CH90592A - Process for the preparation of isopropylallylbarbituric acid. - Google Patents

Process for the preparation of isopropylallylbarbituric acid.

Info

Publication number
CH90592A
CH90592A CH90592DA CH90592A CH 90592 A CH90592 A CH 90592A CH 90592D A CH90592D A CH 90592DA CH 90592 A CH90592 A CH 90592A
Authority
CH
Switzerland
Prior art keywords
sep
acid
preparation
isopropylallylbarbituric
solution
Prior art date
Application number
Other languages
German (de)
Inventor
F Hoffmann- Aktiengesellschaft
Original Assignee
Hoffmann La Roche
Priority date (The priority date is an assumption and is not a legal conclusion. Google has not performed a legal analysis and makes no representation as to the accuracy of the date listed.)
Filing date
Publication date
Application filed by Hoffmann La Roche filed Critical Hoffmann La Roche
Publication of CH90592A publication Critical patent/CH90592A/en

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Classifications

    • CCHEMISTRY; METALLURGY
    • C07ORGANIC CHEMISTRY
    • C07DHETEROCYCLIC COMPOUNDS
    • C07D239/00Heterocyclic compounds containing 1,3-diazine or hydrogenated 1,3-diazine rings
    • C07D239/02Heterocyclic compounds containing 1,3-diazine or hydrogenated 1,3-diazine rings not condensed with other rings
    • C07D239/24Heterocyclic compounds containing 1,3-diazine or hydrogenated 1,3-diazine rings not condensed with other rings having three or more double bonds between ring members or between ring members and non-ring members
    • C07D239/28Heterocyclic compounds containing 1,3-diazine or hydrogenated 1,3-diazine rings not condensed with other rings having three or more double bonds between ring members or between ring members and non-ring members with hetero atoms or with carbon atoms having three bonds to hetero atoms with at the most one bond to halogen, directly attached to ring carbon atoms
    • C07D239/46Two or more oxygen, sulphur or nitrogen atoms
    • C07D239/60Three or more oxygen or sulfur atoms
    • C07D239/62Barbituric acids

Landscapes

  • Chemical & Material Sciences (AREA)
  • Organic Chemistry (AREA)
  • Organic Low-Molecular-Weight Compounds And Preparation Thereof (AREA)

Description

  

  Verfahren zur Darstellung von     Isopropylallylbarbitursättre.       Gegenstand der vorliegenden     =Erfindung     ist ein Verfahren zur Darstellung von     Iso-          propylallylbai@bitursliure;    welches darin besteht,  dass man auf die     Alkaliverbindungen    der     Mono-          isopropylbarbitursäure        Allylhalogenid    bei nie  derer Temperatur.     und    ohne Anwendung von  Druck einwirken lässt.  



  Die     Isopropylallylbai,bitursäure    bildet farb  lose. Kristalle vom Schmelzpunkt 137-138 .  Sie ist in Wasser ziemlich schwer; in Al  kohol leicht löslich und im Vergleich zu den  bekannten     Dialkylbarbitursäuren    sehr leicht       löslich    in     Aether.    Die wässerige Lösung  reagiert auf Lackmus neutral. Die neue Ver  bindung löst sich in kalter verdünnter Natron  lauge     und    wird aus ihrer alkalischen Lösung  durch Ansäuern unverändert abgeschieden.  



  Die     Isopropylallylba rbitursäure    soll zu  therapeutischen Zwecken Verwendung     finden.          BeispAel:     170 Gewichtsteile     Isopropylbarbitursäure     werden mit 500 Gewichtsteilen Wasser über  gossen und durch Zufügen von 135 Gewichts  teilen     30prozentiger    Natronlauge in Lösung    gebracht. Nach erfolgter Lösung setzt man  130 U     ewichtsteile        Allylbromid    hinzu und ver  rührt     emulgierend    bei einer inneren Tempe  ratur von etwa 250.- Die     Reaktion    ist an  fänglich von einer geringen     Wärmeentwicklung    ,  begleitet.

   Nach 12 Stunden ist die     Reaktion     beendet. Die von abgeschiedener     Isopropy        1-          allylbarbitursäure    dünnbreiige Masse wird  nach gutem Abkühlen abgesaugt. Die Aus  beute beträgt über     80o/0    der theoretisch     be-          rechneten        11Ienge.    Durch einmaliges     -Umkri-          stallisieren    aus verdünntem Alkohol wird die       Isopropylallylbarbitursäure    rein in Form farb  loser Kristalle vom Schmelzpunkt 137-138   erhalten. .



  Process for the preparation of isopropylallyl barbiturates. The present invention relates to a process for the preparation of isopropylallylbai @ bitursliure; which consists in the fact that one on the alkali compounds of the mono-isopropylbarbituric acid allyl halide at low temperature. and let it take effect without applying pressure.



  The Isopropylallylbai, bituric acid forms colorless. Crystals with a melting point of 137-138. It's quite heavy in water; Easily soluble in alcohol and, compared to the known dialkylbarbituric acids, very easily soluble in ether. The aqueous solution reacts neutrally to litmus. The new connection dissolves in cold, dilute caustic soda and is separated from its alkaline solution unchanged by acidification.



  The isopropylallylba rbituric acid is said to be used for therapeutic purposes. Example: 170 parts by weight of isopropylbarbituric acid are poured over 500 parts by weight of water and dissolved by adding 135 parts by weight of 30 percent sodium hydroxide solution. After the solution is complete, 130 parts by weight of allyl bromide are added and the mixture is stirred in an emulsifying manner at an internal temperature of about 250. The reaction is initially accompanied by a slight evolution of heat.

   The reaction has ended after 12 hours. The thin-pulpy mass of isopropyl 1-allylbarbituric acid that has separated out is filtered off with suction after cooling well. The yield is over 80o / 0 of the theoretically calculated 11length. A single recrystallization from dilute alcohol gives isopropylallylbarbituric acid in pure form in the form of colorless crystals with a melting point of 137-138. .

 

Claims (1)

PATENTANSPRUCH: Verfahren zur-Darstellung von Isopropyl- ällylbarbitursäure, dadurch -gekennzeichnet, dass man auf die Alkaliverbindungen der Monoisopropylparbitursäure Allylhalogenide bei niederer Temperatur ohne Anwendung von Druck einwirken: lässt. Die Isopropylallylbarbitursäure bildet farb lose Kristalle vom Schmelzpunkt 137-138 . PATENT CLAIM: Process for the preparation of isopropyl ällylbarbituric acid, characterized in that allyl halides are allowed to act on the alkali compounds of monoisopropyl parbituric acid at low temperature without the application of pressure. Isopropylallylbarbituric acid forms colorless crystals with a melting point of 137-138. die ist in Wasser ziemlich schwer,* in Alkohol EMI0002.0001 leicht <SEP> löslich <SEP> und <SEP> im <SEP> Vergleich <SEP> zu <SEP> den <SEP> be kannten <SEP> _Dialkylbarbitursäuren <SEP> sehr <SEP> leicht <tb> löslich. <SEP> lu <SEP> Aetlier. <SEP> Die <SEP> wiisserige_Lösung <SEP> rea giert <SEP> auf <SEP> Lackmus <SEP> neutral-. <SEP> Die <SEP> neue <SEP> Verbin- dung <SEP> ldst#sich <SEP> in <SEP> kalter <SEP> verdünnter <SEP> Natron- EMI0002.0002 lauge <SEP> und <SEP> wird. <SEP> aus <SEP> ihrer <SEP> 21käliscben <SEP> Lösung <tb> durch <SEP> Ansäuern <SEP> unverändert- <SEP> äbgeschiöden. <tb> Die <SEP> IsopropY-lallylbarbitursäui.e <SEP> soll'- <SEP> zu <tb> therapeutischen <SEP> Zwecken <SEP> Verwendung <SEP> finden. it's pretty heavy in water, * in alcohol EMI0002.0001 slightly <SEP> soluble <SEP> and <SEP> in the <SEP> comparison <SEP> to <SEP> the <SEP> known <SEP> _dialkylbarbituric acids <SEP> very <SEP> easily <tb> soluble. <SEP> lu <SEP> Aetlier. <SEP> The <SEP> wiisserige_solution <SEP> reacts <SEP> to <SEP> litmus <SEP> neutrally. <SEP> The <SEP> new <SEP> connection <SEP> can be found # <SEP> in <SEP> cold <SEP> diluted <SEP> soda EMI0002.0002 lauge <SEP> and <SEP> will. <SEP> from <SEP> your <SEP> 21käliscben <SEP> solution <tb> by <SEP> acidification <SEP> unchanged - <SEP> lower floors. <tb> The <SEP> IsopropY-lallylbarbitursäui.e <SEP> shall'- <SEP> too <tb> therapeutic <SEP> purposes <SEP> find use <SEP>.
CH90592D 1920-09-17 1920-09-17 Process for the preparation of isopropylallylbarbituric acid. CH90592A (en)

Applications Claiming Priority (1)

Application Number Priority Date Filing Date Title
CH90592T 1920-09-17

Publications (1)

Publication Number Publication Date
CH90592A true CH90592A (en) 1921-11-01

Family

ID=4347867

Family Applications (1)

Application Number Title Priority Date Filing Date
CH90592D CH90592A (en) 1920-09-17 1920-09-17 Process for the preparation of isopropylallylbarbituric acid.

Country Status (1)

Country Link
CH (1) CH90592A (en)

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