CH294247A - Process for the production of a brown, chromium-containing dye. - Google Patents

Process for the production of a brown, chromium-containing dye.

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Publication number
CH294247A
CH294247A CH294247DA CH294247A CH 294247 A CH294247 A CH 294247A CH 294247D A CH294247D A CH 294247DA CH 294247 A CH294247 A CH 294247A
Authority
CH
Switzerland
Prior art keywords
parts
brown
chromium
production
dye
Prior art date
Application number
Other languages
German (de)
Inventor
Ag J R Geigy
Original Assignee
Ag J R Geigy
Priority date (The priority date is an assumption and is not a legal conclusion. Google has not performed a legal analysis and makes no representation as to the accuracy of the date listed.)
Filing date
Publication date
Application filed by Ag J R Geigy filed Critical Ag J R Geigy
Publication of CH294247A publication Critical patent/CH294247A/en

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Classifications

    • CCHEMISTRY; METALLURGY
    • C09DYES; PAINTS; POLISHES; NATURAL RESINS; ADHESIVES; COMPOSITIONS NOT OTHERWISE PROVIDED FOR; APPLICATIONS OF MATERIALS NOT OTHERWISE PROVIDED FOR
    • C09BORGANIC DYES OR CLOSELY-RELATED COMPOUNDS FOR PRODUCING DYES, e.g. PIGMENTS; MORDANTS; LAKES
    • C09B45/00Complex metal compounds of azo dyes
    • C09B45/01Complex metal compounds of azo dyes characterised by the method of metallisation
    • CCHEMISTRY; METALLURGY
    • C09DYES; PAINTS; POLISHES; NATURAL RESINS; ADHESIVES; COMPOSITIONS NOT OTHERWISE PROVIDED FOR; APPLICATIONS OF MATERIALS NOT OTHERWISE PROVIDED FOR
    • C09BORGANIC DYES OR CLOSELY-RELATED COMPOUNDS FOR PRODUCING DYES, e.g. PIGMENTS; MORDANTS; LAKES
    • C09B45/00Complex metal compounds of azo dyes
    • C09B45/02Preparation from dyes containing in o-position a hydroxy group and in o'-position hydroxy, alkoxy, carboxyl, amino or keto groups
    • C09B45/14Monoazo compounds
    • C09B45/16Monoazo compounds containing chromium

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  • Chemical & Material Sciences (AREA)
  • Organic Chemistry (AREA)
  • Coloring (AREA)

Description

  

      Zusatzpatent    zum Hauptpatent Nr. 291812.    Verfahren     zur        Herstellung    eines     braunen,        ehromhaltigen    Farbstoffes.    Gegenstand vorliegenden Patentes ist ein  Verfahren zur Herstellung eines braunen,       ehromhaltigen    Farbstoffes. Das Verfahren ist.  
EMI0001.0007     
    mit chromabgebenden Mitteln in solchen Men  gen behandelt, dass auf 2 Moleküle     Azofarb-          stoff    mindestens 1 Atom entfällt.  



  Die erhaltene neue, gemischte     Chromkom-          plexverbindung    stellt ein schwarzes Pulver  dar, das Wolle aus schwach essigsaurem Bade  in tiefbraunen Tönen färbt.         Beispiel:     18,8 Teile     2-Amino-phenol-4-sulfamid    wer  den in 150 Teilen Wasser mit 17 Teilen kon  zentrierter Salzsäure gelöst, auf 5  abgekühlt  und durch Zugabe von 6,9 Teilen Natrium  nitrit (als     33proz.    Lösung) dianotiert. Durch  Zugabe von     Natriumhydrogenkarbonat    wird  die überschüssige Salzsäure neutralisiert.

   Die  neutrale     Anschlämmung    der     Diazoniumver-          bindung    giesst man bei 3  in eine Lösung von  18,3 Teilen     1-Phenyl-3-methyl-5-pyrazolon    in    dadurch gekennzeichnet, dass man ein Gemisch       äquimolekularerMengen    der     Azofarbstoffe     
EMI0001.0022     
    200 Teilen Wasser und 20 Teilen wasserfreiem  Natriumkarbonat.

   Nachdem die Kupplung be  endet ist, isoliert man den Farbstoff (Farb  stoff I) durch Filtration. 18,7 Teile     2-Amino-          phenol-4-methylsulfon    werden in 150 Teilen  Wasser mit 17 Teilen konzentrierter Salzsäure  gelöst, auf 5  abgekühlt und unter zeitweiser  Zugabe von Eis mit 6,9 Teilen     Natriumnitrit     100 % (als     33proz.    Lösung) versetzt.

   Die     Di-          a,zoverbindung    wird mit     Natriumhydrogen-          karbonat    neutralisiert und bei 0 bis 3  in eine  Lösung von 22,8 Teilen     Carbomethoxyamino-          naphthol-(1,7)    in 250 Teilen Wasser, 10,5     Vo-          lumteilen        10n-Natronlauge    und 15 Teilen was  serfreiem Natriumkarbonat gegossen. Die  Kupplung ist nach einigen Stunden beendet.

    Man erhitzt auf 70 , fällt. den teilweise in Lö  sung gegangenen Farbstoff durch Zugabe von       Natriumchlorid    aus und filtriert ihn ab  (Farbstoff     II).         Farbstoff I schlämmt man mit 37 Teilen       Mononatriumsalz    des Farbstoffes     II    in 2000  Teilen Wasser an, gibt 210 Teile einer Lösung  von     ehromsalieylsaurem    Ammonium (ent  sprechend 5,45 Teilen     Cr)    zu und erhitzt  während 4 Stunden zum Sieden. Es bildet  sieh eine schwarzbraune     Lösung,    die man  mit     Natriumchlorid    versetzt. Dabei fällt der  Mischkomplex aus. Er wird     abfiltriert    und  getrocknet.

   Er stellt ein schwarzes Pulver dar,  
EMI0002.0008     
    mit     ehromabgebenden    Mitteln in solchen Men  gen behandelt, dass auf 2 Moleküle     Azofarb-          stoff        mindestens    1 Atom Chrom entfällt.  



  Die erhaltene neue gemischte Chrom  komplexverbindung stellt ein schwarzes Pul-    das Wolle aus schwach essigsaurem Bade in       tiefbralanen    Tönen von sehr guter     Lichteeht-          heit    und guten     Nassechtheiten    färbt.



      Additional patent to the main patent No. 291812. Process for the production of a brown, Ehrom-containing dye. The subject of the present patent is a process for the production of a brown, Ehrom-containing dye. The procedure is.
EMI0001.0007
    Treated with chromium-releasing agents in such quantities that there are at least 1 atom per 2 molecules of azo dye.



  The new, mixed chromium complex compound obtained is a black powder that dyes wool from a weakly acetic acid bath in deep brown shades. Example: 18.8 parts of 2-aminophenol-4-sulfamide are dissolved in 150 parts of water with 17 parts of concentrated hydrochloric acid, cooled to 5 and dianotized by adding 6.9 parts of sodium nitrite (as a 33% solution). The excess hydrochloric acid is neutralized by adding sodium hydrogen carbonate.

   The neutral suspension of the diazonium compound is poured at 3 into a solution of 18.3 parts of 1-phenyl-3-methyl-5-pyrazolone, characterized in that a mixture of equimolecular amounts of the azo dyes is used
EMI0001.0022
    200 parts of water and 20 parts of anhydrous sodium carbonate.

   After the coupling has ended, the dye (dye I) is isolated by filtration. 18.7 parts of 2-aminophenol-4-methylsulfone are dissolved in 150 parts of water with 17 parts of concentrated hydrochloric acid, cooled to 5 and mixed with 6.9 parts of 100% sodium nitrite (as a 33% solution) with the occasional addition of ice.

   The di-a, zo compound is neutralized with sodium hydrogen carbonate and at 0 to 3 in a solution of 22.8 parts of carbomethoxyaminonaphthol (1.7) in 250 parts of water, 10.5 parts by volume of 10N sodium hydroxide solution and 15 Share what was poured anhydrous sodium carbonate. The coupling is complete after a few hours.

    It is heated to 70%. the dye, which has partially gone into solution, by adding sodium chloride and filtering it off (dye II). Dye I is slurried with 37 parts of the monosodium salt of dye II in 2000 parts of water, 210 parts of a solution of Ehromsalieylsaurem ammonium (accordingly 5.45 parts of Cr) are added and the mixture is heated to the boil for 4 hours. A black-brown solution forms to which sodium chloride is added. The mixed complex precipitates in the process. It is filtered off and dried.

   It represents a black powder
EMI0002.0008
    Treated with chromium-releasing agents in such quantities that there is at least 1 atom of chromium for every 2 molecules of azo dye.



  The new mixed chromium complex compound obtained is a black powder that dyes wool from weakly acetic acid bath in deep bralan shades of very good lightfastness and good wet fastness properties.

 

Claims (1)

PATENTANSPRUCH Verfahren zur Herstellung eines braunen, ehromhaltigen Farbstoffes, dadurch gekenn zeichnet, dass man ein Gemisch äquimole- kularer Mengen der Azofarbstoffe EMI0002.0023 ver dar, das Wolle aus schwach essigsaurem Bade in tiefbraunen Tönen färbt.. PATENT CLAIM Process for the production of a brown, Ehrom-containing dye, characterized in that a mixture of equimolecular amounts of the azo dyes EMI0002.0023 ver dar, which dyes wool from weakly acetic acid bath in deep brown shades.
CH294247D 1951-01-11 1951-01-11 Process for the production of a brown, chromium-containing dye. CH294247A (en)

Applications Claiming Priority (2)

Application Number Priority Date Filing Date Title
CH294247T 1951-01-11
CH291812T 1951-01-11

Publications (1)

Publication Number Publication Date
CH294247A true CH294247A (en) 1953-10-31

Family

ID=25733154

Family Applications (1)

Application Number Title Priority Date Filing Date
CH294247D CH294247A (en) 1951-01-11 1951-01-11 Process for the production of a brown, chromium-containing dye.

Country Status (1)

Country Link
CH (1) CH294247A (en)

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