CH291937A - Process for the preparation of a new thioether. - Google Patents

Process for the preparation of a new thioether.

Info

Publication number
CH291937A
CH291937A CH291937DA CH291937A CH 291937 A CH291937 A CH 291937A CH 291937D A CH291937D A CH 291937DA CH 291937 A CH291937 A CH 291937A
Authority
CH
Switzerland
Prior art keywords
new
dimethylamino
thioether
phenyl
production
Prior art date
Application number
Other languages
German (de)
Inventor
Aktiengesellschaft Cilag
Original Assignee
Cilag Ag
Priority date (The priority date is an assumption and is not a legal conclusion. Google has not performed a legal analysis and makes no representation as to the accuracy of the date listed.)
Filing date
Publication date
Application filed by Cilag Ag filed Critical Cilag Ag
Publication of CH291937A publication Critical patent/CH291937A/en

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  • Organic Low-Molecular-Weight Compounds And Preparation Thereof (AREA)
  • Acyclic And Carbocyclic Compounds In Medicinal Compositions (AREA)

Description

  

  <B>verfahren</B>     zur   <B>Herstellung</B>     eines   <B>neuen</B>     Thioäthers.       Gegenstand des vorliegenden Patentes ist  ein Verfahren zur Herstellung eines neuen       Thioäthers,    nämlich des     1.-Dimethylamino-          3    -     aminoinethyl    -     3-phenyl-5-methylmercapto-          pentans.     



  Dieser neue Äther soll als Zwischen pro   < lukt zur Herstellung von     analgetisch    und  antiallergisch wirkenden Verbindungen ver  wendet werden.  



  Das den Gegenstand des Patentes bildende  Verfahren ist dadurch gekennzeichnet, dass  man die Verbindung der Formel  
EMI0001.0011     
    reduziert.  Die Reduktion kann in bekannter Weise  mit     nascierenden    oder katalytisch aktiviertem  Wasserstoff erfolgen. Als sehr vorteilhaft hat  sieh die Reduktion mit     Lithiumaluminium-          liydrid    in Äther erwiesen. Das in dieser Weise  erhaltene     1-Dimethylamino-3-aminomethyl-3-          pheny        1-5-methylmercapto-pentan    bildet ein  unter 0,02 mm bei 126-127  siedendes hell  gelbes öl. Seine     N-Acetylverbindung    schmilz  bei 50 .  



       Beispiel:     30 g     1-Dimethylamino-3-cyano-3-phenyl-5-          metliyimercapto-pentan,    gelöst in 150     cms        abs.     Äther, werden unter     Turbinieren    mit einer    Suspension von 10,4 g     Lithiumaluminium-          hydrid    in 200     em3        abs.    Äther tropfenweise  versetzt. Nach 24 Stunden wird vorsichtig mit  Wasser versetzt, bis der     Lithiumaluminium-          hydrid-Überschuss    zersetzt ist und dann  100     cm3        2n-Essigsäure    zugegeben.

   Von die  sem Gemisch wird der Äther     abdestilliert    und  die     wässrige    Lösung mit     konz.    Natronlauge       alkalisiert.    Die ölige Ausscheidung wird in  Äther aufgenommen und die     vereinigten     Ätherextrakte getrocknet und verdampft. Der  Rückstand wird im Hochvakuum destilliert.

         Klan    erhält so 26 g des unter 0,02 mm bei  126-127  siedenden     1-Dimethylamino-3-amino-          methyl    - 3 -     phenyl    - 5     -methylmercapto-pentans.     Die neue Base     ist    wenig löslich     in    Wasser,  gut löslich in den gebräuchlichen organischen  Lösungsmitteln. Die N -     Acetylverbindung     schmilzt bei 50 .



  <B> process </B> for <B> production </B> of a <B> new </B> thioether. The subject of the present patent is a process for the production of a new thioether, namely 1.-dimethylamino-3-aminoinethyl-3-phenyl-5-methylmercaptopentane.



  This new ether is to be used as an intermediate product for the production of compounds with an analgesic and antiallergic effect.



  The process forming the subject of the patent is characterized in that the compound of the formula
EMI0001.0011
    reduced. The reduction can take place in a known manner with nascent or catalytically activated hydrogen. The reduction with lithium aluminum hydride in ether has proven to be very advantageous. The 1-dimethylamino-3-aminomethyl-3-pheny 1-5-methylmercapto-pentane obtained in this way forms a pale yellow oil boiling below 0.02 mm at 126-127. Its N-acetyl compound melts at 50.



       Example: 30 g of 1-dimethylamino-3-cyano-3-phenyl-5-methylimercapto-pentane, dissolved in 150 cms of abs. Ether, are turbinated with a suspension of 10.4 g of lithium aluminum hydride in 200 em3 abs. Ether added dropwise. After 24 hours, water is carefully added until the excess lithium aluminum hydride has decomposed and 100 cm3 of 2N acetic acid are then added.

   From this mixture the ether is distilled off and the aqueous solution with conc. Caustic soda alkalizes. The oily excretion is taken up in ether and the combined ether extracts are dried and evaporated. The residue is distilled in a high vacuum.

         Klan thus receives 26 g of 1-dimethylamino-3-aminomethyl-3-phenyl-5-methylmercaptopentane which boils below 0.02 mm at 126-127. The new base is sparingly soluble in water and readily soluble in common organic solvents. The N - acetyl compound melts at 50.

 

Claims (1)

<B>PATENTANSPRUCH:</B> Verfahren zur Herstellung eines neuen Thioäthers, nämlich des 1-Dimethylamino- 3 - aminomethyl - 3-phenyl- 5-methylmercapto- pentans, dadurch gekennzeichnet, dass man die Verbindung der Formel EMI0001.0055 reduziert. Das so erhaltene 1-Dimethylamino-3-amino- methyl-3-phenyl-5-methylmercapto-pentan bil det ein unter 0,02 mm bei 12G-127 siedendes hellgelbes Öl. Seine Aeetylverbindung schmilzt bei 50 . <B> PATENT CLAIM: </B> Process for the production of a new thioether, namely 1-dimethylamino- 3-aminomethyl-3-phenyl-5-methylmercaptopentane, characterized in that the compound of the formula EMI0001.0055 reduced. The 1-dimethylamino-3-aminomethyl-3-phenyl-5-methylmercapto-pentane obtained in this way forms a pale yellow oil boiling below 0.02 mm at 12G-127. Its ethyl compound melts at 50. Der neue Thioäther soll als Zwisehenpro- dukt zur Herstellung von analgetiseh und antiallergiseh wirkenden Verbindungen ver wendet. werden. The new thioether is said to be used as an intermediate product for the production of analgesic and antiallergic compounds. will.
CH291937D 1953-08-23 1950-08-23 Process for the preparation of a new thioether. CH291937A (en)

Applications Claiming Priority (1)

Application Number Priority Date Filing Date Title
CH291937T 1953-08-23

Publications (1)

Publication Number Publication Date
CH291937A true CH291937A (en) 1953-07-15

Family

ID=4487624

Family Applications (1)

Application Number Title Priority Date Filing Date
CH291937D CH291937A (en) 1953-08-23 1950-08-23 Process for the preparation of a new thioether.

Country Status (1)

Country Link
CH (1) CH291937A (en)

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