CH300023A - Process for the preparation of a trisazo dye. - Google Patents

Process for the preparation of a trisazo dye.

Info

Publication number
CH300023A
CH300023A CH300023DA CH300023A CH 300023 A CH300023 A CH 300023A CH 300023D A CH300023D A CH 300023DA CH 300023 A CH300023 A CH 300023A
Authority
CH
Switzerland
Prior art keywords
preparation
parts
coupling
trisazo dye
water
Prior art date
Application number
Other languages
German (de)
Inventor
Aktiengesellschaft Ciba
Original Assignee
Ciba Geigy
Priority date (The priority date is an assumption and is not a legal conclusion. Google has not performed a legal analysis and makes no representation as to the accuracy of the date listed.)
Filing date
Publication date
Application filed by Ciba Geigy filed Critical Ciba Geigy
Publication of CH300023A publication Critical patent/CH300023A/en

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Classifications

    • CCHEMISTRY; METALLURGY
    • C09DYES; PAINTS; POLISHES; NATURAL RESINS; ADHESIVES; COMPOSITIONS NOT OTHERWISE PROVIDED FOR; APPLICATIONS OF MATERIALS NOT OTHERWISE PROVIDED FOR
    • C09BORGANIC DYES OR CLOSELY-RELATED COMPOUNDS FOR PRODUCING DYES, e.g. PIGMENTS; MORDANTS; LAKES
    • C09B35/00Disazo and polyazo dyes of the type A<-D->B prepared by diazotising and coupling
    • C09B35/38Trisazo dyes ot the type
    • C09B35/44Trisazo dyes ot the type the component K being a hydroxy amine
    • C09B35/46Trisazo dyes ot the type the component K being a hydroxy amine the component K being an amino naphthol
    • C09B35/463D being derived from diaminodiphenyl

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  • Chemical & Material Sciences (AREA)
  • Organic Chemistry (AREA)
  • Paper (AREA)

Description

  

  Verfahren zur Herstellung eines     Trisazofarbstoffes.       Es     wurde        (gefunden,    dass man zu einem wertvollen     Trisazofarbatoff    gelangt, wenn       man    eine     Diazoverbindung    der Formel  
EMI0001.0007     
    worin     Y    eine     diazotierte        Aminogruppe    bedeu  tet, mit 2 -     OYt        naphthalin    - 3,6 -     disulfonsäure     kuppelt.  



  Der neue     Farbstoff    bildet ein schwarzes  Pulver, das sieh in Wasser leicht löst und       eliromgegerbtes    Leder in     rotstichig    marine  blauen Tönen färbt.  



  Die     Diazoverbindungen    der obigen Formel  können hergestellt     werden,    indem man     tetrazo-          tiertes        4,4'-Diamino-diphenyl    in saurem Me  dium einseitig mit     1-Amino-8-oxvnaphthalin-          3;6-disulfonsäure    kuppelt und die so erhaltene       Verbindung    hierauf in alkalischem Medium  mit.     diazotierter        1.-Aminobenzol-4-sttlfonsäure     vereinigt.

   Die Kupplung der so erhältlichen       Diazodisazoverbindungen        mit    der     2-Oxvnaph-          tlialin-3,6-clisulfonsätire    erfolgt zweckmässig  in alkalischem Medium.  



       Beispiel:          l1an        tetrazotiert    19 Teile     4,4'-Diamino-          diplien        y1    in     bekannter    Weise. Zu dieser       Tetrazolösung    tropft man     innert    einer Stunde  eine klare Lösung von 34,1 Teilen     1-Amino-8-          oxvnaphtlialin-3,6-disttlfonsäure    in 300 Tei-    ).en Wasser, die einen PH-Wert von 5,6 zeigt.  Die Temperatur beträgt 10 bis 15 .

   Durch all  mähliches     Zutropfen    einer verdünnten, wäs  serigen Lösung von     Natriumcarbonat    stumpft  man die bei der Kupplung frei werdende     Mine-          ralsäure    ab, das Gemisch soll aber immer deut  lich kongosauer reagieren. Nach zwölf Stun  den lässt man bei 5  die     Diazoniumlösung    aus  17,3 Teilen     1-Aminobenzol-4-sulfonsäure        zi1-          laufen    und stürzt unter kräftigem Rühren  eine Lösung von 26 Teilen     Natriumcarbonat    in  120 Teilen Wasser zum Kupplungsgemisch;  der     pH-Wert    soll nicht höher als 8,5 sein.

   Nach  30 Minuten wird eine Lösung aus 30,4; Teilen       2-Oxpnaphthalin-3,6-disulfonsäure    und 5 Tei  len     Natriumcarbonat    in 150 Teilen Wasser zu  gegeben. Nach zweistündigem Rühren wird  durch Zugabe von Salzsäure das Reaktions  gemisch schwach sauer gestellt, der abgeschie  dene Farbstoff     abfiltriert    und     getroeknet.  



  Process for the preparation of a trisazo dye. It has been found that a valuable trisazo carbate is obtained by using a diazo compound of the formula
EMI0001.0007
    where Y is a diazotized amino group, coupled with 2 - OYt naphthalene - 3,6 - disulfonic acid.



  The new dye forms a black powder that dissolves easily in water and dyes Elirom-tanned leather in reddish marine blue tones.



  The diazo compounds of the above formula can be prepared by coupling tetrazoated 4,4'-diamino-diphenyl in acidic medium on one side with 1-amino-8-oxvnaphthalene-3; 6-disulfonic acid and then coupling the compound so obtained in alkaline Medium with. diazotized 1.-aminobenzene-4-sttlfonsäure combined.

   The coupling of the diazodisazo compounds obtainable in this way with the 2-oxynaphthalene-3,6-clisulfonate is expediently carried out in an alkaline medium.



       Example: 19 parts of 4,4'-diamino diplomas y1 tetrazotized in a known manner. A clear solution of 34.1 parts of 1-amino-8-oxvnaphtlialin-3,6-distulfonic acid in 300 parts of water, which has a pH of 5.6, is added dropwise to this tetrazo solution over the course of one hour. The temperature is 10 to 15.

   Gradual dropwise addition of a dilute, aqueous solution of sodium carbonate blunted the mineral acid released during the coupling, but the mixture should always be clearly acidic to the Congo. After twelve hours, the diazonium solution of 17.3 parts of 1-aminobenzene-4-sulfonic acid is allowed to run at 5 and a solution of 26 parts of sodium carbonate in 120 parts of water is added to the coupling mixture with vigorous stirring; the pH should not be higher than 8.5.

   After 30 minutes a solution of 30.4; Parts of 2-oxpnaphthalene-3,6-disulfonic acid and 5 parts of sodium carbonate in 150 parts of water are added. After two hours of stirring, the reaction mixture is made weakly acidic by adding hydrochloric acid, and the dyestuff deposited is filtered off and dried.

 

Claims (1)

PATENTANSPRUCH: Verfahren zur Herstellung eines Trisazo- farbstoffes, dadurch gekennzeichnet, dass man eine Diazoverbindung der Formel EMI0002.0001 worin X eine diazotierte Aminogruppe bedeu tet, mit 2-0xinaphthalin-3,6-disulfonsäure kuppelt. Der neue Farbstoff bildet ein schwarzes Pulver, das sieh in Wasser leicht löst und chromgegerbtes Leder in rotstichig marine blauen Tönen färbt. Claim: Process for the preparation of a trisazo dye, characterized in that a diazo compound of the formula EMI0002.0001 wherein X is a diazotized amino group, coupled with 2-oxinaphthalene-3,6-disulfonic acid. The new dye forms a black powder that dissolves easily in water and colors chrome-tanned leather in reddish-tinged marine blue tones. <B>UNTERANSPRUCH:</B> Verfahren -emäss Patentansprueh, da durch gekennzeiehnet, dalS man die Iiupplttng in alkalischem Medium durchführt. <B> SUBSTANTIAL CLAIM: </B> Method according to patent claim, as it is characterized by the fact that the coupling is carried out in an alkaline medium.
CH300023D 1951-06-25 1951-06-25 Process for the preparation of a trisazo dye. CH300023A (en)

Applications Claiming Priority (1)

Application Number Priority Date Filing Date Title
CH300023T 1951-06-25

Publications (1)

Publication Number Publication Date
CH300023A true CH300023A (en) 1954-07-15

Family

ID=4490521

Family Applications (1)

Application Number Title Priority Date Filing Date
CH300023D CH300023A (en) 1951-06-25 1951-06-25 Process for the preparation of a trisazo dye.

Country Status (1)

Country Link
CH (1) CH300023A (en)

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