IE831148L - PYRROLO £3,4-d| £2| BENZAZEPINES - Google Patents

PYRROLO £3,4-d| £2| BENZAZEPINES

Info

Publication number
IE831148L
IE831148L IE831148A IE114883A IE831148L IE 831148 L IE831148 L IE 831148L IE 831148 A IE831148 A IE 831148A IE 114883 A IE114883 A IE 114883A IE 831148 L IE831148 L IE 831148L
Authority
IE
Ireland
Prior art keywords
signifies
alkyl
hydrogen
formula
hydroxy
Prior art date
Application number
IE831148A
Other versions
IE55134B1 (en
Original Assignee
Hoffmann La Roche
Priority date (The priority date is an assumption and is not a legal conclusion. Google has not performed a legal analysis and makes no representation as to the accuracy of the date listed.)
Filing date
Publication date
Application filed by Hoffmann La Roche filed Critical Hoffmann La Roche
Publication of IE831148L publication Critical patent/IE831148L/en
Publication of IE55134B1 publication Critical patent/IE55134B1/en

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Classifications

    • CCHEMISTRY; METALLURGY
    • C07ORGANIC CHEMISTRY
    • C07DHETEROCYCLIC COMPOUNDS
    • C07D487/00Heterocyclic compounds containing nitrogen atoms as the only ring hetero atoms in the condensed system, not provided for by groups C07D451/00 - C07D477/00
    • C07D487/02Heterocyclic compounds containing nitrogen atoms as the only ring hetero atoms in the condensed system, not provided for by groups C07D451/00 - C07D477/00 in which the condensed system contains two hetero rings
    • C07D487/04Ortho-condensed systems
    • CCHEMISTRY; METALLURGY
    • C07ORGANIC CHEMISTRY
    • C07CACYCLIC OR CARBOCYCLIC COMPOUNDS
    • C07C255/00Carboxylic acid nitriles
    • CCHEMISTRY; METALLURGY
    • C07ORGANIC CHEMISTRY
    • C07CACYCLIC OR CARBOCYCLIC COMPOUNDS
    • C07C29/00Preparation of compounds having hydroxy or O-metal groups bound to a carbon atom not belonging to a six-membered aromatic ring
    • C07C29/132Preparation of compounds having hydroxy or O-metal groups bound to a carbon atom not belonging to a six-membered aromatic ring by reduction of an oxygen containing functional group
    • C07C29/136Preparation of compounds having hydroxy or O-metal groups bound to a carbon atom not belonging to a six-membered aromatic ring by reduction of an oxygen containing functional group of >C=O containing groups, e.g. —COOH
    • C07C29/147Preparation of compounds having hydroxy or O-metal groups bound to a carbon atom not belonging to a six-membered aromatic ring by reduction of an oxygen containing functional group of >C=O containing groups, e.g. —COOH of carboxylic acids or derivatives thereof
    • CCHEMISTRY; METALLURGY
    • C07ORGANIC CHEMISTRY
    • C07CACYCLIC OR CARBOCYCLIC COMPOUNDS
    • C07C45/00Preparation of compounds having >C = O groups bound only to carbon or hydrogen atoms; Preparation of chelates of such compounds
    • C07C45/27Preparation of compounds having >C = O groups bound only to carbon or hydrogen atoms; Preparation of chelates of such compounds by oxidation
    • C07C45/30Preparation of compounds having >C = O groups bound only to carbon or hydrogen atoms; Preparation of chelates of such compounds by oxidation with halogen containing compounds, e.g. hypohalogenation
    • C07C45/305Preparation of compounds having >C = O groups bound only to carbon or hydrogen atoms; Preparation of chelates of such compounds by oxidation with halogen containing compounds, e.g. hypohalogenation with halogenochromate reagents, e.g. pyridinium chlorochromate
    • CCHEMISTRY; METALLURGY
    • C07ORGANIC CHEMISTRY
    • C07CACYCLIC OR CARBOCYCLIC COMPOUNDS
    • C07C51/00Preparation of carboxylic acids or their salts, halides or anhydrides
    • C07C51/347Preparation of carboxylic acids or their salts, halides or anhydrides by reactions not involving formation of carboxyl groups
    • CCHEMISTRY; METALLURGY
    • C07ORGANIC CHEMISTRY
    • C07DHETEROCYCLIC COMPOUNDS
    • C07D207/00Heterocyclic compounds containing five-membered rings not condensed with other rings, with one nitrogen atom as the only ring hetero atom
    • C07D207/02Heterocyclic compounds containing five-membered rings not condensed with other rings, with one nitrogen atom as the only ring hetero atom with only hydrogen or carbon atoms directly attached to the ring nitrogen atom
    • C07D207/30Heterocyclic compounds containing five-membered rings not condensed with other rings, with one nitrogen atom as the only ring hetero atom with only hydrogen or carbon atoms directly attached to the ring nitrogen atom having two double bonds between ring members or between ring members and non-ring members
    • C07D207/34Heterocyclic compounds containing five-membered rings not condensed with other rings, with one nitrogen atom as the only ring hetero atom with only hydrogen or carbon atoms directly attached to the ring nitrogen atom having two double bonds between ring members or between ring members and non-ring members with hetero atoms or with carbon atoms having three bonds to hetero atoms with at the most one bond to halogen, e.g. ester or nitrile radicals, directly attached to ring carbon atoms
    • CCHEMISTRY; METALLURGY
    • C07ORGANIC CHEMISTRY
    • C07DHETEROCYCLIC COMPOUNDS
    • C07D209/00Heterocyclic compounds containing five-membered rings, condensed with other rings, with one nitrogen atom as the only ring hetero atom
    • C07D209/56Ring systems containing three or more rings
    • C07D209/80[b, c]- or [b, d]-condensed
    • C07D209/94[b, c]- or [b, d]-condensed containing carbocyclic rings other than six-membered

Landscapes

  • Chemical & Material Sciences (AREA)
  • Organic Chemistry (AREA)
  • Chemical Kinetics & Catalysis (AREA)
  • Engineering & Computer Science (AREA)
  • Oil, Petroleum & Natural Gas (AREA)
  • Pharmaceuticals Containing Other Organic And Inorganic Compounds (AREA)
  • Nitrogen Condensed Heterocyclic Rings (AREA)

Abstract

1. Claims (for the Contracting States : BE, CH, DE, FR, GB, IT, LI, LU, NL, SE) Pyrrolo[3,4-d][2]benzazepine derivatives of the general formula see diagramm : EP0094668,P27,F1 wherein R1 and R3 signify hydrogen, (C1 -C7 )-alkyl, hydroxy, (C1 -C7 )-alkoxy or the group -OCOR', R' signifies hydrogen (C1 -C6 )-alkyl or phenyl and R2 and R4 signify hydrogen or R1 and R2 and/or R3 and R4 together signify oxo groups, with the proviso that at least one oxo group is present, R signifies hydrogen, (C1 -C7 )-alkyl, hydroxy-(C2 -C7 )-alkyl, amino-(C2 -C7 )-alkyl, mono- or di-(C1 -C7 )-alkylamino-(C2 -C7 )-alkyl or the group -(C1 -C6 )-alkyl-COR**21 , R**21 signifies hydroxy, (C1 -C7 )-alkoxy, amino or mono- or di-(C1 -C7 )-alkylamino, R5 signifies halogen with an atomic number not exceeding 35 or hydrogen and R6 signifies halogen with an atomic number not exceeding 35, with the proviso that R signifies (C1 -C7 )-alkyl or hydrogen when R1 or R3 signifies hydroxy, (C1 -C7 )-alkoxy or -OCOR', the N-oxides and the pharmaceutically acceptable salts thereof. 1. Claims (for the Contracting State AT) A process for the manufacture of pyrrolo[3,4-d][2]benzazepine derivatives of the general formula see diagramm : EP0094668,P29,F2 wherein R1 and R3 signify hydrogen, (C1 -C7 )-alkyl, hydroxy, (C1 -C7 )-alkoxy or the group -OCOR', R' signifies hydrogen, (C1 -C6 )-alkyl or phenyl and R2 and R4 signify hydrogen or R1 and R2 and/or R3 and R4 together signify oxo groups, with the proviso that at least one oxo group is present, R signifies hydrogen, (C1 -C7 )-alkyl, hydroxy-(C2 -C7 )-alkyl, amino-(C2 -C7 )-alkyl, mono- or di-(C1 -C7 )-alkylamino-(C2 -C7 )-alkyl or the group -(C1 -C6 )-alkyl-COR**21 , R**21 signifies hydroxy, (C1 -C7 )-alkoxy, amino or mono- or di-(C1 -C7 )-alkylamino, R5 signifies halogen with an atomic number not exceeding 35 or hydrogen and R6 signifies halogen with an atomic number not exceeding 35, with the proviso that R signifies (C1 -C7 )-alkyl or hydrogen when R1 or R3 signifies hydroxy, (C1 -C7 )-alkoxy or -OCOR', of N-oxides and of pharmaceutically acceptable salts thereof, characterized by a) for the manufacture of compounds of formula I above in which R1 or R3 signifies hydrogen or (C1 -C7 )-alkyl and the remaining symbols have the above significance and of N-oxides thereof, oxidizing a compound of the general formula see diagramm : EP0094668,P30,F1 wherein one of R11 and R31 signifies hydrogen and the other signifies hydrogen or (C1 -C7 )-alkyl and R, R5 and R6 have the above significance, with a peracid, or b) for the manufacture of compounds of formula I above in which R1 or R3 signifies hydroxy and the remaining substituents have the above significance or R1 and R3 and R4 in each case together signify oxo groups and the remaining symbols have the above significance, oxidizing a compound of formula I in which R1 or R3 signifies hydrogen and the remaining substituents have the above significance or a compound of formula II above in which R11 and R31 signify hydrogen with a lead (IV) carboxylate in the presence of a strong acid, or c) for the manufacture of compounds of formula I above in which R1 or R3 signifies acetoxy and the remaining substituents have the above significance, treating a compound of formula I in which R1 or R3 signifies hydrogen and the remaining substituents have the above significance or a compound of formula II above in which R11 and R31 signify hydrogen with lead tetraacetate in acetic acid, or d) for the manufacture of compounds of formula I above in which R1 or R3 signifies -OCOR' and the remaining substituents have the above significance, treating a compound of formula I in which R1 or R3 signifies hydroxy and the remaining substituents have the above significance with a carboxylic acid anhydride in the presence of a base, or e) for the manufacture of compounds of formula I above in which R1 or R3 signifies (C1 -C7 )-alkoxy and the remaining substituents have the above significance, treating a compound of formula I in which R1 or R3 signifies -OCOR' or hydroxy and the remaining substituents have the above significance or a compound of the formula see diagramm : EP0094668,P30,F2 wherein R12 signifies acetoxy and R, R5 and R6 have the above significance, with a (C1 -C7 )-alkanol in the presence of a strong acid, or f) for the manufacture of compounds of formula I above in which R1 or R3 signifies hydrogen or (C1 -C7 )-alkyl and the remaining substituents have the above significance, desoxidizing an N-oxide of the general formula see diagramm : EP0094668,P31,F1 wherein R, R1 , R2 , R3 , R4 , R5 and R6 have the above significance, and, if desired, g) converting a compound of formula I into a pharmaceutically acceptable salt or converting a pharmaceutically acceptable salt of a compound of formula I into another pharmaceutically acceptable salt. [EP0094668A2]
IE1148/83A 1982-05-18 1983-05-17 Pyrrolo(3,4-d)(2)benzazepine derivatives IE55134B1 (en)

Applications Claiming Priority (2)

Application Number Priority Date Filing Date Title
US37940082A 1982-05-18 1982-05-18
US39314282A 1982-06-28 1982-06-28

Publications (2)

Publication Number Publication Date
IE831148L true IE831148L (en) 1983-11-18
IE55134B1 IE55134B1 (en) 1990-06-06

Family

ID=27008604

Family Applications (1)

Application Number Title Priority Date Filing Date
IE1148/83A IE55134B1 (en) 1982-05-18 1983-05-17 Pyrrolo(3,4-d)(2)benzazepine derivatives

Country Status (9)

Country Link
EP (1) EP0094668B1 (en)
AU (1) AU558354B2 (en)
CA (1) CA1202970A (en)
DE (1) DE3372369D1 (en)
DK (1) DK218583A (en)
IE (1) IE55134B1 (en)
IL (1) IL68711A (en)
NZ (1) NZ204242A (en)
PH (1) PH19004A (en)

Family Cites Families (2)

* Cited by examiner, † Cited by third party
Publication number Priority date Publication date Assignee Title
NL7605526A (en) * 1976-05-24 1977-11-28 Akzo Nv NEW TETRACYCLICAL DERIVATIVES.
US4354973A (en) * 1980-08-05 1982-10-19 Hoffmann-La Roche Inc. Pyrrolo[3,4-d][2]benzazepines

Also Published As

Publication number Publication date
AU558354B2 (en) 1987-01-29
EP0094668A2 (en) 1983-11-23
PH19004A (en) 1985-12-03
CA1202970A (en) 1986-04-08
IL68711A0 (en) 1983-09-30
EP0094668A3 (en) 1985-01-16
AU1460583A (en) 1983-11-24
DK218583A (en) 1983-11-19
EP0094668B1 (en) 1987-07-08
IL68711A (en) 1986-12-31
NZ204242A (en) 1986-08-08
IE55134B1 (en) 1990-06-06
DE3372369D1 (en) 1987-08-13
DK218583D0 (en) 1983-05-17

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