WO2006097663A3 - Cellule de pile à combustible haute température à conduction mixte anionique et protonique - Google Patents

Cellule de pile à combustible haute température à conduction mixte anionique et protonique Download PDF

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Publication number
WO2006097663A3
WO2006097663A3 PCT/FR2006/050235 FR2006050235W WO2006097663A3 WO 2006097663 A3 WO2006097663 A3 WO 2006097663A3 FR 2006050235 W FR2006050235 W FR 2006050235W WO 2006097663 A3 WO2006097663 A3 WO 2006097663A3
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WIPO (PCT)
Prior art keywords
fuel cell
conduction
high temperature
temperature fuel
reforming
Prior art date
Legal status (The legal status is an assumption and is not a legal conclusion. Google has not performed a legal analysis and makes no representation as to the accuracy of the status listed.)
Ceased
Application number
PCT/FR2006/050235
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English (en)
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WO2006097663A2 (fr
Inventor
Alain Thorel
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Association pour la Recherche et le Developpement des Methodes et Processus Industriels
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Association pour la Recherche et le Developpement des Methodes et Processus Industriels
Priority date (The priority date is an assumption and is not a legal conclusion. Google has not performed a legal analysis and makes no representation as to the accuracy of the date listed.)
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Application filed by Association pour la Recherche et le Developpement des Methodes et Processus Industriels filed Critical Association pour la Recherche et le Developpement des Methodes et Processus Industriels
Priority to US11/886,493 priority Critical patent/US7927757B2/en
Priority to EP06726255A priority patent/EP1859502B1/fr
Priority to JP2008501387A priority patent/JP2008533678A/ja
Priority to AT06726255T priority patent/ATE556458T1/de
Publication of WO2006097663A2 publication Critical patent/WO2006097663A2/fr
Publication of WO2006097663A3 publication Critical patent/WO2006097663A3/fr
Anticipated expiration legal-status Critical
Ceased legal-status Critical Current

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    • H—ELECTRICITY
    • H01—ELECTRIC ELEMENTS
    • H01M—PROCESSES OR MEANS, e.g. BATTERIES, FOR THE DIRECT CONVERSION OF CHEMICAL ENERGY INTO ELECTRICAL ENERGY
    • H01M8/00—Fuel cells; Manufacture thereof
    • H01M8/06—Combination of fuel cells with means for production of reactants or for treatment of residues
    • H01M8/0606—Combination of fuel cells with means for production of reactants or for treatment of residues with means for production of gaseous reactants
    • H01M8/0612—Combination of fuel cells with means for production of reactants or for treatment of residues with means for production of gaseous reactants from carbon-containing material
    • C—CHEMISTRY; METALLURGY
    • C01—INORGANIC CHEMISTRY
    • C01B—NON-METALLIC ELEMENTS; COMPOUNDS THEREOF; METALLOIDS OR COMPOUNDS THEREOF NOT COVERED BY SUBCLASS C01C
    • C01B3/00—Hydrogen; Gaseous mixtures containing hydrogen; Separation of hydrogen from mixtures containing it; Purification of hydrogen; Reversible storage of hydrogen
    • C01B3/02—Production of hydrogen; Production of gaseous mixtures containing hydrogen
    • C01B3/22—Production of hydrogen; Production of gaseous mixtures containing hydrogen by decomposition of gaseous or liquid organic compounds
    • C01B3/24—Production of hydrogen; Production of gaseous mixtures containing hydrogen by decomposition of gaseous or liquid organic compounds of hydrocarbons
    • C01B3/26—Production of hydrogen; Production of gaseous mixtures containing hydrogen by decomposition of gaseous or liquid organic compounds of hydrocarbons using catalysts
    • C—CHEMISTRY; METALLURGY
    • C25—ELECTROLYTIC OR ELECTROPHORETIC PROCESSES; APPARATUS THEREFOR
    • C25B—ELECTROLYTIC OR ELECTROPHORETIC PROCESSES FOR THE PRODUCTION OF COMPOUNDS OR NON-METALS; APPARATUS THEREFOR
    • C25B1/00—Electrolytic production of inorganic compounds or non-metals
    • C25B1/01—Products
    • C25B1/02—Hydrogen or oxygen
    • C25B1/04—Hydrogen or oxygen by electrolysis of water
    • H—ELECTRICITY
    • H01—ELECTRIC ELEMENTS
    • H01M—PROCESSES OR MEANS, e.g. BATTERIES, FOR THE DIRECT CONVERSION OF CHEMICAL ENERGY INTO ELECTRICAL ENERGY
    • H01M4/00—Electrodes
    • H01M4/86—Inert electrodes with catalytic activity, e.g. for fuel cells
    • H01M4/8605—Porous electrodes
    • H01M4/8621—Porous electrodes containing only metallic or ceramic material, e.g. made by sintering or sputtering
    • H—ELECTRICITY
    • H01—ELECTRIC ELEMENTS
    • H01M—PROCESSES OR MEANS, e.g. BATTERIES, FOR THE DIRECT CONVERSION OF CHEMICAL ENERGY INTO ELECTRICAL ENERGY
    • H01M4/00—Electrodes
    • H01M4/86—Inert electrodes with catalytic activity, e.g. for fuel cells
    • H01M4/90—Selection of catalytic material
    • H01M4/9016—Oxides, hydroxides or oxygenated metallic salts
    • H01M4/9025—Oxides specially used in fuel cell operating at high temperature, e.g. SOFC
    • H01M4/9033—Complex oxides, optionally doped, of the type M1MeO3, M1 being an alkaline earth metal or a rare earth, Me being a metal, e.g. perovskites
    • H—ELECTRICITY
    • H01—ELECTRIC ELEMENTS
    • H01M—PROCESSES OR MEANS, e.g. BATTERIES, FOR THE DIRECT CONVERSION OF CHEMICAL ENERGY INTO ELECTRICAL ENERGY
    • H01M4/00—Electrodes
    • H01M4/86—Inert electrodes with catalytic activity, e.g. for fuel cells
    • H01M4/90—Selection of catalytic material
    • H01M4/9041—Metals or alloys
    • H01M4/905—Metals or alloys specially used in fuel cell operating at high temperature, e.g. SOFC
    • H01M4/9066—Metals or alloys specially used in fuel cell operating at high temperature, e.g. SOFC of metal-ceramic composites or mixtures, e.g. cermets
    • H—ELECTRICITY
    • H01—ELECTRIC ELEMENTS
    • H01M—PROCESSES OR MEANS, e.g. BATTERIES, FOR THE DIRECT CONVERSION OF CHEMICAL ENERGY INTO ELECTRICAL ENERGY
    • H01M8/00—Fuel cells; Manufacture thereof
    • H01M8/10—Fuel cells with solid electrolytes
    • H01M8/12—Fuel cells with solid electrolytes operating at high temperature, e.g. with stabilised ZrO2 electrolyte
    • H01M8/124—Fuel cells with solid electrolytes operating at high temperature, e.g. with stabilised ZrO2 electrolyte characterised by the process of manufacturing or by the material of the electrolyte
    • H—ELECTRICITY
    • H01—ELECTRIC ELEMENTS
    • H01M—PROCESSES OR MEANS, e.g. BATTERIES, FOR THE DIRECT CONVERSION OF CHEMICAL ENERGY INTO ELECTRICAL ENERGY
    • H01M8/00—Fuel cells; Manufacture thereof
    • H01M8/10—Fuel cells with solid electrolytes
    • H01M8/12—Fuel cells with solid electrolytes operating at high temperature, e.g. with stabilised ZrO2 electrolyte
    • H01M8/124—Fuel cells with solid electrolytes operating at high temperature, e.g. with stabilised ZrO2 electrolyte characterised by the process of manufacturing or by the material of the electrolyte
    • H01M8/1246—Fuel cells with solid electrolytes operating at high temperature, e.g. with stabilised ZrO2 electrolyte characterised by the process of manufacturing or by the material of the electrolyte the electrolyte consisting of oxides
    • H01M8/1253—Fuel cells with solid electrolytes operating at high temperature, e.g. with stabilised ZrO2 electrolyte characterised by the process of manufacturing or by the material of the electrolyte the electrolyte consisting of oxides the electrolyte containing zirconium oxide
    • H—ELECTRICITY
    • H01—ELECTRIC ELEMENTS
    • H01M—PROCESSES OR MEANS, e.g. BATTERIES, FOR THE DIRECT CONVERSION OF CHEMICAL ENERGY INTO ELECTRICAL ENERGY
    • H01M8/00—Fuel cells; Manufacture thereof
    • H01M8/10—Fuel cells with solid electrolytes
    • H01M8/12—Fuel cells with solid electrolytes operating at high temperature, e.g. with stabilised ZrO2 electrolyte
    • H01M8/124—Fuel cells with solid electrolytes operating at high temperature, e.g. with stabilised ZrO2 electrolyte characterised by the process of manufacturing or by the material of the electrolyte
    • H01M8/1246—Fuel cells with solid electrolytes operating at high temperature, e.g. with stabilised ZrO2 electrolyte characterised by the process of manufacturing or by the material of the electrolyte the electrolyte consisting of oxides
    • H01M8/126—Fuel cells with solid electrolytes operating at high temperature, e.g. with stabilised ZrO2 electrolyte characterised by the process of manufacturing or by the material of the electrolyte the electrolyte consisting of oxides the electrolyte containing cerium oxide
    • C—CHEMISTRY; METALLURGY
    • C01—INORGANIC CHEMISTRY
    • C01B—NON-METALLIC ELEMENTS; COMPOUNDS THEREOF; METALLOIDS OR COMPOUNDS THEREOF NOT COVERED BY SUBCLASS C01C
    • C01B2203/00—Integrated processes for the production of hydrogen or synthesis gas
    • C01B2203/02—Processes for making hydrogen or synthesis gas
    • C01B2203/0266—Processes for making hydrogen or synthesis gas containing a decomposition step
    • C01B2203/0277—Processes for making hydrogen or synthesis gas containing a decomposition step containing a catalytic decomposition step
    • C—CHEMISTRY; METALLURGY
    • C01—INORGANIC CHEMISTRY
    • C01B—NON-METALLIC ELEMENTS; COMPOUNDS THEREOF; METALLOIDS OR COMPOUNDS THEREOF NOT COVERED BY SUBCLASS C01C
    • C01B2203/00—Integrated processes for the production of hydrogen or synthesis gas
    • C01B2203/06—Integration with other chemical processes
    • C01B2203/066—Integration with other chemical processes with fuel cells
    • C01B2203/067—Integration with other chemical processes with fuel cells the reforming process taking place in the fuel cell
    • C—CHEMISTRY; METALLURGY
    • C01—INORGANIC CHEMISTRY
    • C01B—NON-METALLIC ELEMENTS; COMPOUNDS THEREOF; METALLOIDS OR COMPOUNDS THEREOF NOT COVERED BY SUBCLASS C01C
    • C01B2203/00—Integrated processes for the production of hydrogen or synthesis gas
    • C01B2203/10—Catalysts for performing the hydrogen forming reactions
    • C01B2203/1041—Composition of the catalyst
    • H—ELECTRICITY
    • H01—ELECTRIC ELEMENTS
    • H01M—PROCESSES OR MEANS, e.g. BATTERIES, FOR THE DIRECT CONVERSION OF CHEMICAL ENERGY INTO ELECTRICAL ENERGY
    • H01M8/00—Fuel cells; Manufacture thereof
    • H01M8/10—Fuel cells with solid electrolytes
    • H01M8/12—Fuel cells with solid electrolytes operating at high temperature, e.g. with stabilised ZrO2 electrolyte
    • H01M2008/1293—Fuel cells with solid oxide electrolytes
    • Y—GENERAL TAGGING OF NEW TECHNOLOGICAL DEVELOPMENTS; GENERAL TAGGING OF CROSS-SECTIONAL TECHNOLOGIES SPANNING OVER SEVERAL SECTIONS OF THE IPC; TECHNICAL SUBJECTS COVERED BY FORMER USPC CROSS-REFERENCE ART COLLECTIONS [XRACs] AND DIGESTS
    • Y02—TECHNOLOGIES OR APPLICATIONS FOR MITIGATION OR ADAPTATION AGAINST CLIMATE CHANGE
    • Y02E—REDUCTION OF GREENHOUSE GAS [GHG] EMISSIONS, RELATED TO ENERGY GENERATION, TRANSMISSION OR DISTRIBUTION
    • Y02E60/00—Enabling technologies; Technologies with a potential or indirect contribution to GHG emissions mitigation
    • Y02E60/30—Hydrogen technology
    • Y02E60/36—Hydrogen production from non-carbon containing sources, e.g. by water electrolysis
    • Y—GENERAL TAGGING OF NEW TECHNOLOGICAL DEVELOPMENTS; GENERAL TAGGING OF CROSS-SECTIONAL TECHNOLOGIES SPANNING OVER SEVERAL SECTIONS OF THE IPC; TECHNICAL SUBJECTS COVERED BY FORMER USPC CROSS-REFERENCE ART COLLECTIONS [XRACs] AND DIGESTS
    • Y02—TECHNOLOGIES OR APPLICATIONS FOR MITIGATION OR ADAPTATION AGAINST CLIMATE CHANGE
    • Y02E—REDUCTION OF GREENHOUSE GAS [GHG] EMISSIONS, RELATED TO ENERGY GENERATION, TRANSMISSION OR DISTRIBUTION
    • Y02E60/00—Enabling technologies; Technologies with a potential or indirect contribution to GHG emissions mitigation
    • Y02E60/30—Hydrogen technology
    • Y02E60/50—Fuel cells
    • Y—GENERAL TAGGING OF NEW TECHNOLOGICAL DEVELOPMENTS; GENERAL TAGGING OF CROSS-SECTIONAL TECHNOLOGIES SPANNING OVER SEVERAL SECTIONS OF THE IPC; TECHNICAL SUBJECTS COVERED BY FORMER USPC CROSS-REFERENCE ART COLLECTIONS [XRACs] AND DIGESTS
    • Y02—TECHNOLOGIES OR APPLICATIONS FOR MITIGATION OR ADAPTATION AGAINST CLIMATE CHANGE
    • Y02P—CLIMATE CHANGE MITIGATION TECHNOLOGIES IN THE PRODUCTION OR PROCESSING OF GOODS
    • Y02P70/00—Climate change mitigation technologies in the production process for final industrial or consumer products
    • Y02P70/50—Manufacturing or production processes characterised by the final manufactured product

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  • Chemical & Material Sciences (AREA)
  • Engineering & Computer Science (AREA)
  • Chemical Kinetics & Catalysis (AREA)
  • Electrochemistry (AREA)
  • Manufacturing & Machinery (AREA)
  • General Chemical & Material Sciences (AREA)
  • Sustainable Development (AREA)
  • Sustainable Energy (AREA)
  • Life Sciences & Earth Sciences (AREA)
  • Materials Engineering (AREA)
  • Organic Chemistry (AREA)
  • Ceramic Engineering (AREA)
  • Inorganic Chemistry (AREA)
  • Composite Materials (AREA)
  • Metallurgy (AREA)
  • Health & Medical Sciences (AREA)
  • General Health & Medical Sciences (AREA)
  • Combustion & Propulsion (AREA)
  • Inert Electrodes (AREA)
  • Fuel Cell (AREA)
  • Electrolytic Production Of Non-Metals, Compounds, Apparatuses Therefor (AREA)

Abstract

La présente invention concerne une cellule de pile à combustible haute température à conduction mixte anionique et protonique comprenant une membrane de reformage à conduction protonique directement couplée à une cellule SOFC (Solid Oxide Fuel CeII) à conduction par ions oxygène, permettant d'éviter la mise en œuvre d'une anode à reformage progressif générant des dépôts de carbone. Le fonctionnement inversé de la présente invention hors l'étage de reformage constitue un électrolyseur à haute température de l'eau apte à produire de façon efficace de l'hydrogène sans avoir à le séparer de l'eau comme c'est le cas dans les systèmes actuels.
PCT/FR2006/050235 2005-03-17 2006-03-17 Cellule de pile à combustible haute température à conduction mixte anionique et protonique Ceased WO2006097663A2 (fr)

Priority Applications (4)

Application Number Priority Date Filing Date Title
US11/886,493 US7927757B2 (en) 2005-03-17 2006-03-17 High temperature fuel cell with mixed anionic and protonic conduction
EP06726255A EP1859502B1 (fr) 2005-03-17 2006-03-17 Cellule de pile à combustible haute température à conduction mixte anionique et protonique
JP2008501387A JP2008533678A (ja) 2005-03-17 2006-03-17 混合アニオン／プロトン伝導を有する高温型燃料電池
AT06726255T ATE556458T1 (de) 2005-03-17 2006-03-17 Hochtemperatur-brennstoffzelle mit gemischter anionischer und protonischer leitung

Applications Claiming Priority (2)

Application Number Priority Date Filing Date Title
FR0550696 2005-03-17
FR0550696A FR2883420B1 (fr) 2005-03-17 2005-03-17 Cellule de pile a combustible haute temperature a conduction mixte anionique et protonique

Publications (2)

Publication Number Publication Date
WO2006097663A2 WO2006097663A2 (fr) 2006-09-21
WO2006097663A3 true WO2006097663A3 (fr) 2007-03-08

Family

ID=35276457

Family Applications (1)

Application Number Title Priority Date Filing Date
PCT/FR2006/050235 Ceased WO2006097663A2 (fr) 2005-03-17 2006-03-17 Cellule de pile à combustible haute température à conduction mixte anionique et protonique

Country Status (6)

Country Link
US (1) US7927757B2 (fr)
EP (1) EP1859502B1 (fr)
JP (1) JP2008533678A (fr)
AT (1) ATE556458T1 (fr)
FR (1) FR2883420B1 (fr)
WO (1) WO2006097663A2 (fr)

Families Citing this family (16)

* Cited by examiner, † Cited by third party
Publication number Priority date Publication date Assignee Title
US8309270B2 (en) 2007-08-03 2012-11-13 Cp Sofc Ip, Llc Solid oxide fuel cell systems with improved gas channeling and heat exchange
JP4946819B2 (ja) * 2007-11-20 2012-06-06 株式会社豊田自動織機 電気化学デバイスおよび排気ガスの浄化装置
US20110151349A1 (en) * 2008-06-10 2011-06-23 Technion Research & Development Foundation Ltd. Double-electrolyte fuel-cell
FR2934717B1 (fr) * 2008-07-29 2010-09-24 Ass Pour La Rech Et Le Dev De Anode a reformage par craquage, de pile a combustible pcfc
US20100028736A1 (en) * 2008-08-01 2010-02-04 Georgia Tech Research Corporation Hybrid Ionomer Electrochemical Devices
KR20110101976A (ko) * 2010-03-10 2011-09-16 삼성전자주식회사 고체산화물 연료전지 및 이의 제조방법
FR2969395B1 (fr) * 2010-12-17 2013-01-11 Ass Pour La Rech Et Le Dev De Methodes Et Processus Ind Armines Pile a combustible avec ensemble electrolytes-membrane monolithique
EP3269845B1 (fr) * 2011-03-26 2019-08-14 Honda Motor Co., Ltd. Procédé de fabrication d'hydrocarbures comme carburants de transport
KR101289203B1 (ko) 2011-08-11 2013-07-29 주식회사 포스코 연료 이용율이 우수한 연료전지 스택
FR2982426B1 (fr) * 2011-11-03 2013-12-27 Ass Pour La Rech Et Le Dev De Methodes Et Processus Ind Armines Pile a combustible avec cathode avec canaux
DE102012102750B4 (de) 2012-03-29 2021-04-22 Deutsches Zentrum für Luft- und Raumfahrt e.V. Brennstoffzellenelement und Brennstoffzellenvorrichtung
DE102014002451A1 (de) * 2014-02-25 2015-08-27 Forschungszentrum Jülich GmbH Elektro-chemischer Energiespeicher sowie Verfahren zum Betreiben desselben
EP3176287B1 (fr) * 2014-07-28 2020-11-18 Nippon Shokubai Co., Ltd. Cellule d'électrolyse de vapeur d'eau
KR101669469B1 (ko) * 2015-07-24 2016-10-26 창원대학교 산학협력단 연료전지용 하이브리드형 단위전지 및 이를 포함하는 연료전지 스택
CN113366150A (zh) * 2019-05-27 2021-09-07 松下知识产权经营株式会社 电化学单元
EP3978652B1 (fr) * 2019-05-27 2025-01-22 Panasonic Intellectual Property Management Co., Ltd. Cellule électrochimique et procédé de génération d'hydrogène

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US4722873A (en) * 1985-12-06 1988-02-02 Mitsubishi Denki Kabushiki Kaisha Fuel cell power generating system
JPH07130382A (ja) * 1993-11-05 1995-05-19 Ishikawajima Harima Heavy Ind Co Ltd 内部改質燃料電池
US6013386A (en) * 1995-03-16 2000-01-11 British Nuclear Fuels Plc Solid oxide fuel cells with specific electrode layers
EP1170812A2 (fr) * 2000-07-04 2002-01-09 Nissan Motor Co., Ltd. Pile à combustible à oxydes solides comportant de l'électrolyte solide perovskite
US20020031695A1 (en) * 2000-07-31 2002-03-14 Smotkin Eugene S. Hydrogen permeable membrane for use in fuel cells, and partial reformate fuel cell system having reforming catalysts in the anode fuel cell compartment
US20040072039A1 (en) * 2002-07-01 2004-04-15 The Regents Of The University Of California MEMS-based fuel cells with integrated catalytic fuel processor and method thereof
JP2005190970A (ja) * 2003-12-26 2005-07-14 Tokyo Institute Of Technology 燃料電池

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US20030235753A1 (en) * 2002-06-25 2003-12-25 David Champion Method for fabricating high surface area catalysts
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US4722873A (en) * 1985-12-06 1988-02-02 Mitsubishi Denki Kabushiki Kaisha Fuel cell power generating system
JPH07130382A (ja) * 1993-11-05 1995-05-19 Ishikawajima Harima Heavy Ind Co Ltd 内部改質燃料電池
US6013386A (en) * 1995-03-16 2000-01-11 British Nuclear Fuels Plc Solid oxide fuel cells with specific electrode layers
EP1170812A2 (fr) * 2000-07-04 2002-01-09 Nissan Motor Co., Ltd. Pile à combustible à oxydes solides comportant de l'électrolyte solide perovskite
US20020031695A1 (en) * 2000-07-31 2002-03-14 Smotkin Eugene S. Hydrogen permeable membrane for use in fuel cells, and partial reformate fuel cell system having reforming catalysts in the anode fuel cell compartment
US20040072039A1 (en) * 2002-07-01 2004-04-15 The Regents Of The University Of California MEMS-based fuel cells with integrated catalytic fuel processor and method thereof
JP2005190970A (ja) * 2003-12-26 2005-07-14 Tokyo Institute Of Technology 燃料電池

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RACHID EL MOUSSAOUI ET AL: "CO-ION LEAKAGE THROUGH BIPOLAR MEMBRANES INFLUENCE ON I-V RESPONSES AND WATER-SPLITTING EFFICIENCY", JOURNAL OF MEMBRANE SCIENCE, ELSEVIER SCIENTIFIC PUBL.COMPANY. AMSTERDAM, NL, vol. 90, no. 3, 4 May 1994 (1994-05-04), pages 283 - 292, XP000490141, ISSN: 0376-7388 *
XU ET AL: "Ion exchange membranes: State of their development and perspective", JOURNAL OF MEMBRANE SCIENCE, ELSEVIER SCIENTIFIC PUBL.COMPANY. AMSTERDAM, NL, vol. 263, no. 1-2, 15 October 2005 (2005-10-15), pages 1 - 29, XP005081239, ISSN: 0376-7388 *

Also Published As

Publication number Publication date
WO2006097663A2 (fr) 2006-09-21
JP2008533678A (ja) 2008-08-21
EP1859502B1 (fr) 2012-05-02
EP1859502A2 (fr) 2007-11-28
FR2883420A1 (fr) 2006-09-22
US7927757B2 (en) 2011-04-19
US20080213639A1 (en) 2008-09-04
FR2883420B1 (fr) 2007-05-11
ATE556458T1 (de) 2012-05-15

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