ATE249102T1 - Verfahren zum beschichten einer trägerplatte und diese trägerplatte enthaltende brennstoffzelle - Google Patents

Verfahren zum beschichten einer trägerplatte und diese trägerplatte enthaltende brennstoffzelle

Info

Publication number
ATE249102T1
ATE249102T1 AT99949465T AT99949465T ATE249102T1 AT E249102 T1 ATE249102 T1 AT E249102T1 AT 99949465 T AT99949465 T AT 99949465T AT 99949465 T AT99949465 T AT 99949465T AT E249102 T1 ATE249102 T1 AT E249102T1
Authority
AT
Austria
Prior art keywords
support plate
coating
fuel cell
cell containing
titanium oxide
Prior art date
Application number
AT99949465T
Other languages
English (en)
Inventor
Robert Christiaan Makkus
Edward Bullock
Arnoldus Hermannus Hen Janssen
Michel Cassir
Original Assignee
Stichting Energie
Gemeenschappelijk Ct Voor Onde
Priority date (The priority date is an assumption and is not a legal conclusion. Google has not performed a legal analysis and makes no representation as to the accuracy of the date listed.)
Filing date
Publication date
Application filed by Stichting Energie, Gemeenschappelijk Ct Voor Onde filed Critical Stichting Energie
Application granted granted Critical
Publication of ATE249102T1 publication Critical patent/ATE249102T1/de

Links

Classifications

    • HELECTRICITY
    • H01ELECTRIC ELEMENTS
    • H01MPROCESSES OR MEANS, e.g. BATTERIES, FOR THE DIRECT CONVERSION OF CHEMICAL ENERGY INTO ELECTRICAL ENERGY
    • H01M8/00Fuel cells; Manufacture thereof
    • H01M8/02Details
    • H01M8/0202Collectors; Separators, e.g. bipolar separators; Interconnectors
    • H01M8/0204Non-porous and characterised by the material
    • H01M8/0206Metals or alloys
    • H01M8/0208Alloys
    • H01M8/021Alloys based on iron
    • CCHEMISTRY; METALLURGY
    • C23COATING METALLIC MATERIAL; COATING MATERIAL WITH METALLIC MATERIAL; CHEMICAL SURFACE TREATMENT; DIFFUSION TREATMENT OF METALLIC MATERIAL; COATING BY VACUUM EVAPORATION, BY SPUTTERING, BY ION IMPLANTATION OR BY CHEMICAL VAPOUR DEPOSITION, IN GENERAL; INHIBITING CORROSION OF METALLIC MATERIAL OR INCRUSTATION IN GENERAL
    • C23CCOATING METALLIC MATERIAL; COATING MATERIAL WITH METALLIC MATERIAL; SURFACE TREATMENT OF METALLIC MATERIAL BY DIFFUSION INTO THE SURFACE, BY CHEMICAL CONVERSION OR SUBSTITUTION; COATING BY VACUUM EVAPORATION, BY SPUTTERING, BY ION IMPLANTATION OR BY CHEMICAL VAPOUR DEPOSITION, IN GENERAL
    • C23C28/00Coating for obtaining at least two superposed coatings either by methods not provided for in a single one of groups C23C2/00 - C23C26/00 or by combinations of methods provided for in subclasses C23C and C25C or C25D
    • C23C28/30Coatings combining at least one metallic layer and at least one inorganic non-metallic layer
    • C23C28/32Coatings combining at least one metallic layer and at least one inorganic non-metallic layer including at least one pure metallic layer
    • C23C28/321Coatings combining at least one metallic layer and at least one inorganic non-metallic layer including at least one pure metallic layer with at least one metal alloy layer
    • C23C28/3215Coatings combining at least one metallic layer and at least one inorganic non-metallic layer including at least one pure metallic layer with at least one metal alloy layer at least one MCrAlX layer
    • CCHEMISTRY; METALLURGY
    • C23COATING METALLIC MATERIAL; COATING MATERIAL WITH METALLIC MATERIAL; CHEMICAL SURFACE TREATMENT; DIFFUSION TREATMENT OF METALLIC MATERIAL; COATING BY VACUUM EVAPORATION, BY SPUTTERING, BY ION IMPLANTATION OR BY CHEMICAL VAPOUR DEPOSITION, IN GENERAL; INHIBITING CORROSION OF METALLIC MATERIAL OR INCRUSTATION IN GENERAL
    • C23CCOATING METALLIC MATERIAL; COATING MATERIAL WITH METALLIC MATERIAL; SURFACE TREATMENT OF METALLIC MATERIAL BY DIFFUSION INTO THE SURFACE, BY CHEMICAL CONVERSION OR SUBSTITUTION; COATING BY VACUUM EVAPORATION, BY SPUTTERING, BY ION IMPLANTATION OR BY CHEMICAL VAPOUR DEPOSITION, IN GENERAL
    • C23C28/00Coating for obtaining at least two superposed coatings either by methods not provided for in a single one of groups C23C2/00 - C23C26/00 or by combinations of methods provided for in subclasses C23C and C25C or C25D
    • C23C28/30Coatings combining at least one metallic layer and at least one inorganic non-metallic layer
    • C23C28/32Coatings combining at least one metallic layer and at least one inorganic non-metallic layer including at least one pure metallic layer
    • C23C28/322Coatings combining at least one metallic layer and at least one inorganic non-metallic layer including at least one pure metallic layer only coatings of metal elements only
    • CCHEMISTRY; METALLURGY
    • C23COATING METALLIC MATERIAL; COATING MATERIAL WITH METALLIC MATERIAL; CHEMICAL SURFACE TREATMENT; DIFFUSION TREATMENT OF METALLIC MATERIAL; COATING BY VACUUM EVAPORATION, BY SPUTTERING, BY ION IMPLANTATION OR BY CHEMICAL VAPOUR DEPOSITION, IN GENERAL; INHIBITING CORROSION OF METALLIC MATERIAL OR INCRUSTATION IN GENERAL
    • C23CCOATING METALLIC MATERIAL; COATING MATERIAL WITH METALLIC MATERIAL; SURFACE TREATMENT OF METALLIC MATERIAL BY DIFFUSION INTO THE SURFACE, BY CHEMICAL CONVERSION OR SUBSTITUTION; COATING BY VACUUM EVAPORATION, BY SPUTTERING, BY ION IMPLANTATION OR BY CHEMICAL VAPOUR DEPOSITION, IN GENERAL
    • C23C28/00Coating for obtaining at least two superposed coatings either by methods not provided for in a single one of groups C23C2/00 - C23C26/00 or by combinations of methods provided for in subclasses C23C and C25C or C25D
    • C23C28/30Coatings combining at least one metallic layer and at least one inorganic non-metallic layer
    • C23C28/34Coatings combining at least one metallic layer and at least one inorganic non-metallic layer including at least one inorganic non-metallic material layer, e.g. metal carbide, nitride, boride, silicide layer and their mixtures, enamels, phosphates and sulphates
    • C23C28/345Coatings combining at least one metallic layer and at least one inorganic non-metallic layer including at least one inorganic non-metallic material layer, e.g. metal carbide, nitride, boride, silicide layer and their mixtures, enamels, phosphates and sulphates with at least one oxide layer
    • CCHEMISTRY; METALLURGY
    • C23COATING METALLIC MATERIAL; COATING MATERIAL WITH METALLIC MATERIAL; CHEMICAL SURFACE TREATMENT; DIFFUSION TREATMENT OF METALLIC MATERIAL; COATING BY VACUUM EVAPORATION, BY SPUTTERING, BY ION IMPLANTATION OR BY CHEMICAL VAPOUR DEPOSITION, IN GENERAL; INHIBITING CORROSION OF METALLIC MATERIAL OR INCRUSTATION IN GENERAL
    • C23CCOATING METALLIC MATERIAL; COATING MATERIAL WITH METALLIC MATERIAL; SURFACE TREATMENT OF METALLIC MATERIAL BY DIFFUSION INTO THE SURFACE, BY CHEMICAL CONVERSION OR SUBSTITUTION; COATING BY VACUUM EVAPORATION, BY SPUTTERING, BY ION IMPLANTATION OR BY CHEMICAL VAPOUR DEPOSITION, IN GENERAL
    • C23C28/00Coating for obtaining at least two superposed coatings either by methods not provided for in a single one of groups C23C2/00 - C23C26/00 or by combinations of methods provided for in subclasses C23C and C25C or C25D
    • C23C28/30Coatings combining at least one metallic layer and at least one inorganic non-metallic layer
    • C23C28/34Coatings combining at least one metallic layer and at least one inorganic non-metallic layer including at least one inorganic non-metallic material layer, e.g. metal carbide, nitride, boride, silicide layer and their mixtures, enamels, phosphates and sulphates
    • C23C28/345Coatings combining at least one metallic layer and at least one inorganic non-metallic layer including at least one inorganic non-metallic material layer, e.g. metal carbide, nitride, boride, silicide layer and their mixtures, enamels, phosphates and sulphates with at least one oxide layer
    • C23C28/3455Coatings combining at least one metallic layer and at least one inorganic non-metallic layer including at least one inorganic non-metallic material layer, e.g. metal carbide, nitride, boride, silicide layer and their mixtures, enamels, phosphates and sulphates with at least one oxide layer with a refractory ceramic layer, e.g. refractory metal oxide, ZrO2, rare earth oxides or a thermal barrier system comprising at least one refractory oxide layer
    • CCHEMISTRY; METALLURGY
    • C23COATING METALLIC MATERIAL; COATING MATERIAL WITH METALLIC MATERIAL; CHEMICAL SURFACE TREATMENT; DIFFUSION TREATMENT OF METALLIC MATERIAL; COATING BY VACUUM EVAPORATION, BY SPUTTERING, BY ION IMPLANTATION OR BY CHEMICAL VAPOUR DEPOSITION, IN GENERAL; INHIBITING CORROSION OF METALLIC MATERIAL OR INCRUSTATION IN GENERAL
    • C23CCOATING METALLIC MATERIAL; COATING MATERIAL WITH METALLIC MATERIAL; SURFACE TREATMENT OF METALLIC MATERIAL BY DIFFUSION INTO THE SURFACE, BY CHEMICAL CONVERSION OR SUBSTITUTION; COATING BY VACUUM EVAPORATION, BY SPUTTERING, BY ION IMPLANTATION OR BY CHEMICAL VAPOUR DEPOSITION, IN GENERAL
    • C23C4/00Coating by spraying the coating material in the molten state, e.g. by flame, plasma or electric discharge
    • C23C4/02Pretreatment of the material to be coated, e.g. for coating on selected surface areas
    • HELECTRICITY
    • H01ELECTRIC ELEMENTS
    • H01MPROCESSES OR MEANS, e.g. BATTERIES, FOR THE DIRECT CONVERSION OF CHEMICAL ENERGY INTO ELECTRICAL ENERGY
    • H01M8/00Fuel cells; Manufacture thereof
    • H01M8/02Details
    • H01M8/0202Collectors; Separators, e.g. bipolar separators; Interconnectors
    • H01M8/0204Non-porous and characterised by the material
    • HELECTRICITY
    • H01ELECTRIC ELEMENTS
    • H01MPROCESSES OR MEANS, e.g. BATTERIES, FOR THE DIRECT CONVERSION OF CHEMICAL ENERGY INTO ELECTRICAL ENERGY
    • H01M8/00Fuel cells; Manufacture thereof
    • H01M8/02Details
    • H01M8/0202Collectors; Separators, e.g. bipolar separators; Interconnectors
    • H01M8/0204Non-porous and characterised by the material
    • H01M8/0215Glass; Ceramic materials
    • H01M8/0217Complex oxides, optionally doped, of the type AMO3, A being an alkaline earth metal or rare earth metal and M being a metal, e.g. perovskites
    • HELECTRICITY
    • H01ELECTRIC ELEMENTS
    • H01MPROCESSES OR MEANS, e.g. BATTERIES, FOR THE DIRECT CONVERSION OF CHEMICAL ENERGY INTO ELECTRICAL ENERGY
    • H01M8/00Fuel cells; Manufacture thereof
    • H01M8/02Details
    • H01M8/0202Collectors; Separators, e.g. bipolar separators; Interconnectors
    • H01M8/0204Non-porous and characterised by the material
    • H01M8/0223Composites
    • H01M8/0228Composites in the form of layered or coated products
    • HELECTRICITY
    • H01ELECTRIC ELEMENTS
    • H01MPROCESSES OR MEANS, e.g. BATTERIES, FOR THE DIRECT CONVERSION OF CHEMICAL ENERGY INTO ELECTRICAL ENERGY
    • H01M8/00Fuel cells; Manufacture thereof
    • H01M8/02Details
    • H01M8/0202Collectors; Separators, e.g. bipolar separators; Interconnectors
    • H01M8/023Porous and characterised by the material
    • H01M8/0232Metals or alloys
    • HELECTRICITY
    • H01ELECTRIC ELEMENTS
    • H01MPROCESSES OR MEANS, e.g. BATTERIES, FOR THE DIRECT CONVERSION OF CHEMICAL ENERGY INTO ELECTRICAL ENERGY
    • H01M8/00Fuel cells; Manufacture thereof
    • H01M8/14Fuel cells with fused electrolytes
    • H01M2008/147Fuel cells with molten carbonates
    • HELECTRICITY
    • H01ELECTRIC ELEMENTS
    • H01MPROCESSES OR MEANS, e.g. BATTERIES, FOR THE DIRECT CONVERSION OF CHEMICAL ENERGY INTO ELECTRICAL ENERGY
    • H01M2300/00Electrolytes
    • H01M2300/0017Non-aqueous electrolytes
    • H01M2300/0048Molten electrolytes used at high temperature
    • H01M2300/0051Carbonates
    • YGENERAL TAGGING OF NEW TECHNOLOGICAL DEVELOPMENTS; GENERAL TAGGING OF CROSS-SECTIONAL TECHNOLOGIES SPANNING OVER SEVERAL SECTIONS OF THE IPC; TECHNICAL SUBJECTS COVERED BY FORMER USPC CROSS-REFERENCE ART COLLECTIONS [XRACs] AND DIGESTS
    • Y02TECHNOLOGIES OR APPLICATIONS FOR MITIGATION OR ADAPTATION AGAINST CLIMATE CHANGE
    • Y02EREDUCTION OF GREENHOUSE GAS [GHG] EMISSIONS, RELATED TO ENERGY GENERATION, TRANSMISSION OR DISTRIBUTION
    • Y02E60/00Enabling technologies; Technologies with a potential or indirect contribution to GHG emissions mitigation
    • Y02E60/30Hydrogen technology
    • Y02E60/50Fuel cells

Landscapes

  • Chemical & Material Sciences (AREA)
  • Engineering & Computer Science (AREA)
  • Chemical Kinetics & Catalysis (AREA)
  • Inorganic Chemistry (AREA)
  • Materials Engineering (AREA)
  • Manufacturing & Machinery (AREA)
  • Sustainable Energy (AREA)
  • Organic Chemistry (AREA)
  • General Chemical & Material Sciences (AREA)
  • Life Sciences & Earth Sciences (AREA)
  • Mechanical Engineering (AREA)
  • Sustainable Development (AREA)
  • Metallurgy (AREA)
  • Electrochemistry (AREA)
  • Ceramic Engineering (AREA)
  • Composite Materials (AREA)
  • Physics & Mathematics (AREA)
  • Plasma & Fusion (AREA)
  • Fuel Cell (AREA)
  • Other Surface Treatments For Metallic Materials (AREA)
  • Inert Electrodes (AREA)
AT99949465T 1998-10-08 1999-10-08 Verfahren zum beschichten einer trägerplatte und diese trägerplatte enthaltende brennstoffzelle ATE249102T1 (de)

Applications Claiming Priority (2)

Application Number Priority Date Filing Date Title
NL1010269A NL1010269C2 (nl) 1998-10-08 1998-10-08 Werkwijze voor het bekleden van een dragerplaat en MCFC-cel voorzien van een dergelijke dragerplaat.
PCT/NL1999/000624 WO2000021152A1 (en) 1998-10-08 1999-10-08 Method for coating a support plate and fuel cell provided with such a support plate

Publications (1)

Publication Number Publication Date
ATE249102T1 true ATE249102T1 (de) 2003-09-15

Family

ID=19767936

Family Applications (1)

Application Number Title Priority Date Filing Date
AT99949465T ATE249102T1 (de) 1998-10-08 1999-10-08 Verfahren zum beschichten einer trägerplatte und diese trägerplatte enthaltende brennstoffzelle

Country Status (10)

Country Link
US (1) US6761927B1 (de)
EP (1) EP1119881B1 (de)
JP (1) JP2002527612A (de)
AT (1) ATE249102T1 (de)
CA (1) CA2346486A1 (de)
DE (1) DE69911043T2 (de)
DK (1) DK1119881T3 (de)
ES (1) ES2211180T3 (de)
NL (1) NL1010269C2 (de)
WO (1) WO2000021152A1 (de)

Families Citing this family (12)

* Cited by examiner, † Cited by third party
Publication number Priority date Publication date Assignee Title
EP1035608A3 (de) * 1999-02-09 2003-02-05 Nisshinbo Industries, Inc. Separator für Brennstoffzellen und Festelektrolytbrennstoffzellen mit diesem Separator
US6649031B1 (en) 1999-10-08 2003-11-18 Hybrid Power Generation Systems, Llc Corrosion resistant coated fuel cell bipolar plate with filled-in fine scale porosities and method of making the same
US7144648B2 (en) * 2002-11-22 2006-12-05 The Research Foundation Of State University Of New York Bipolar plate
US20050003261A1 (en) * 2003-07-04 2005-01-06 Ayumi Horiuchi Porous fuel cell separator, method of manufacture thereof, and solid polymer fuel cell
US8338058B2 (en) 2005-02-01 2012-12-25 Neomax Materials Co., Ltd. Separator for fuel cell having intermediate layer and method for manufacturing same
US8377607B2 (en) * 2005-06-30 2013-02-19 GM Global Technology Operations LLC Fuel cell contact element including a TiO2 layer and a conductive layer
US20070003813A1 (en) * 2005-06-30 2007-01-04 General Motors Corporation Stable conductive and hydrophilic fuel cell contact element
US20070287057A1 (en) * 2006-06-09 2007-12-13 Elhamid Mahmoud H Abd Method for making a hydrophilic corrosion resistant coating on low grade stainless steel/alloys for bipolar plates
US8603703B2 (en) * 2006-07-26 2013-12-10 GM Global Technology Operations LLC Method for making super-hydrophilic and electrically conducting surfaces for fuel cell bipolar plates
US20080044716A1 (en) * 2006-08-16 2008-02-21 Gm Global Technology Operations, Inc. Durable layer structure and method for making same
JP5312855B2 (ja) * 2008-06-20 2013-10-09 東邦瓦斯株式会社 インターコネクタおよびその製造方法
GB201910455D0 (en) * 2019-07-22 2019-09-04 Teer Coatings Ltd Coating for the surface of an article and process for forming the coating

Family Cites Families (11)

* Cited by examiner, † Cited by third party
Publication number Priority date Publication date Assignee Title
DE2619417A1 (de) * 1976-05-03 1977-11-24 Walter H R Ott Verfahren zur herstellung von festhaftenden auftragungen im thermischen spritzverfahren mit dem spritzzusatzwerkstoff titan ausgefuehrt
US4226897A (en) * 1977-12-05 1980-10-07 Plasma Physics Corporation Method of forming semiconducting materials and barriers
JPH0192350A (ja) * 1987-10-01 1989-04-11 Osaka Gas Co Ltd 伝熱面の処理方法
US5805973A (en) * 1991-03-25 1998-09-08 General Electric Company Coated articles and method for the prevention of fuel thermal degradation deposits
JPH05339748A (ja) * 1992-06-10 1993-12-21 Mitsubishi Heavy Ind Ltd 複合皮膜の製造方法
US5287730A (en) * 1992-06-18 1994-02-22 Securus, Inc. Plumbing leakage test apparatus and method of use
CN1109126C (zh) * 1993-12-28 2003-05-21 西铁城钟表有限公司 白色覆饰件及其生产方法
DE19523637C2 (de) * 1994-12-27 1997-08-14 Mtu Friedrichshafen Gmbh Verfahren zur Herstellung einer Korrosionsschutzbeschichtung, Substrat mit einer Korrosionsschutzbeschichtung sowie Verwendung eines solchen Substrats
WO1996035825A1 (de) * 1995-05-08 1996-11-14 Helmut Tannenberger Werkstück für anwendungen bei hohen temperaturen und verfahren zu seiner herstellung
DE19628823C2 (de) * 1996-07-17 1998-08-20 Mtu Friedrichshafen Gmbh Stromführendes Bauteil für eine Schmelzkarbonatbrennstoffzelle mit Korrosionsschutzbeschichtung
US6335105B1 (en) * 1999-06-21 2002-01-01 General Electric Company Ceramic superalloy articles

Also Published As

Publication number Publication date
NL1010269C2 (nl) 2000-04-11
WO2000021152A1 (en) 2000-04-13
EP1119881B1 (de) 2003-09-03
EP1119881A1 (de) 2001-08-01
US6761927B1 (en) 2004-07-13
DE69911043D1 (de) 2003-10-09
ES2211180T3 (es) 2004-07-01
DK1119881T3 (da) 2003-12-08
DE69911043T2 (de) 2004-06-03
JP2002527612A (ja) 2002-08-27
CA2346486A1 (en) 2000-04-13

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