE DIRECT CONVERSION OF CHEMICAL ENERGY INTO ELECTRICAL ENERGY
    • H01M8/00—Fuel cells; Manufacture thereof
    • H01M8/02—Details
    • H01M8/0202—Collectors; Separators, e.g. bipolar separators; Interconnectors
    • H01M8/0204—Non-porous and characterised by the material
    • H01M8/0215—Glass; Ceramic materials
    • H01M8/0217—Complex oxides, optionally doped, of the type AMO3, A being an alkaline earth metal or rare earth metal and M being a metal, e.g. perovskites
    • H—ELECTRICITY
    • H01—ELECTRIC ELEMENTS
    • H01M—PROCESSES OR MEANS, e.g. BATTERIES, FOR THE DIRECT CONVERSION OF CHEMICAL ENERGY INTO ELECTRICAL ENERGY
    • H01M8/00—Fuel cells; Manufacture thereof
    • H01M8/02—Details
    • H01M8/0202—Collectors; Separators, e.g. bipolar separators; Interconnectors
    • H01M8/0204—Non-porous and characterised by the material
    • H01M8/0223—Composites
    • H01M8/0228—Composites in the form of layered or coated products
    • H—ELECTRICITY
    • H01—ELECTRIC ELEMENTS
    • H01M—PROCESSES OR MEANS, e.g. BATTERIES, FOR THE DIRECT CONVERSION OF CHEMICAL ENERGY INTO ELECTRICAL ENERGY
    • H01M8/00—Fuel cells; Manufacture thereof
    • H01M8/02—Details
    • H01M8/0202—Collectors; Separators, e.g. bipolar separators; Interconnectors
    • H01M8/0247—Collectors; Separators, e.g. bipolar separators; Interconnectors characterised by the form
    • H—ELECTRICITY
    • H01—ELECTRIC ELEMENTS
    • H01M—PROCESSES OR MEANS, e.g. BATTERIES, FOR THE DIRECT CONVERSION OF CHEMICAL ENERGY INTO ELECTRICAL ENERGY
    • H01M8/00—Fuel cells; Manufacture thereof
    • H01M8/02—Details
    • H01M8/0202—Collectors; Separators, e.g. bipolar separators; Interconnectors
    • H01M8/0247—Collectors; Separators, e.g. bipolar separators; Interconnectors characterised by the form
    • H01M8/0256—Vias, i.e. connectors passing through the separator material
    • H—ELECTRICITY
    • H01—ELECTRIC ELEMENTS
    • H01M—PROCESSES OR MEANS, e.g. BATTERIES, FOR THE DIRECT CONVERSION OF CHEMICAL ENERGY INTO ELECTRICAL ENERGY
    • H01M8/00—Fuel cells; Manufacture thereof
    • H01M8/02—Details
    • H01M8/0202—Collectors; Separators, e.g. bipolar separators; Interconnectors
    • H01M8/0258—Collectors; Separators, e.g. bipolar separators; Interconnectors characterised by the configuration of channels, e.g. by the flow field of the reactant or coolant
    • H—ELECTRICITY
    • H01—ELECTRIC ELEMENTS
    • H01M—PROCESSES OR MEANS, e.g. BATTERIES, FOR THE DIRECT CONVERSION OF CHEMICAL ENERGY INTO ELECTRICAL ENERGY
    • H01M8/00—Fuel cells; Manufacture thereof
    • H01M8/02—Details
    • H01M8/0202—Collectors; Separators, e.g. bipolar separators; Interconnectors
    • H01M8/0258—Collectors; Separators, e.g. bipolar separators; Interconnectors characterised by the configuration of channels, e.g. by the flow field of the reactant or coolant
    • H01M8/026—Collectors; Separators, e.g. bipolar separators; Interconnectors characterised by the configuration of channels, e.g. by the flow field of the reactant or coolant characterised by grooves, e.g. their pitch or depth
    • H—ELECTRICITY
    • H01—ELECTRIC ELEMENTS
    • H01M—PROCESSES OR MEANS, e.g. BATTERIES, FOR THE DIRECT CONVERSION OF CHEMICAL ENERGY INTO ELECTRICAL ENERGY
    • H01M8/00—Fuel cells; Manufacture thereof
    • H01M8/02—Details
    • H01M8/0202—Collectors; Separators, e.g. bipolar separators; Interconnectors
    • H01M8/0258—Collectors; Separators, e.g. bipolar separators; Interconnectors characterised by the configuration of channels, e.g. by the flow field of the reactant or coolant
    • H01M8/0265—Collectors; Separators, e.g. bipolar separators; Interconnectors characterised by the configuration of channels, e.g. by the flow field of the reactant or coolant the reactant or coolant channels having varying cross sections
    • H—ELECTRICITY
    • H01—ELECTRIC ELEMENTS
    • H01M—PROCESSES OR MEANS, e.g. BATTERIES, FOR THE DIRECT CONVERSION OF CHEMICAL ENERGY INTO ELECTRICAL ENERGY
    • H01M8/00—Fuel cells; Manufacture thereof
    • H01M8/24—Grouping of fuel cells, e.g. stacking of fuel cells
    • H01M8/241—Grouping of fuel cells, e.g. stacking of fuel cells with solid or matrix-supported electrolytes
    • H01M8/2425—High-temperature cells with solid electrolytes
    • H01M8/2432—Grouping of unit cells of planar configuration
    • C—CHEMISTRY; METALLURGY
    • C25—ELECTROLYTIC OR ELECTROPHORETIC PROCESSES; APPARATUS THEREFOR
    • C25B—ELECTROLYTIC OR ELECTROPHORETIC PROCESSES FOR THE PRODUCTION OF COMPOUNDS OR NON-METALS; APPARATUS THEREFOR
    • C25B1/00—Electrolytic production of inorganic compounds or non-metals
    • C25B1/01—Products
    • C25B1/02—Hydrogen or oxygen
    • C25B1/04—Hydrogen or oxygen by electrolysis of water
    • C25B1/042—Hydrogen or oxygen by electrolysis of water by electrolysis of steam
    • C—CHEMISTRY; METALLURGY
    • C25—ELECTROLYTIC OR ELECTROPHORETIC PROCESSES; APPARATUS THEREFOR
    • C25B—ELECTROLYTIC OR ELECTROPHORETIC PROCESSES FOR THE PRODUCTION OF COMPOUNDS OR NON-METALS; APPARATUS THEREFOR
    • C25B9/00—Cells or assemblies of cells; Constructional parts of cells; Assemblies of constructional parts, e.g. electrode-diaphragm assemblies; Process-related cell features
    • C25B9/70—Assemblies comprising two or more cells
    • C25B9/73—Assemblies comprising two or more cells of the filter-press type
    • C25B9/77—Assemblies comprising two or more cells of the filter-press type having diaphragms
    • H—ELECTRICITY
    • H01—ELECTRIC ELEMENTS
    • H01M—PROCESSES OR MEANS, e.g. BATTERIES, FOR THE DIRECT CONVERSION OF CHEMICAL ENERGY INTO ELECTRICAL ENERGY
    • H01M8/00—Fuel cells; Manufacture thereof
    • H01M8/10—Fuel cells with solid electrolytes
    • H01M8/12—Fuel cells with solid electrolytes operating at high temperature, e.g. with stabilised ZrO2 electrolyte
    • H01M2008/1293—Fuel cells with solid oxide electrolytes
    • Y—GENERAL TAGGING OF NEW TECHNOLOGICAL DEVELOPMENTS; GENERAL TAGGING OF CROSS-SECTIONAL TECHNOLOGIES SPANNING OVER SEVERAL SECTIONS OF THE IPC; TECHNICAL SUBJECTS COVERED BY FORMER USPC CROSS-REFERENCE ART COLLECTIONS [XRACs] AND DIGESTS
    • Y02—TECHNOLOGIES OR APPLICATIONS FOR MITIGATION OR ADAPTATION AGAINST CLIMATE CHANGE
    • Y02E—REDUCTION OF GREENHOUSE GAS [GHG] EMISSIONS, RELATED TO ENERGY GENERATION, TRANSMISSION OR DISTRIBUTION
    • Y02E60/00—Enabling technologies; Technologies with a potential or indirect contribution to GHG emissions mitigation
    • Y02E60/30—Hydrogen technology
    • Y02E60/50—Fuel cells

Landscapes

  • Chemical & Material Sciences (AREA)
  • Engineering & Computer Science (AREA)
  • Chemical Kinetics & Catalysis (AREA)
  • Electrochemistry (AREA)
  • General Chemical & Material Sciences (AREA)
  • Manufacturing & Machinery (AREA)
  • Sustainable Energy (AREA)
  • Sustainable Development (AREA)
  • Life Sciences & Earth Sciences (AREA)
  • Materials Engineering (AREA)
  • Metallurgy (AREA)
  • Organic Chemistry (AREA)
  • Composite Materials (AREA)
  • Ceramic Engineering (AREA)
  • Fuel Cell (AREA)
  • Electrolytic Production Of Non-Metals, Compounds, Apparatuses Therefor (AREA)

Abstract

L'objet principal de l'invention est un interconnecteur (5) pour un empilement de cellules à oxydes solides de type SOEC/SOFC, destiné à être agencé entre deux cellules électrochimiques adjacentes, formé par l’assemblage d’au moins trois plaques allongées (22, 23) selon des premier et deuxième axes de symétrie, la plaque centrale (22) comportant des lumières (71, 72, 73, 74), chaque lumière comportant des languettes espacées les unes des autres pour former un peigne et des fentes, caractérisé en ce qu’au moins l’une de la première plaque d’extrémité et de la deuxième plaque d’extrémité (23) est recouverte en partie centrale d’une couche de contact (90), dont la surface est supérieure à celle de la partie centrale de la plaque centrale, comportant au moins une lumière de contact (92) allongée sur une longueur (Lc) supérieure à la longueur (Lp) de la partie centrale et formée en superposition d’au moins une lumière (71, 72, 73, 74) de la plaque centrale (22). Figure pour l’abrégé : Figure 5
FR2213927A 2022-12-20 2022-12-20 Interconnecteur pour empilement de cellules à oxydes solides de type SOEC/SOFC comportant une couche de contact ajourée Active FR3143634B1 (fr)

Priority Applications (4)

Application Number Priority Date Filing Date Title
FR2213927A FR3143634B1 (fr) 2022-12-20 2022-12-20 Interconnecteur pour empilement de cellules à oxydes solides de type SOEC/SOFC comportant une couche de contact ajourée
PCT/FR2023/052075 WO2024134101A1 (fr) 2022-12-20 2023-12-20 Interconnecteur pour empilement de cellules à oxydes solides de type soec/sofc comportant une couche de contact ajourée
JP2025536837A JP2026504339A (ja) 2022-12-20 2023-12-20 穿孔された接触層を含むｓｏｅｃ／ｓｏｆｃタイプの固体酸化物セルのスタックのためのインターコネクター
EP23841523.6A EP4638834A1 (fr) 2022-12-20 2023-12-20 Interconnecteur pour empilement de cellules à oxydes solides de type soec/sofc comportant une couche de contact ajourée

Applications Claiming Priority (2)

Application Number Priority Date Filing Date Title
FR2213927 2022-12-20
FR2213927A FR3143634B1 (fr) 2022-12-20 2022-12-20 Interconnecteur pour empilement de cellules à oxydes solides de type SOEC/SOFC comportant une couche de contact ajourée

Publications (2)

Publication Number Publication Date
FR3143634A1 FR3143634A1 (fr) 2024-06-21
FR3143634B1 true FR3143634B1 (fr) 2025-10-10

Family

ID=85685763

Family Applications (1)

Application Number Title Priority Date Filing Date
FR2213927A Active FR3143634B1 (fr) 2022-12-20 2022-12-20 Interconnecteur pour empilement de cellules à oxydes solides de type SOEC/SOFC comportant une couche de contact ajourée

Country Status (4)

Country Link
EP (1) EP4638834A1 (fr)
JP (1) JP2026504339A (fr)
FR (1) FR3143634B1 (fr)
WO (1) WO2024134101A1 (fr)

Family Cites Families (9)

* Cited by examiner, † Cited by third party
Publication number Priority date Publication date Assignee Title
CA2424728A1 (fr) * 2000-11-08 2002-05-16 Global Thermoelectric Inc. Interconnexion pour cellule electrochimique
JP4429571B2 (ja) * 2002-05-31 2010-03-10 本田技研工業株式会社 燃料電池のセパレータ
JP4692001B2 (ja) * 2005-02-08 2011-06-01 トヨタ自動車株式会社 燃料電池のセパレータ
FR2996065B1 (fr) 2012-09-26 2017-02-24 Commissariat Energie Atomique Composant constituant un interconnecteur d'electrolyseur eht ou de pile a combustible sofc et procedes de realisation associes
FR2999612B1 (fr) * 2012-12-17 2015-02-20 Commissariat Energie Atomique Procede d'electrolyse a haute temperature de la vapeur d'eau et d'un autre gaz, interconnecteur, reacteur et procedes de fonctionnement associes
FR3024985B1 (fr) 2014-08-22 2020-01-17 Commissariat A L'energie Atomique Et Aux Energies Alternatives Procede d'electrolyse ou de co-electrolyse a haute temperature, procede de production d'electricite par pile a combustible sofc, interconnecteurs, reacteurs et procedes de fonctionnement associes.
FR3045215B1 (fr) 2015-12-15 2023-03-03 Commissariat Energie Atomique Systeme de serrage autonome d'un empilement a oxydes solides de type soec/sofc a haute temperature
FR3056337B1 (fr) 2016-09-22 2021-01-22 Commissariat Energie Atomique Reacteur d'electrolyse de l'eau (soec) ou pile a combustible (sofc) a taux d'utilisation de vapeur d'eau ou respectivement de combustible augmente
FR3104324B1 (fr) * 2019-12-10 2021-12-03 Commissariat A L Energie Atomique Et Aux Energies Alternatives Procédé de réalisation amélioré d’un composant constituant un interconnecteur d’électrolyseur EHT ou de pile à combustible SOFC.

Also Published As

Publication number Publication date
JP2026504339A (ja) 2026-02-05
FR3143634A1 (fr) 2024-06-21
EP4638834A1 (fr) 2025-10-29
WO2024134101A1 (fr) 2024-06-27

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