CH235237A - Process for the preparation of 2 ', 3', 5'-trimethyl-cyclopentane-1 ', 5-spiro-1-methyl-2,4,6-triketo-hexahydropyrimidine. - Google Patents

Process for the preparation of 2 ', 3', 5'-trimethyl-cyclopentane-1 ', 5-spiro-1-methyl-2,4,6-triketo-hexahydropyrimidine.

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Publication number
CH235237A
CH235237A CH235237DA CH235237A CH 235237 A CH235237 A CH 235237A CH 235237D A CH235237D A CH 235237DA CH 235237 A CH235237 A CH 235237A
Authority
CH
Switzerland
Prior art keywords
sep
cyclopentane
triketo
methyl
trimethyl
Prior art date
Application number
Other languages
German (de)
Inventor
Ag J R Geigy
Original Assignee
Ag J R Geigy
Priority date (The priority date is an assumption and is not a legal conclusion. Google has not performed a legal analysis and makes no representation as to the accuracy of the date listed.)
Filing date
Publication date
Application filed by Ag J R Geigy filed Critical Ag J R Geigy
Publication of CH235237A publication Critical patent/CH235237A/en

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Description

  

  Verfahren     zur    Herstellung von     2',3',5'-Trimethyl-cyclopentau-1',5-spiro-l-methyl-          2,4,6-triketo-hegahydropyrimidin.     
EMI0001.0004     
  
    Gegenstand <SEP> vorliegenden <SEP> Zusatzpatentes
<tb>  ist <SEP> ein <SEP> Verfahren <SEP> zur <SEP> Herstellung <SEP> von
<tb>  2', <SEP> 3', <SEP> 5' <SEP> - <SEP> Trnmethyl <SEP> - <SEP> cyclio,pentan1-1', <SEP> 5 <SEP> - <SEP> sipiro <SEP> -1  methyl <SEP> - <SEP> 2,4,6 <SEP> - <SEP> triketo <SEP> - <SEP> hexahydropyrimidin,
<tb>  welches <SEP> dadurch <SEP> gekennz@eiehniet <SEP> ist, <SEP> dass <SEP> man
<tb>  2,3,5-Tritm!ethyl-cycliopentan-l-cya.n-l-,carbon  ssäureester <SEP> mit <SEP> Dii.cyandiamid <SEP> kondensiert,

   <SEP> das
<tb>  Kondensiationsprodukt <SEP> methyliert <SEP> und <SEP> an  schliessend <SEP> der <SEP> I-Iydtrolys,e <SEP> unterwirft.
<tb>  



  Dia <SEP> neue <SEP> Verbindung <SEP> ist <SEP> ein <SEP> hochviskoses,
<tb>  schwach <SEP> gelblich <SEP> gefärbtes <SEP> 01, <SEP> Kp. <SEP> p,4 <SEP> 139 <SEP> bis
<tb>  141 . <SEP> Sie <SEP> besitzt <SEP> na.rkotn)s,che <SEP> -Wirkung.
<tb>  



  <I>Beispiel:</I>
<tb>  Zu <SEP> einer <SEP> Lösung <SEP> von <SEP> 4,6 <SEP> Teilen <SEP> Natrium
<tb>  in <SEP> 70 <SEP> Teilen <SEP> absolutem <SEP> Alkohol <SEP> fügt <SEP> man
<tb>  <B>20,9</B> <SEP> Teile <SEP> 2, <SEP> 3, <SEP> 5 <SEP> - <SEP> Trimetliyl <SEP> - <SEP> cyelop <SEP> entan <SEP> -1  cyan-l-.ca,rbunLäureäthylestp-,r <SEP> und <SEP> 10 <SEP> Teile
<tb>  Dicya-näiamid <SEP> und <SEP> erhitzt <SEP> 10 <SEP> Stunden <SEP> lang
<tb>  unten <SEP> Rückflsusslkühl!un#g. <SEP> Naaob:

   <SEP> dem <SEP> Erkalten
<tb>  gibt <SEP> man <SEP> tropfenweise <SEP> 12,6 <SEP> Teile <SEP> Dimetliyl  sufat <SEP> hinzu, <SEP> wobei <SEP> man <SEP> durch <SEP> Kühlung <SEP> die
<tb>  Temperatur <SEP> unterhalb <SEP> 50  <SEP> hälit. <SEP> Hierauf       ,destilliert man den     Alkohol    ab und     erbnitzt     !den Rückstand mit     dem    sechsfachen Menge  Schwefelsäure     (25%ig)

      8     Stunden    lang zum       Sieden.    Die     neue        Verbindung        läss    t     sieh        nricht     in     kristallisierter    Form     erhalten,    sie     wded     durch     Ausiäthern        iss,okert    und nach leim  Trocknen über     entwässertem        Natriumsulfat          und    Verjagen des     Äthers    im     Vakuum          destilliert.  



  Process for the preparation of 2 ', 3', 5'-trimethyl-cyclopentau-1 ', 5-spiro-1-methyl-2,4,6-triketo-hegahydropyrimidine.
EMI0001.0004
  
    Subject <SEP> of the present <SEP> additional patent
<tb> <SEP> is a <SEP> process <SEP> for <SEP> production <SEP> of
<tb> 2 ', <SEP> 3', <SEP> 5 '<SEP> - <SEP> Trnmethyl <SEP> - <SEP> cyclio, pentane1-1', <SEP> 5 <SEP> - <SEP> sipiro <SEP> -1 methyl <SEP> - <SEP> 2,4,6 <SEP> - <SEP> triketo <SEP> - <SEP> hexahydropyrimidine,
<tb> which <SEP> is marked with <SEP> @ eiehniet <SEP>, <SEP> that <SEP> man
<tb> 2,3,5-Tritm! ethyl-cycliopentane-l-cya.n-l-, carboxylic acid ester <SEP> condensed with <SEP> di.cyandiamide <SEP>,

   <SEP> that
<tb> Condensation product <SEP> methylates <SEP> and <SEP> followed by <SEP> which subjects <SEP> Iydtrolys, e <SEP>.
<tb>



  The <SEP> new <SEP> connection <SEP> is <SEP> a <SEP> highly viscous,
<tb> weak <SEP> yellowish <SEP> colored <SEP> 01, <SEP> Kp. <SEP> p, 4 <SEP> 139 <SEP> to
<tb> 141. <SEP> You <SEP> has <SEP> na.rkotn) s, che <SEP> effect.
<tb>



  <I> Example: </I>
<tb> To <SEP> a <SEP> solution <SEP> of <SEP> 4.6 <SEP> parts <SEP> sodium
<tb> in <SEP> 70 <SEP> parts <SEP> absolute <SEP> alcohol <SEP> adds <SEP> man
<tb> <B> 20,9 </B> <SEP> parts <SEP> 2, <SEP> 3, <SEP> 5 <SEP> - <SEP> Trimetliyl <SEP> - <SEP> cyelop <SEP> entan <SEP> -1 cyan-l-.ca, rbunLäureäthylestp-, r <SEP> and <SEP> 10 <SEP> parts
<tb> Dicya-Näiamid <SEP> and <SEP> heats <SEP> for 10 <SEP> hours <SEP>
<tb> below <SEP> reflux oil cool! un # g. <SEP> Naaob:

   <SEP> the <SEP> cooling down
<tb> <SEP> one <SEP> <SEP> drop by drop <SEP> 12.6 <SEP> parts <SEP> Dimethylsufat <SEP>, <SEP> whereby <SEP> one <SEP> by <SEP> cooling <SEP > the
<tb> temperature <SEP> below <SEP> 50 <SEP> holds. <SEP> Then, the alcohol is distilled off and the residue is carved out with six times the amount of sulfuric acid (25%)

      Simmer for 8 hours. The new compound cannot be preserved in crystallized form, it is eaten by dieting, okert and after glue drying over dehydrated sodium sulphate and expulsion of the ether, it is distilled in a vacuum.

 

Claims (1)

EMI0001.0027 PATENTANSPRUCH: <tb> Verfahren <SEP> zur <SEP> Herstellung <SEP> von <SEP> 2',3',5' Tri,m,edhyl- <SEP> cyclopentan-1',5 <SEP> -ispi.ro-1-methyl 2,4,6 <SEP> - <SEP> triketo <SEP> - <SEP> hex-ahydropyrimidin, <SEP> dadurch <tb> gekennzeichnet, <SEP> ,dass, <SEP> man <SEP> 2,3,5-Trimethyl cyclopentan <SEP> -1- <SEP> Cyan <SEP> -1- <SEP> ca.rbonsäureester <SEP> mit <tb> Dicyanä,ami-cl <SEP> kondiensn,ert, <SEP> das <SEP> K.ondensa tionsproduklt <SEP> methyliert <SEP> und <SEP> anschliessend <SEP> ,der <tb> Hydrolyse <SEP> unterwimft. <tb> Die <SEP> neue <SEP> Verbindung <SEP> ist <SEP> ein <SEP> hochviskoses, <tb> schwach <SEP> gelblich <SEP> gefärbtes <SEP> @0<B>1</B>, <SEP> KP- <SEP> 0,4 <SEP> 1,39 <SEP> bis <tb> 141 . <SEP> Sie <SEP> besitzt <SEP> narkotische <SEP> Wirkung. EMI0001.0027 PATENT CLAIM: <tb> Process <SEP> for <SEP> production <SEP> of <SEP> 2 ', 3', 5 'Tri, m, edhyl- <SEP> cyclopentane-1', 5 <SEP> -ispi.ro- 1-methyl 2,4,6 <SEP> - <SEP> triketo <SEP> - <SEP> hex-ahydropyrimidine, <SEP> thereby <tb> marked, <SEP> that, <SEP> man <SEP> 2,3,5-trimethyl cyclopentane <SEP> -1- <SEP> cyano <SEP> -1- <SEP> approx. carboxylic acid ester <SEP > with <tb> Dicyanä, ami-cl <SEP> kondiensn, ert, <SEP> the <SEP> condensation product <SEP> methylated <SEP> and <SEP> then <SEP>, the <tb> Hydrolysis <SEP> subject. <tb> The <SEP> new <SEP> connection <SEP> is <SEP> a <SEP> highly viscous, <tb> weak <SEP> yellowish <SEP> colored <SEP> @ 0 <B> 1 </B>, <SEP> KP- <SEP> 0.4 <SEP> 1.39 <SEP> to <tb> 141. <SEP> You <SEP> has <SEP> narcotic <SEP> effect.
CH235237D 1942-07-29 1942-07-29 Process for the preparation of 2 ', 3', 5'-trimethyl-cyclopentane-1 ', 5-spiro-1-methyl-2,4,6-triketo-hexahydropyrimidine. CH235237A (en)

Applications Claiming Priority (2)

Application Number Priority Date Filing Date Title
CH235237T 1942-07-29
CH230367T 1942-07-29

Publications (1)

Publication Number Publication Date
CH235237A true CH235237A (en) 1944-11-15

Family

ID=25727476

Family Applications (1)

Application Number Title Priority Date Filing Date
CH235237D CH235237A (en) 1942-07-29 1942-07-29 Process for the preparation of 2 ', 3', 5'-trimethyl-cyclopentane-1 ', 5-spiro-1-methyl-2,4,6-triketo-hexahydropyrimidine.

Country Status (1)

Country Link
CH (1) CH235237A (en)

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