PL409040A1 - Chiral polyampholites, derivatives of dimethyl organophosphorous acid, polyalkylenepolyamines and 1- phenylethylamine and method do produce them - Google Patents

Chiral polyampholites, derivatives of dimethyl organophosphorous acid, polyalkylenepolyamines and 1- phenylethylamine and method do produce them

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Publication number
PL409040A1
PL409040A1 PL409040A PL40904014A PL409040A1 PL 409040 A1 PL409040 A1 PL 409040A1 PL 409040 A PL409040 A PL 409040A PL 40904014 A PL40904014 A PL 40904014A PL 409040 A1 PL409040 A1 PL 409040A1
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PL
Poland
Prior art keywords
phenylethylamine
fragment
polyampholyte
fragments
acid
Prior art date
Application number
PL409040A
Other languages
Polish (pl)
Other versions
PL223384B1 (en
Inventor
Mirosław Soroka
Elżbieta Wojaczyńska
Andrzej Hendrys
Iwona Sobczak
Original Assignee
Politechnika Wrocławska
Priority date (The priority date is an assumption and is not a legal conclusion. Google has not performed a legal analysis and makes no representation as to the accuracy of the date listed.)
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Publication date
Application filed by Politechnika Wrocławska filed Critical Politechnika Wrocławska
Priority to PL409040A priority Critical patent/PL223384B1/en
Publication of PL409040A1 publication Critical patent/PL409040A1/en
Publication of PL223384B1 publication Critical patent/PL223384B1/en

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Abstract

Wynalazek dotyczy poliamfolitów pochodnych kwasu dimetylofosfinowego, polialkilenopoliamin i 1 -fenyloetyloaminy o wzorze ogólnym I, w którym A oznacza fragment struktury kwasu dimetylofosfinowego, x oznacza liczbę takich fragmentów w poliamfolicie, natomiast B oznacza fragment struktury polialkilenopoliaminy, w którym n i p mogą być takie same lub różne i oznaczają liczby całkowite od 2 do 12, natomiast q jest liczbą struktur aminopolialkenowych i wynosi od 2 do 6, y oznacza liczbę fragmentów poliaminopolialkenowych w polimerze, natomiast C oznacza fragment struktury 1-fenyloetyloaminy, a z oznacza liczbę takich fragmentów w poliamfolicie, przy czym wolne miejsca fragmentu A mogą się wiązać tylko z wolnymi miejscami we fragmencie B i C. Wynalazek ujawnia również sposób wytwarzania poliamfolitów pochodnych kwasu dimetylofosfmowego, polialkilenopoliamin i 1-fenyloetyloaminy o wzorze ogólnym I, który polega na tym, że w pierwszym etapie jedną część molową kwasu fosfinowego poddaje się reakcji z co najmniej jedną częścią molową formaldehydu i co najmniej dwiema częściami molowymi grup -NH-, na które składa się suma grup -NH- pochodzących od polialkilenopoliaminy i grup -NH- pochodzących od 1-fenyloetyloaminy, a reakcję prowadzi się w temperaturze 273-373K, w wodzie, w obecności aktywatora w postaci dowolnego kwasu Bronsteda, aż do przereagowania substratów i utworzenia się poliamfolitu zawierającego fragmenty strukturalne kwasu dimetylofosfinowego, polialkilenopoliaminy i 1-fenyloetyloaminy, który w trzecim etapie poddaje się dosieciowaniu co najmniej 0,5 części molowej formaldehydu. Otrzymany w wyniku poliamfolit wydziela się z mieszaniny poreakcyjnej przez odparowanie lotnych składników pod zmniejszonym ciśnieniem, dekantację, sączenie lub wirowanie.The invention relates to polyampholytes derived from dimethylphosphinic acid, polyalkylene polyamines and 1-phenylethylamine of the general formula I, in which A is a fragment of the structure of dimethylphosphinic acid, x is the number of such fragments in the polyampholyte, and B is a fragment of the polyalkylene polyamine structure, in which n and p may be the same or different and denote integers from 2 to 12, while q is the number of aminopolyalkene structures and ranges from 2 to 6, y denotes the number of polyaminopolyalkene fragments in the polymer, while C denotes a fragment of the 1-phenylethylamine structure, and z denotes the number of such fragments in polyampholyte, where the free sites of fragment A can only bind to free sites in fragment B and C. The invention also discloses a method for preparing polyampholytes of dimethylphosphinic acid derivatives, polyalkylene polyamines and 1-phenylethylamine of the general formula I, which consists in the fact that in the first step one mole part of phosphinic acid is reacted with at least one mole part of formaldehyde and at least two mole parts of -NH- groups, which consist of the sum of -NH- groups derived from polyalkylene polyamine and -NH- groups derived from 1-phenylethylamine, and the reaction is carried out at 273-373K, in water, in the presence of an activator in the form of any Bronsted acid, until the reactants are reacted and a polyampholyte is formed containing structural fragments of dimethylphosphinic acid, polyalkylene polyamine and 1-phenylethylamine, which is cross-linked in the third stage with at least 0.5 mole part formaldehyde. The resulting polyampholyte is isolated from the post-reaction mixture by evaporation of volatile components under reduced pressure, decantation, filtration or centrifugation.

PL409040A 2014-07-31 2014-07-31 Chiral polyampholites, derivatives of dimethyl organophosphorous acid, polyalkylenepolyamines and 1- phenylethylamine and method do produce them PL223384B1 (en)

Priority Applications (1)

Application Number Priority Date Filing Date Title
PL409040A PL223384B1 (en) 2014-07-31 2014-07-31 Chiral polyampholites, derivatives of dimethyl organophosphorous acid, polyalkylenepolyamines and 1- phenylethylamine and method do produce them

Applications Claiming Priority (1)

Application Number Priority Date Filing Date Title
PL409040A PL223384B1 (en) 2014-07-31 2014-07-31 Chiral polyampholites, derivatives of dimethyl organophosphorous acid, polyalkylenepolyamines and 1- phenylethylamine and method do produce them

Publications (2)

Publication Number Publication Date
PL409040A1 true PL409040A1 (en) 2015-03-02
PL223384B1 PL223384B1 (en) 2016-10-31

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Application Number Title Priority Date Filing Date
PL409040A PL223384B1 (en) 2014-07-31 2014-07-31 Chiral polyampholites, derivatives of dimethyl organophosphorous acid, polyalkylenepolyamines and 1- phenylethylamine and method do produce them

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PL (1) PL223384B1 (en)

Also Published As

Publication number Publication date
PL223384B1 (en) 2016-10-31

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