ES8401511A1 - Procedimiento para la obtencion de medios de revestimiento a base de dispersiones acuosas de poliuretano. - Google Patents

Procedimiento para la obtencion de medios de revestimiento a base de dispersiones acuosas de poliuretano.

Info

Publication number
ES8401511A1
ES8401511A1 ES515315A ES515315A ES8401511A1 ES 8401511 A1 ES8401511 A1 ES 8401511A1 ES 515315 A ES515315 A ES 515315A ES 515315 A ES515315 A ES 515315A ES 8401511 A1 ES8401511 A1 ES 8401511A1
Authority
ES
Spain
Prior art keywords
weight
molecular weight
finishes
aqueous polyurethane
coating compositions
Prior art date
Legal status (The legal status is an assumption and is not a legal conclusion. Google has not performed a legal analysis and makes no representation as to the accuracy of the status listed.)
Expired
Application number
ES515315A
Other languages
English (en)
Other versions
ES515315A0 (es
Current Assignee (The listed assignees may be inaccurate. Google has not performed a legal analysis and makes no representation or warranty as to the accuracy of the list.)
Bayer AG
Original Assignee
Bayer AG
Priority date (The priority date is an assumption and is not a legal conclusion. Google has not performed a legal analysis and makes no representation as to the accuracy of the date listed.)
Filing date
Publication date
Application filed by Bayer AG filed Critical Bayer AG
Publication of ES515315A0 publication Critical patent/ES515315A0/es
Publication of ES8401511A1 publication Critical patent/ES8401511A1/es
Expired legal-status Critical Current

Links

Classifications

    • C—CHEMISTRY; METALLURGY
    • C08—ORGANIC MACROMOLECULAR COMPOUNDS; THEIR PREPARATION OR CHEMICAL WORKING-UP; COMPOSITIONS BASED THEREON
    • C08G—MACROMOLECULAR COMPOUNDS OBTAINED OTHERWISE THAN BY REACTIONS ONLY INVOLVING UNSATURATED CARBON-TO-CARBON BONDS
    • C08G18/00—Polymeric products of isocyanates or isothiocyanates
    • C08G18/06—Polymeric products of isocyanates or isothiocyanates with compounds having active hydrogen
    • C08G18/08—Processes
    • C08G18/0804—Manufacture of polymers containing ionic or ionogenic groups
    • C—CHEMISTRY; METALLURGY
    • C08—ORGANIC MACROMOLECULAR COMPOUNDS; THEIR PREPARATION OR CHEMICAL WORKING-UP; COMPOSITIONS BASED THEREON
    • C08G—MACROMOLECULAR COMPOUNDS OBTAINED OTHERWISE THAN BY REACTIONS ONLY INVOLVING UNSATURATED CARBON-TO-CARBON BONDS
    • C08G18/00—Polymeric products of isocyanates or isothiocyanates
    • C08G18/06—Polymeric products of isocyanates or isothiocyanates with compounds having active hydrogen
    • C08G18/08—Processes
    • C08G18/10—Prepolymer processes involving reaction of isocyanates or isothiocyanates with compounds having active hydrogen in a first reaction step
    • C08G18/12—Prepolymer processes involving reaction of isocyanates or isothiocyanates with compounds having active hydrogen in a first reaction step using two or more compounds having active hydrogen in the first polymerisation step
    • C—CHEMISTRY; METALLURGY
    • C08—ORGANIC MACROMOLECULAR COMPOUNDS; THEIR PREPARATION OR CHEMICAL WORKING-UP; COMPOSITIONS BASED THEREON
    • C08G—MACROMOLECULAR COMPOUNDS OBTAINED OTHERWISE THAN BY REACTIONS ONLY INVOLVING UNSATURATED CARBON-TO-CARBON BONDS
    • C08G18/00—Polymeric products of isocyanates or isothiocyanates
    • C08G18/06—Polymeric products of isocyanates or isothiocyanates with compounds having active hydrogen
    • C08G18/28—Polymeric products of isocyanates or isothiocyanates with compounds having active hydrogen characterised by the compounds used containing active hydrogen
    • C08G18/40—High-molecular-weight compounds
    • C08G18/42—Polycondensates having carboxylic or carbonic ester groups in the main chain
    • C—CHEMISTRY; METALLURGY
    • C08—ORGANIC MACROMOLECULAR COMPOUNDS; THEIR PREPARATION OR CHEMICAL WORKING-UP; COMPOSITIONS BASED THEREON
    • C08G—MACROMOLECULAR COMPOUNDS OBTAINED OTHERWISE THAN BY REACTIONS ONLY INVOLVING UNSATURATED CARBON-TO-CARBON BONDS
    • C08G18/00—Polymeric products of isocyanates or isothiocyanates
    • C08G18/06—Polymeric products of isocyanates or isothiocyanates with compounds having active hydrogen
    • C08G18/28—Polymeric products of isocyanates or isothiocyanates with compounds having active hydrogen characterised by the compounds used containing active hydrogen
    • C08G18/40—High-molecular-weight compounds
    • C08G18/42—Polycondensates having carboxylic or carbonic ester groups in the main chain
    • C08G18/4236—Polycondensates having carboxylic or carbonic ester groups in the main chain containing only aliphatic groups
    • C08G18/4238—Polycondensates having carboxylic or carbonic ester groups in the main chain containing only aliphatic groups derived from dicarboxylic acids and dialcohols
    • C—CHEMISTRY; METALLURGY
    • C08—ORGANIC MACROMOLECULAR COMPOUNDS; THEIR PREPARATION OR CHEMICAL WORKING-UP; COMPOSITIONS BASED THEREON
    • C08G—MACROMOLECULAR COMPOUNDS OBTAINED OTHERWISE THAN BY REACTIONS ONLY INVOLVING UNSATURATED CARBON-TO-CARBON BONDS
    • C08G18/00—Polymeric products of isocyanates or isothiocyanates
    • C08G18/06—Polymeric products of isocyanates or isothiocyanates with compounds having active hydrogen
    • C08G18/28—Polymeric products of isocyanates or isothiocyanates with compounds having active hydrogen characterised by the compounds used containing active hydrogen
    • C08G18/40—High-molecular-weight compounds
    • C08G18/42—Polycondensates having carboxylic or carbonic ester groups in the main chain
    • C08G18/44—Polycarbonates
    • C—CHEMISTRY; METALLURGY
    • C08—ORGANIC MACROMOLECULAR COMPOUNDS; THEIR PREPARATION OR CHEMICAL WORKING-UP; COMPOSITIONS BASED THEREON
    • C08G—MACROMOLECULAR COMPOUNDS OBTAINED OTHERWISE THAN BY REACTIONS ONLY INVOLVING UNSATURATED CARBON-TO-CARBON BONDS
    • C08G18/00—Polymeric products of isocyanates or isothiocyanates
    • C08G18/06—Polymeric products of isocyanates or isothiocyanates with compounds having active hydrogen
    • C08G18/28—Polymeric products of isocyanates or isothiocyanates with compounds having active hydrogen characterised by the compounds used containing active hydrogen
    • C08G18/65—Low-molecular-weight compounds having active hydrogen with high-molecular-weight compounds having active hydrogen
    • C08G18/66—Compounds of groups C08G18/42, C08G18/48, or C08G18/52
    • C08G18/6633—Compounds of group C08G18/42
    • C08G18/6637—Compounds of group C08G18/42 with compounds of group C08G18/32 or polyamines of C08G18/38
    • C08G18/664—Compounds of group C08G18/42 with compounds of group C08G18/32 or polyamines of C08G18/38 with compounds of group C08G18/3203
    • C08G18/6644—Compounds of group C08G18/42 with compounds of group C08G18/32 or polyamines of C08G18/38 with compounds of group C08G18/3203 having at least three hydroxy groups
    • C—CHEMISTRY; METALLURGY
    • C08—ORGANIC MACROMOLECULAR COMPOUNDS; THEIR PREPARATION OR CHEMICAL WORKING-UP; COMPOSITIONS BASED THEREON
    • C08G—MACROMOLECULAR COMPOUNDS OBTAINED OTHERWISE THAN BY REACTIONS ONLY INVOLVING UNSATURATED CARBON-TO-CARBON BONDS
    • C08G18/00—Polymeric products of isocyanates or isothiocyanates
    • C08G18/06—Polymeric products of isocyanates or isothiocyanates with compounds having active hydrogen
    • C08G18/70—Polymeric products of isocyanates or isothiocyanates with compounds having active hydrogen characterised by the isocyanates or isothiocyanates used
    • C08G18/72—Polyisocyanates or polyisothiocyanates
    • C08G18/721—Two or more polyisocyanates not provided for in one single group C08G18/73 - C08G18/80
    • C08G18/722—Combination of two or more aliphatic and/or cycloaliphatic polyisocyanates
    • C—CHEMISTRY; METALLURGY
    • C08—ORGANIC MACROMOLECULAR COMPOUNDS; THEIR PREPARATION OR CHEMICAL WORKING-UP; COMPOSITIONS BASED THEREON
    • C08G—MACROMOLECULAR COMPOUNDS OBTAINED OTHERWISE THAN BY REACTIONS ONLY INVOLVING UNSATURATED CARBON-TO-CARBON BONDS
    • C08G18/00—Polymeric products of isocyanates or isothiocyanates
    • C08G18/06—Polymeric products of isocyanates or isothiocyanates with compounds having active hydrogen
    • C08G18/70—Polymeric products of isocyanates or isothiocyanates with compounds having active hydrogen characterised by the isocyanates or isothiocyanates used
    • C08G18/72—Polyisocyanates or polyisothiocyanates
    • C08G18/74—Polyisocyanates or polyisothiocyanates cyclic
    • C08G18/75—Polyisocyanates or polyisothiocyanates cyclic cycloaliphatic
    • C—CHEMISTRY; METALLURGY
    • C08—ORGANIC MACROMOLECULAR COMPOUNDS; THEIR PREPARATION OR CHEMICAL WORKING-UP; COMPOSITIONS BASED THEREON
    • C08J—WORKING-UP; GENERAL PROCESSES OF COMPOUNDING; AFTER-TREATMENT NOT COVERED BY SUBCLASSES C08B, C08C, C08F, C08G or C08H
    • C08J7/00—Chemical treatment or coating of shaped articles made of macromolecular substances
    • C08J7/04—Coating
    • C08J7/0427—Coating with only one layer of a composition containing a polymer binder
    • C—CHEMISTRY; METALLURGY
    • C08—ORGANIC MACROMOLECULAR COMPOUNDS; THEIR PREPARATION OR CHEMICAL WORKING-UP; COMPOSITIONS BASED THEREON
    • C08J—WORKING-UP; GENERAL PROCESSES OF COMPOUNDING; AFTER-TREATMENT NOT COVERED BY SUBCLASSES C08B, C08C, C08F, C08G or C08H
    • C08J7/00—Chemical treatment or coating of shaped articles made of macromolecular substances
    • C08J7/04—Coating
    • C08J7/043—Improving the adhesiveness of the coatings per se, e.g. forming primers
    • C—CHEMISTRY; METALLURGY
    • C08—ORGANIC MACROMOLECULAR COMPOUNDS; THEIR PREPARATION OR CHEMICAL WORKING-UP; COMPOSITIONS BASED THEREON
    • C08J—WORKING-UP; GENERAL PROCESSES OF COMPOUNDING; AFTER-TREATMENT NOT COVERED BY SUBCLASSES C08B, C08C, C08F, C08G or C08H
    • C08J7/00—Chemical treatment or coating of shaped articles made of macromolecular substances
    • C08J7/04—Coating
    • C08J7/046—Forming abrasion-resistant coatings; Forming surface-hardening coatings
    • C—CHEMISTRY; METALLURGY
    • C08—ORGANIC MACROMOLECULAR COMPOUNDS; THEIR PREPARATION OR CHEMICAL WORKING-UP; COMPOSITIONS BASED THEREON
    • C08J—WORKING-UP; GENERAL PROCESSES OF COMPOUNDING; AFTER-TREATMENT NOT COVERED BY SUBCLASSES C08B, C08C, C08F, C08G or C08H
    • C08J2327/00—Characterised by the use of homopolymers or copolymers of compounds having one or more unsaturated aliphatic radicals, each having only one carbon-to-carbon double bond, and at least one being terminated by a halogen; Derivatives of such polymers
    • C08J2327/02—Characterised by the use of homopolymers or copolymers of compounds having one or more unsaturated aliphatic radicals, each having only one carbon-to-carbon double bond, and at least one being terminated by a halogen; Derivatives of such polymers not modified by chemical after-treatment
    • C08J2327/04—Characterised by the use of homopolymers or copolymers of compounds having one or more unsaturated aliphatic radicals, each having only one carbon-to-carbon double bond, and at least one being terminated by a halogen; Derivatives of such polymers not modified by chemical after-treatment containing chlorine atoms
    • C08J2327/06—Homopolymers or copolymers of vinyl chloride
    • Y—GENERAL TAGGING OF NEW TECHNOLOGICAL DEVELOPMENTS; GENERAL TAGGING OF CROSS-SECTIONAL TECHNOLOGIES SPANNING OVER SEVERAL SECTIONS OF THE IPC; TECHNICAL SUBJECTS COVERED BY FORMER USPC CROSS-REFERENCE ART COLLECTIONS [XRACs] AND DIGESTS
    • Y10—TECHNICAL SUBJECTS COVERED BY FORMER USPC
    • Y10T—TECHNICAL SUBJECTS COVERED BY FORMER US CLASSIFICATION
    • Y10T428/00—Stock material or miscellaneous articles
    • Y10T428/31504—Composite [nonstructural laminate]
    • Y10T428/31551—Of polyamidoester [polyurethane, polyisocyanate, polycarbamate, etc.]
    • Y10T428/31573—Next to addition polymer of ethylenically unsaturated monomer
    • Y10T428/3158—Halide monomer type [polyvinyl chloride, etc.]

Landscapes

  • Chemical & Material Sciences (AREA)
  • Health & Medical Sciences (AREA)
  • Chemical Kinetics & Catalysis (AREA)
  • Medicinal Chemistry (AREA)
  • Polymers & Plastics (AREA)
  • Organic Chemistry (AREA)
  • Engineering & Computer Science (AREA)
  • Manufacturing & Machinery (AREA)
  • Paints Or Removers (AREA)
  • Polyurethanes Or Polyureas (AREA)

Abstract

PROCEDIMIENTO PARA LA OBTENCION DE MEDIOS DE REVESTIMIENTO A BASE DE DISPERSIONES ACUOSAS DE POLIURETANO.SE ADICIONAN LOS SIGUIENTES ELEMENTOS: 1.O) DE 30 A 60 EN PESO DE HEXANDIOL-1,6-POLIESTERDIOL DE PESO MOLECULAR 500 A 6.000; 2.O) DE 0 A 8 EN PESO DE UN TRIAL DE BAJO PESO MOLECULAR; 3.O) DE 3 A 30 DE UNO O VARIOS COMPUESTOS MONO O POLIVALENTES; 4.O) DE 20 A 50 DE UN DIISOCIANATO; 5.O) DE 2,5 A 20 EN PESO DE OTROS DIISOCIANATOS ALIFATICOS Y/O CICLOALIFATICOS, SE PREPARA UN PREPOLIMERO DE NCO CON GRUPOS NCO EN POSICION FINAL, BAJO PROLONGACIONDE CADENA SE TRANSFORMA CON 0,5 A 4 EN PESO DE HIDRAZINA EN UNA DISPERSION DE POLIURETANO.COMO TRIOL SE EMPLEA GLICERINA Y/O TRIMETILOLPROPANO.
ES515315A 1981-08-28 1982-08-27 Procedimiento para la obtencion de medios de revestimiento a base de dispersiones acuosas de poliuretano. Expired ES8401511A1 (es)

Applications Claiming Priority (1)

Application Number Priority Date Filing Date Title
DE19813134161 DE3134161A1 (de) 1981-08-28 1981-08-28 Ueberzugsmittel aus polyurethan-dispersionen und ihre verwendung fuer deckstriche und finishs

Publications (2)

Publication Number Publication Date
ES515315A0 ES515315A0 (es) 1983-12-16
ES8401511A1 true ES8401511A1 (es) 1983-12-16

Family

ID=6140386

Family Applications (1)

Application Number Title Priority Date Filing Date
ES515315A Expired ES8401511A1 (es) 1981-08-28 1982-08-27 Procedimiento para la obtencion de medios de revestimiento a base de dispersiones acuosas de poliuretano.

Country Status (6)

Country Link
US (2) US4594385A (es)
EP (1) EP0073392B1 (es)
CA (1) CA1241142A (es)
DE (2) DE3134161A1 (es)
ES (1) ES8401511A1 (es)
HU (1) HU196231B (es)

Families Citing this family (39)

* Cited by examiner, † Cited by third party
Publication number Priority date Publication date Assignee Title
DE3233605A1 (de) * 1982-09-10 1984-03-15 Basf Ag, 6700 Ludwigshafen Verfahren zur herstellung von vernetzten polyurethan-ionomerdispersionen
DE3309992A1 (de) * 1983-03-19 1984-09-20 Bayer Ag, 5090 Leverkusen Verfahren zum beschichten von (spalt)leder
DE3344693A1 (de) * 1983-12-10 1985-06-20 Bayer Ag, 5090 Leverkusen Waessrige loesungen oder dispersionen von polyisocyanat-polyadditionsprodukten, ein verfahren zu ihrer herstellung, sowie ihre verwendung als bzw. zur herstellung von klebemittel
DE3417265A1 (de) * 1984-05-10 1985-11-14 Bayer Ag, 5090 Leverkusen Polyurethan-dispersionen und ihre verwendung als finish-mittel
DE3521762A1 (de) * 1985-06-19 1987-01-02 Bayer Ag Ionisch modifizierte pur-streichpasten und ihre verwendung
DE3522978A1 (de) * 1985-06-27 1987-01-15 Bayer Ag Verfahren zur herstellung von lichtechten, loesungsmittelbestaendigen polyurethanharnstoffelastomerbeschichtungen im reaktiv-beschichtungsverfahren
DE3630045A1 (de) * 1986-09-04 1988-03-17 Bayer Ag Klebstoff und die verwendung des klebstoffs zur herstellung von verklebungen
DE3768246D1 (de) * 1987-01-16 1991-04-04 Agfa Gevaert Nv Bildempfangsmaterial zur verwendung in diffusionsuebertragungs-umkehrverfahren.
GB8721533D0 (en) * 1987-09-14 1987-10-21 Polyvinyl Chemical Ind Aqueous dispersions
DE3778545D1 (de) * 1987-09-29 1992-05-27 Agfa Gevaert Nv Farbstoffbildempfangsmaterial.
DE3735587A1 (de) * 1987-10-21 1989-05-11 Bayer Ag Verfahren zur herstellung von waessrigen polyurethan-polyharnstoffdispersionen
DE3736652A1 (de) 1987-10-29 1989-05-11 Bayer Ag Verfahren zur herstellung von beschichtungen
US4822685A (en) * 1987-12-10 1989-04-18 Ppg Industries, Inc. Method for preparing multi-layered coated articles and the coated articles prepared by the method
GB8904102D0 (en) * 1988-03-09 1989-04-05 Ici Resins Bv Polyurethane coating compositions
US4895894A (en) * 1988-05-31 1990-01-23 The Dow Chemical Company Modulus modification of water borne polyurethane-ureas
DE3839940A1 (de) * 1988-11-26 1990-05-31 Stockhausen Chem Fab Gmbh Waessrige polyurethan- bzw. polyurethanharnstoff-dispersionen und verfahren zum beflocken elastomerer formkoerper unter verwendung dieser dispersionen
DE3936794A1 (de) * 1989-11-04 1991-05-08 Bayer Ag Waessriges ueberzugsmittel und die verwendung von in wasser dispergierbaren polyurethanpolyharnstoffen als bindemittel
US5137967A (en) * 1990-07-06 1992-08-11 Reichhold Chemicals, Inc. Hydrazine extended aqueous polyurethane
EP0469451B1 (en) * 1990-07-25 1997-02-05 CLARK-HURTH COMPONENTS S.p.A. Three-shaft gearbox particularly for industrial vehicles in general
DE4115042A1 (de) * 1991-05-08 1992-11-12 Herberts Gmbh Physikalisch trocknendes ueberzugsmittel auf waessriger basis und dessen verwendung
DE4115015A1 (de) * 1991-05-08 1992-11-12 Herberts Gmbh Physikalisch trocknendes ueberzugsmittel auf waessriger basis und dessen verwendung
DE4125454A1 (de) * 1991-08-01 1993-02-04 Bayer Ag Beschichtungsmittel und ihre verwendung zur erzeugung wasserdampfdurchlaessiger beschichtungen
DE4129951A1 (de) * 1991-09-10 1993-03-11 Bayer Ag Beschichtungsmittel, ein verfahren zu ihrer herstellung und ihre verwendung zur herstellung von beschichtungen
US5192608A (en) * 1991-10-24 1993-03-09 Pdi, Inc. Vinyl based coatings
DE4137660A1 (de) * 1991-11-15 1993-05-19 Basf Ag Waessrige polyurethandispersionen
AU6491494A (en) * 1993-04-07 1994-10-24 Rexham Industries Corp. Method of coating microporous membranes and resulting products
DE4413562A1 (de) * 1994-04-19 1995-10-26 Herberts Gmbh Wäßrige Dispersion von Siloxanbrücken enthaltenden Polyurethanen, deren Herstellung und Verwendung in Überzugsmitteln
DE19504012A1 (de) * 1995-02-07 1996-08-14 Thomas Dr Streil Folie zur Hemmung der Diffusion oder Konvektion von Gasen
US5900457A (en) * 1996-03-05 1999-05-04 H.B. Fuller Licensing & Financing, Inc. Aqueous polyurethane dispersions formed from polyisocyanates having a methylene bridge
JP4070256B2 (ja) * 1996-10-21 2008-04-02 日華化学株式会社 ポリカーボネート系ポリウレタン樹脂組成物
US6376082B1 (en) * 1997-01-09 2002-04-23 Ellay, Inc. Exterior weatherable abrasion-resistant foldable plastic window for convertible tops
US6165239A (en) * 1997-07-28 2000-12-26 3M Innovative Properties Company Aqueous sulfopolyurea colloidal dispersions, films and abrasive articles
US6136890A (en) * 1998-02-17 2000-10-24 3M Innovative Properties Company Ink jet ink containing polyurethane dispersant
DE50004723D1 (de) 1999-02-03 2004-01-22 Basf Coatings Ag Polyurethan und seine verwendung in der wässrigen kunststofflackierung
US6517821B1 (en) 2000-07-27 2003-02-11 L'oreal Reshapable hair styling composition comprising aqueous colloidal dispersions of sulfonated polyurethane urea
US6649727B1 (en) 2000-07-27 2003-11-18 3M Innovative Properties Company Aqueous colloidal dispersions of sulfonated polyurethane ureas and products
US7147923B2 (en) * 2003-12-19 2006-12-12 3M Innovative Properties Company Flexible polymer window
DE102006012354A1 (de) * 2006-03-17 2007-09-20 Bayer Materialscience Ag Wässrige Dispersionen auf Basis von Nitrocellulose-Polyurethan-Teilchen
EP2271685B1 (en) * 2007-12-26 2018-01-03 Dow Global Technologies LLC Polyurethane dispersions and coatings produced therefrom

Family Cites Families (8)

* Cited by examiner, † Cited by third party
Publication number Priority date Publication date Assignee Title
US3262805A (en) * 1963-03-14 1966-07-26 Toyo Cloth Company Ltd Process of coating to make leather substitute and resulting article
DE1769387A1 (de) * 1968-05-17 1971-10-28 Bayer Ag Verwendung von waessrigen Polyurethan-Dispersionen zum Verkleben von weichmacherhaltigen Polyvinylchlorid-Kunststoffen
DE2035730A1 (de) * 1970-07-18 1972-01-27 Bayer Verfahren zur Herstellung wäßriger Suspensionen oder Pasten von fasrigen, vernetzten Teilchen und deren Verwendung
US4108814A (en) * 1974-09-28 1978-08-22 Bayer Aktiengesellschaft Aqueous polyurethane dispersions from solvent-free prepolymers using sulfonate diols
US4017493A (en) * 1975-06-11 1977-04-12 Gaf Corporation Textured polyurethane surface
US4045600A (en) * 1976-11-18 1977-08-30 Armstrong Cork Company Method of inhibiting plasticizer migration from plasticized poly(vinyl chloride) substrates
DE2807479A1 (de) * 1978-02-22 1979-08-23 Bayer Ag Ueberzugsmittel
DE2811148A1 (de) * 1978-03-15 1979-09-20 Bayer Ag Verfahren zur herstellung von waessrigen polyurethan-dispersionen und -loesungen

Also Published As

Publication number Publication date
US4594385A (en) 1986-06-10
CA1241142A (en) 1988-08-23
ES515315A0 (es) 1983-12-16
US4652466A (en) 1987-03-24
HU196231B (en) 1988-10-28
DE3274648D1 (en) 1987-01-22
EP0073392B1 (de) 1986-12-10
EP0073392A1 (de) 1983-03-09
DE3134161A1 (de) 1983-08-11

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