PL439951A1 - Method of producing a biodegradable polymer composite - Google Patents

Method of producing a biodegradable polymer composite

Info

Publication number
PL439951A1
PL439951A1 PL439951A PL43995121A PL439951A1 PL 439951 A1 PL439951 A1 PL 439951A1 PL 439951 A PL439951 A PL 439951A PL 43995121 A PL43995121 A PL 43995121A PL 439951 A1 PL439951 A1 PL 439951A1
Authority
PL
Poland
Prior art keywords
sup
pla
poly
mixture
zone
Prior art date
Application number
PL439951A
Other languages
Polish (pl)
Other versions
PL244349B1 (en
Inventor
Andrzej Stasiek
Natalia Puszczykowska
Kacper Fiedurek
Jarosław Nycz
Mariusz Błaszkowski
Elżbieta Kopczyńska
Original Assignee
Sieć Badawcza Łukasiewicz - Instytut Inżynierii Materiałów Polimerowych I Barwników
Priority date (The priority date is an assumption and is not a legal conclusion. Google has not performed a legal analysis and makes no representation as to the accuracy of the date listed.)
Filing date
Publication date
Application filed by Sieć Badawcza Łukasiewicz - Instytut Inżynierii Materiałów Polimerowych I Barwników filed Critical Sieć Badawcza Łukasiewicz - Instytut Inżynierii Materiałów Polimerowych I Barwników
Priority to PL439951A priority Critical patent/PL244349B1/en
Publication of PL439951A1 publication Critical patent/PL439951A1/en
Publication of PL244349B1 publication Critical patent/PL244349B1/en

Links

Classifications

    • CCHEMISTRY; METALLURGY
    • C08ORGANIC MACROMOLECULAR COMPOUNDS; THEIR PREPARATION OR CHEMICAL WORKING-UP; COMPOSITIONS BASED THEREON
    • C08LCOMPOSITIONS OF MACROMOLECULAR COMPOUNDS
    • C08L67/00Compositions of polyesters obtained by reactions forming a carboxylic ester link in the main chain; Compositions of derivatives of such polymers
    • C08L67/04Polyesters derived from hydroxycarboxylic acids, e.g. lactones
    • BPERFORMING OPERATIONS; TRANSPORTING
    • B29WORKING OF PLASTICS; WORKING OF SUBSTANCES IN A PLASTIC STATE IN GENERAL
    • B29CSHAPING OR JOINING OF PLASTICS; SHAPING OF MATERIAL IN A PLASTIC STATE, NOT OTHERWISE PROVIDED FOR; AFTER-TREATMENT OF THE SHAPED PRODUCTS, e.g. REPAIRING
    • B29C48/00Extrusion moulding, i.e. expressing the moulding material through a die or nozzle which imparts the desired form; Apparatus therefor
    • BPERFORMING OPERATIONS; TRANSPORTING
    • B29WORKING OF PLASTICS; WORKING OF SUBSTANCES IN A PLASTIC STATE IN GENERAL
    • B29CSHAPING OR JOINING OF PLASTICS; SHAPING OF MATERIAL IN A PLASTIC STATE, NOT OTHERWISE PROVIDED FOR; AFTER-TREATMENT OF THE SHAPED PRODUCTS, e.g. REPAIRING
    • B29C48/00Extrusion moulding, i.e. expressing the moulding material through a die or nozzle which imparts the desired form; Apparatus therefor
    • B29C48/25Component parts, details or accessories; Auxiliary operations
    • B29C48/36Means for plasticising or homogenising the moulding material or forcing it through the nozzle or die
    • B29C48/395Means for plasticising or homogenising the moulding material or forcing it through the nozzle or die using screws surrounded by a cooperating barrel, e.g. single screw extruders
    • B29C48/40Means for plasticising or homogenising the moulding material or forcing it through the nozzle or die using screws surrounded by a cooperating barrel, e.g. single screw extruders using two or more parallel screws or at least two parallel non-intermeshing screws, e.g. twin screw extruders
    • B29C48/405Intermeshing co-rotating screws
    • CCHEMISTRY; METALLURGY
    • C08ORGANIC MACROMOLECULAR COMPOUNDS; THEIR PREPARATION OR CHEMICAL WORKING-UP; COMPOSITIONS BASED THEREON
    • C08KUse of inorganic or non-macromolecular organic substances as compounding ingredients
    • C08K3/00Use of inorganic substances as compounding ingredients
    • C08K3/34Silicon-containing compounds
    • CCHEMISTRY; METALLURGY
    • C08ORGANIC MACROMOLECULAR COMPOUNDS; THEIR PREPARATION OR CHEMICAL WORKING-UP; COMPOSITIONS BASED THEREON
    • C08LCOMPOSITIONS OF MACROMOLECULAR COMPOUNDS
    • C08L67/00Compositions of polyesters obtained by reactions forming a carboxylic ester link in the main chain; Compositions of derivatives of such polymers
    • C08L67/02Polyesters derived from dicarboxylic acids and dihydroxy compounds

Landscapes

  • Chemical & Material Sciences (AREA)
  • Health & Medical Sciences (AREA)
  • Chemical Kinetics & Catalysis (AREA)
  • Medicinal Chemistry (AREA)
  • Polymers & Plastics (AREA)
  • Organic Chemistry (AREA)
  • Engineering & Computer Science (AREA)
  • Mechanical Engineering (AREA)
  • Biological Depolymerization Polymers (AREA)
  • Processing And Handling Of Plastics And Other Materials For Molding In General (AREA)
  • Extrusion Moulding Of Plastics Or The Like (AREA)

Abstract

Przedmiotem zgłoszenia jest sposób wytwarzania biodegradowalnego kompozytu polimerowego na bazie poli(kwasu mlekowego) (PLA) oraz poli(adypinianu-co-tereftalanu butylenu) (PBAT) charakteryzujący się tym, że poli(kwas mlekowy) (PLA) w postaci granulek w ilości 50-70% masowych o gęstości 1240 kg/m<sup>3</sup>, masowym wskaźniku szybkości płynięcia (MFR) od 3 g/10 min. mierzonym w temperaturze 190°C pod naciskiem 2,16 kg, zawartości wilgoci (W) poniżej 0,4%, czystości stereochemicznej (zawartości L-izomerów) 96%, temperaturze topnienia 155°C i wytrzymałością na rozciąganie 45 MPa, miesza się z uprzednio zgranulowaną kompozycją polimerów poli(adypinianu-co-tereftalanu butylenu) (PBAT) i PLA w ilości 5-15% masowych o gęstości od 1370 kg/m<sup>3</sup> do 1400 kg/m<sup>3</sup>, masowym wskaźniku szybkości płynięcia (MFR) 6,75 g/10 min. mierzonym w temperaturze 135°C pod naciskiem 2,16 kg i temperaturach topnienia od 110 do 120°C oraz od 140 do 155°C, którą to mieszaninę uzupełnia się sproszkowanym talkiem w ilości 25-35% masowych, którego głównym składnikiem jest (97%) uwodniony krzemian magnezu (KWM) o mediana wielkości cząstek (D<sub>50</sub>) równą 4,5 µm, pH 9,1 i powierzchnią właściwą 6 m<sup>2</sup>/g otrzymując 100% masowych składników mieszaniny, którą miesza się mechanicznie w mieszalniku lub ręcznie, po czym tak sporządzoną mieszaninę PLA, PLA/PBAT i KWM przy pomocy wykalibrowanego dozownika wolumetrycznego wyposażonego w ślimak wprowadza się do strefy zasilania (3) wytłaczarki wieloślimakowej, korzystnie dwuślimakowej współbieżnej, w której układzie uplastyczniającym poddaje się działaniu sił ścinających w strefie sprężania (4), a następnie uplastycznioną w strefie uplastyczniania (5) i ujednorodnioną w strefie intensywnego mieszania (7) mieszaninę poprzez strefę dozowania (9) przetłacza się do głowicy wytaczarskiej formującej wyrób, który po uformowaniu w znany sposób chłodzi się i sezonuje się w temperaturze otoczenia.The subject of the application is a method of producing a biodegradable polymer composite based on poly(lactic acid) (PLA) and poly(butylene adipate-co-terephthalate) (PBAT) characterized in that poly(lactic acid) (PLA) in the form of granules in the amount of 50 -70% by mass with a density of 1240 kg/m<sup>3</sup>, a melt flow rate (MFR) from 3 g/10 min. measured at 190°C under a pressure of 2.16 kg, moisture content (W) below 0.4%, stereochemical purity (L-isomer content) 96%, melting point 155°C and tensile strength 45 MPa, mixed with previously granulated polymer composition of poly(butylene adipate-co-terephthalate) (PBAT) and PLA in the amount of 5-15% by weight with a density of 1370 kg/m<sup>3</sup> to 1400 kg/m<sup>3< /sup>, mass flow rate (MFR) 6.75 g/10 min. measured at 135°C under a pressure of 2.16 kg and melting points of 110 to 120°C and 140 to 155°C, the mixture being supplemented with talc powder in the amount of 25-35% by mass, the main component of which is (97 %) hydrated magnesium silicate (KWM) with a median particle size (D<sub>50</sub>) of 4.5 µm, pH 9.1 and a specific surface area of 6 m<sup>2</sup>/g to give 100 mass % of the components of the mixture, which is mechanically mixed in a mixer or manually, and then the mixture of PLA, PLA/PBAT and KWM prepared in this way is fed into the feed zone (3) of a multi-screw extruder, preferably a co-rotating twin screw, in whose plasticizing system is subjected to shear forces in the compression zone (4), and then plasticized in the plasticizing zone (5) and homogenized in the intensive mixing zone (7), the mixture is pumped through the dosing zone (9) to the boring head forming the product, which after formed in a known manner, cooled and seasoned at ambient temperature.

PL439951A 2021-12-21 2021-12-21 Method of producing a biodegradable polymer composite PL244349B1 (en)

Priority Applications (1)

Application Number Priority Date Filing Date Title
PL439951A PL244349B1 (en) 2021-12-21 2021-12-21 Method of producing a biodegradable polymer composite

Applications Claiming Priority (1)

Application Number Priority Date Filing Date Title
PL439951A PL244349B1 (en) 2021-12-21 2021-12-21 Method of producing a biodegradable polymer composite

Publications (2)

Publication Number Publication Date
PL439951A1 true PL439951A1 (en) 2023-06-26
PL244349B1 PL244349B1 (en) 2024-01-15

Family

ID=86945239

Family Applications (1)

Application Number Title Priority Date Filing Date
PL439951A PL244349B1 (en) 2021-12-21 2021-12-21 Method of producing a biodegradable polymer composite

Country Status (1)

Country Link
PL (1) PL244349B1 (en)

Also Published As

Publication number Publication date
PL244349B1 (en) 2024-01-15

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