GB790038A - Improvements in or relating to emulsions - Google Patents

Improvements in or relating to emulsions

Info

Publication number
GB790038A
GB790038A GB3108/56A GB310856A GB790038A GB 790038 A GB790038 A GB 790038A GB 3108/56 A GB3108/56 A GB 3108/56A GB 310856 A GB310856 A GB 310856A GB 790038 A GB790038 A GB 790038A
Authority
GB
United Kingdom
Prior art keywords
mols
mol
titanates
specified
zirconates
Prior art date
Legal status (The legal status is an assumption and is not a legal conclusion. Google has not performed a legal analysis and makes no representation as to the accuracy of the status listed.)
Expired
Application number
GB3108/56A
Current Assignee (The listed assignees may be inaccurate. Google has not performed a legal analysis and makes no representation or warranty as to the accuracy of the list.)
Midland Silicones Ltd
Original Assignee
Midland Silicones Ltd
Priority date (The priority date is an assumption and is not a legal conclusion. Google has not performed a legal analysis and makes no representation as to the accuracy of the date listed.)
Filing date
Publication date
Application filed by Midland Silicones Ltd filed Critical Midland Silicones Ltd
Publication of GB790038A publication Critical patent/GB790038A/en
Expired legal-status Critical Current

Links

Classifications

    • DTEXTILES; PAPER
    • D06TREATMENT OF TEXTILES OR THE LIKE; LAUNDERING; FLEXIBLE MATERIALS NOT OTHERWISE PROVIDED FOR
    • D06MTREATMENT, NOT PROVIDED FOR ELSEWHERE IN CLASS D06, OF FIBRES, THREADS, YARNS, FABRICS, FEATHERS OR FIBROUS GOODS MADE FROM SUCH MATERIALS
    • D06M15/00Treating fibres, threads, yarns, fabrics, or fibrous goods made from such materials, with macromolecular compounds; Such treatment combined with mechanical treatment
    • D06M15/19Treating fibres, threads, yarns, fabrics, or fibrous goods made from such materials, with macromolecular compounds; Such treatment combined with mechanical treatment with synthetic macromolecular compounds
    • D06M15/37Macromolecular compounds obtained otherwise than by reactions only involving carbon-to-carbon unsaturated bonds
    • D06M15/643Macromolecular compounds obtained otherwise than by reactions only involving carbon-to-carbon unsaturated bonds containing silicon in the main chain
    • D06M15/6436Macromolecular compounds obtained otherwise than by reactions only involving carbon-to-carbon unsaturated bonds containing silicon in the main chain containing amino groups
    • AHUMAN NECESSITIES
    • A61MEDICAL OR VETERINARY SCIENCE; HYGIENE
    • A61KPREPARATIONS FOR MEDICAL, DENTAL OR TOILETRY PURPOSES
    • A61K8/00Cosmetics or similar toiletry preparations
    • A61K8/18Cosmetics or similar toiletry preparations characterised by the composition
    • A61K8/72Cosmetics or similar toiletry preparations characterised by the composition containing organic macromolecular compounds
    • A61K8/84Cosmetics or similar toiletry preparations characterised by the composition containing organic macromolecular compounds obtained by reactions otherwise than those involving only carbon-carbon unsaturated bonds
    • A61K8/89Polysiloxanes
    • A61K8/896Polysiloxanes containing atoms other than silicon, carbon, oxygen and hydrogen, e.g. dimethicone copolyol phosphate
    • A61K8/898Polysiloxanes containing atoms other than silicon, carbon, oxygen and hydrogen, e.g. dimethicone copolyol phosphate containing nitrogen, e.g. amodimethicone, trimethyl silyl amodimethicone or dimethicone propyl PG-betaine
    • CCHEMISTRY; METALLURGY
    • C08ORGANIC MACROMOLECULAR COMPOUNDS; THEIR PREPARATION OR CHEMICAL WORKING-UP; COMPOSITIONS BASED THEREON
    • C08GMACROMOLECULAR COMPOUNDS OBTAINED OTHERWISE THAN BY REACTIONS ONLY INVOLVING UNSATURATED CARBON-TO-CARBON BONDS
    • C08G77/00Macromolecular compounds obtained by reactions forming a linkage containing silicon with or without sulfur, nitrogen, oxygen or carbon in the main chain of the macromolecule
    • C08G77/04Polysiloxanes
    • C08G77/14Polysiloxanes containing silicon bound to oxygen-containing groups
    • C08G77/16Polysiloxanes containing silicon bound to oxygen-containing groups to hydroxyl groups
    • CCHEMISTRY; METALLURGY
    • C08ORGANIC MACROMOLECULAR COMPOUNDS; THEIR PREPARATION OR CHEMICAL WORKING-UP; COMPOSITIONS BASED THEREON
    • C08GMACROMOLECULAR COMPOUNDS OBTAINED OTHERWISE THAN BY REACTIONS ONLY INVOLVING UNSATURATED CARBON-TO-CARBON BONDS
    • C08G77/00Macromolecular compounds obtained by reactions forming a linkage containing silicon with or without sulfur, nitrogen, oxygen or carbon in the main chain of the macromolecule
    • C08G77/04Polysiloxanes
    • C08G77/22Polysiloxanes containing silicon bound to organic groups containing atoms other than carbon, hydrogen and oxygen
    • C08G77/26Polysiloxanes containing silicon bound to organic groups containing atoms other than carbon, hydrogen and oxygen nitrogen-containing groups
    • CCHEMISTRY; METALLURGY
    • C08ORGANIC MACROMOLECULAR COMPOUNDS; THEIR PREPARATION OR CHEMICAL WORKING-UP; COMPOSITIONS BASED THEREON
    • C08GMACROMOLECULAR COMPOUNDS OBTAINED OTHERWISE THAN BY REACTIONS ONLY INVOLVING UNSATURATED CARBON-TO-CARBON BONDS
    • C08G77/00Macromolecular compounds obtained by reactions forming a linkage containing silicon with or without sulfur, nitrogen, oxygen or carbon in the main chain of the macromolecule
    • C08G77/42Block-or graft-polymers containing polysiloxane sequences
    • C08G77/46Block-or graft-polymers containing polysiloxane sequences containing polyether sequences
    • CCHEMISTRY; METALLURGY
    • C08ORGANIC MACROMOLECULAR COMPOUNDS; THEIR PREPARATION OR CHEMICAL WORKING-UP; COMPOSITIONS BASED THEREON
    • C08LCOMPOSITIONS OF MACROMOLECULAR COMPOUNDS
    • C08L83/00Compositions of macromolecular compounds obtained by reactions forming in the main chain of the macromolecule a linkage containing silicon with or without sulfur, nitrogen, oxygen or carbon only; Compositions of derivatives of such polymers
    • CCHEMISTRY; METALLURGY
    • C08ORGANIC MACROMOLECULAR COMPOUNDS; THEIR PREPARATION OR CHEMICAL WORKING-UP; COMPOSITIONS BASED THEREON
    • C08LCOMPOSITIONS OF MACROMOLECULAR COMPOUNDS
    • C08L83/00Compositions of macromolecular compounds obtained by reactions forming in the main chain of the macromolecule a linkage containing silicon with or without sulfur, nitrogen, oxygen or carbon only; Compositions of derivatives of such polymers
    • C08L83/04Polysiloxanes
    • CCHEMISTRY; METALLURGY
    • C08ORGANIC MACROMOLECULAR COMPOUNDS; THEIR PREPARATION OR CHEMICAL WORKING-UP; COMPOSITIONS BASED THEREON
    • C08LCOMPOSITIONS OF MACROMOLECULAR COMPOUNDS
    • C08L83/00Compositions of macromolecular compounds obtained by reactions forming in the main chain of the macromolecule a linkage containing silicon with or without sulfur, nitrogen, oxygen or carbon only; Compositions of derivatives of such polymers
    • C08L83/04Polysiloxanes
    • C08L83/08Polysiloxanes containing silicon bound to organic groups containing atoms other than carbon, hydrogen and oxygen
    • CCHEMISTRY; METALLURGY
    • C09DYES; PAINTS; POLISHES; NATURAL RESINS; ADHESIVES; COMPOSITIONS NOT OTHERWISE PROVIDED FOR; APPLICATIONS OF MATERIALS NOT OTHERWISE PROVIDED FOR
    • C09KMATERIALS FOR MISCELLANEOUS APPLICATIONS, NOT PROVIDED FOR ELSEWHERE
    • C09K23/00Use of substances as emulsifying, wetting, dispersing, or foam-producing agents
    • C09K23/54Silicon compounds

Landscapes

  • Chemical & Material Sciences (AREA)
  • Health & Medical Sciences (AREA)
  • Chemical Kinetics & Catalysis (AREA)
  • Organic Chemistry (AREA)
  • Medicinal Chemistry (AREA)
  • Polymers & Plastics (AREA)
  • Engineering & Computer Science (AREA)
  • Life Sciences & Earth Sciences (AREA)
  • Materials Engineering (AREA)
  • Textile Engineering (AREA)
  • Birds (AREA)
  • Epidemiology (AREA)
  • Animal Behavior & Ethology (AREA)
  • General Health & Medical Sciences (AREA)
  • Public Health (AREA)
  • Veterinary Medicine (AREA)
  • Compositions Of Macromolecular Compounds (AREA)
  • Silicon Polymers (AREA)

Abstract

Water-soluble organic titanates and zirconates are made by reacting (merely by mixing) from 1 to 4 mols. of one or more alkanolamines of the general formula (HOR)nNH3-n, wherein R is an alkylene radical of from 2 to 6 carbon atoms and n is 2 or 3, with 1 mol. of a compound of the general formula M(OR1)4, in which each R1 is an alkyl radical of from 1 to 10 carbon atoms and M is Ti or Zr. The alcohol formed by the ester interchange may be removed. Alkanolamines specified are triethanolamine, di-sec.-pentanolamine, trihexanolamine and di - tertiary-butanolamine. Alkyl titanates and zirconates specified are tetrabutyl -, tetraisopropyl -, ditertiary - butyldimethyl -, tetraisoamyl - and decyl - triethyl - titanates, and tertaisopropyl-, tetraiso - octyl -, tetraethyl - and triethylbutyl - zirconates. In Examples the titanates or zirconates were made (1) by adding 2 mols. of the specified alkanolamines to 1 mol. of the respective alkyl titanates; (2) by reacting triethanolamine with tetraisopropyl titanate in the molar amounts specified; (3), (8) by reacting 2 mols. of triethanolamine with 1 mol. of tetraisopropyl titanate; and (10) by mixing 14.9 g. of triethanolamine with 19.4 g. of tetraisopropyl zirconate having 1 mol. of isopropanol of crystallization.ALSO:An oil-in-water emulsion comprises (1) from 0.5 to 20 per cent by weight of a hydrocarbon solvent-soluble polysiloxane having an average of 0.05 to 1 silicon-bonded hydrogen and an average of 1.75 to 2.5 total monovalent hydrocarbon radicals and hydrogen atoms per silicon atom, and (2) from 80 to 99.5 per cent by weight of water and a water-soluble metal compound which is a reaction product of from 4 to 1 mols. of one or more alkanolamines of the general formula (HOR)nNH3-n, in which R is an alkylene radical containing from 2 to 6 inclusive carbon atoms and n is 2 or 3, with 1 mol. of a compound of the general formula M(OR1)4, in which each R1 is an alkyl radical containing from 1 to 10 inclusive carbon atoms and M is Ti or Zr, or a partial hydrolysate of the reaction product, the metal compound being present in amount to provide in the emulsion from 0.5 to 15 per cent by weight of metal based on the weight of the siloxane. Silicon-bonded hydrocarbon radicals specified are methyl, ethyl, octadecyl, vinyl, allyl, hexenyl, cyclohexyl, cyclopentyl, cyclohexenyl, phenyl, tolyl, benzyl and xenyl. Emulsifying agents, preferably of the non-ionic type such as glycerol mono-oleate, glycerol stearate and polyvinyl alcohol, may be added, as well as aminoplasts such as urea- and melamine-formaldehyde resins. Examples 1 to 3 and 4 to 9 disclose emulsions containing titanium catalysts and Example 10 discloses an emulsion containing a zirconium catalyst. The emulsions are used for waterproofing inorganic and organic fabrics (see Group VIII). The catalysts may be made by mixing the desired number of mols. of the alkanolamine with the alkyl titanate or zirconate (see Group IV (b)), and effecting partial hydrolysis and subsequent condensation of the resulting product.
GB3108/56A 1955-03-28 1956-01-31 Improvements in or relating to emulsions Expired GB790038A (en)

Applications Claiming Priority (1)

Application Number Priority Date Filing Date Title
US790038XA 1955-03-28 1955-03-28

Publications (1)

Publication Number Publication Date
GB790038A true GB790038A (en) 1958-01-29

Family

ID=22147603

Family Applications (1)

Application Number Title Priority Date Filing Date
GB3108/56A Expired GB790038A (en) 1955-03-28 1956-01-31 Improvements in or relating to emulsions

Country Status (1)

Country Link
GB (1) GB790038A (en)

Cited By (3)

* Cited by examiner, † Cited by third party
Publication number Priority date Publication date Assignee Title
US3223665A (en) * 1960-08-26 1965-12-14 Wacker Chemie Gmbh Stable aqueous emulsions of organohydrogensiloxanes containing a watersoluble aldehyde
DE1282597B (en) * 1964-02-19 1968-11-14 Hoechst Ag Process for making textiles water repellent with organopolysiloxane emulsions
US4683068A (en) * 1981-10-29 1987-07-28 Dowell Schlumberger Incorporated Fracturing of subterranean formations

Cited By (3)

* Cited by examiner, † Cited by third party
Publication number Priority date Publication date Assignee Title
US3223665A (en) * 1960-08-26 1965-12-14 Wacker Chemie Gmbh Stable aqueous emulsions of organohydrogensiloxanes containing a watersoluble aldehyde
DE1282597B (en) * 1964-02-19 1968-11-14 Hoechst Ag Process for making textiles water repellent with organopolysiloxane emulsions
US4683068A (en) * 1981-10-29 1987-07-28 Dowell Schlumberger Incorporated Fracturing of subterranean formations

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