CN102995446A - Attapulgite-modified polyvinyl chloride synthetic leather and manufacturing method thereof - Google Patents

Attapulgite-modified polyvinyl chloride synthetic leather and manufacturing method thereof Download PDF

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Publication number
CN102995446A
CN102995446A CN2012104064893A CN201210406489A CN102995446A CN 102995446 A CN102995446 A CN 102995446A CN 2012104064893 A CN2012104064893 A CN 2012104064893A CN 201210406489 A CN201210406489 A CN 201210406489A CN 102995446 A CN102995446 A CN 102995446A
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polyvinyl chloride
synthetic leather
surface layer
slurry
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CN2012104064893A
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CN102995446B (en
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藏德虎
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HEFEI ANSHAN COATING FABRICS CO Ltd
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HEFEI ANSHAN COATING FABRICS CO Ltd
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Abstract

The invention discloses attapulgite-modified polyvinyl chloride (PVC) synthetic leather. The attapulgite-modified PVC synthetic leather comprises a surface layer, a foamed layer, a bonding layer and a brushing fabric, and is characterized in that the surface layer is prepared by mixing the following raw materials in parts by weight to form slurry: 70 to 80 parts of SG-2 type PVC resin, 30 to 40 parts of SG-5 type PVC resin, 10 to 15 parts of triethyl citrate, 30 to 35 parts of epoxy butyl oleate, 20 to 25 parts of n-butyl methacrylate, 5 to 6 parts of PVC color paste, 1 to 2 parts of dibasic lead phosphate, 1 to 2 parts of tribasic lead sulfate and 5 to 10 parts of modified diatomite. Through the improvements of the formula and the process, the flexibility of the synthetic leather is improved, and the synthetic leather has a natural comfortable hand feeling similar to that of natural leather and is difficult to damage or tear after being used for 3 to 5 years.

Description

Attapulgite modified polyvinyl chloride synthetic leather and manufacture method thereof
Technical field
The invention belongs to a kind of chemical synthesis leather facing material processing technique field, specifically a kind of attapulgite modified polyvinyl chloride synthetic leather and manufacture method thereof.
Background technology
At present, the field of furniture such as commercial family property and family expenses family property extensively adopts polyurethane and attapulgite modified polyvinyl chloride synthetic leather.Synthetic Leather has the advantages such as emulation height, good hand touch, obtains the extensive favor in market.Yet a large amount of the use has certain toxicity and volatile DMF solvent in its manufacture process, even also can have abundant residues through sufficient dry DMF, becomes the source that room air VOC exceeds standard and pollutes; Simultaneously, Synthetic Leather is because the problems such as hydrolysis, weatherability deficiency have limited its further extensive use.Attapulgite modified polyvinyl chloride synthetic leather has excellent hydrolysis, wear-resisting, scratch resistance, the advantage such as fire-retardant, but the product quality existing problems.
Summary of the invention
The object of the present invention is to provide a kind of attapulgite modified polyvinyl chloride synthetic leather and manufacture method thereof, the synthetic leather good product quality of production.
Purpose of the present invention can be achieved through the following technical solutions:
A kind of attapulgite modified polyvinyl chloride synthetic leather comprises surface layer, foaming layer and adhesive linkage, nylon loop, it is characterized in that:
Described surface layer is made into slurry by following raw materials in part by weight and makes:
SG-2 type polyvinyl chloride resin 70-80, SG-5 type polyvinyl chloride resin 30-40, triethyl citrate 10-15, epoxyoleic acid butyl ester 30-35, n-BMA 20-25, PVC color 5-6, dibasic lead phosphite 1-2, lead sulfate tribasic 1-2, modification infusorial earth 5-10, aluminium oxide 30-35, nano-calcium carbonate 40-45, the fast carbon black N660 20-25 that extrudes, titanate coupling agent TMC-TTS 1-2, irgasfos 168 1-2, the N-2-(aminoethyl)-3-aminopropyl trimethoxysilane 1-2, Silane coupling agent KH550 1-2, protein powder 3-4;
Described foaming layer is made into slurry by following raw materials in part by weight and makes:
SG-4 type polyvinyl chloride resin 40-50, SG-6 type polyvinyl chloride resin 70-80, adipic acid propanediol polyester 30-35, n-BMA 25-30, decanedioic acid propanediol polyester 15-20, n-BMA 20-25, unifor 1-2, blowing agent (461DU40) 1-2, sodium sulfate of polyethenoxy ether of fatty alcohol 1-2, Imarcaptoacetate dioctyltin 1-2, calcium stearate 1-2, dimethyl dimercapto 2-ethyl hexyl ethanoate tin 1-2, attapulgite modified 5-10, carbon black N220 40-45, precipitated silica 30-35, antioxidant 1010 1-2,3-aminopropyl trimethoxysilane 2-3, crosslinking agent TAC 1-2;
Described attapulgite modified by the following method preparation:
With attapulgite at 750-800 ℃ of lower roasting 4-5 hour, after put into the 10-15% hydrochloric acid solution and soak after 3-4 hour, pull out, dry to moisture 2-3%, add the dibutyl maleate of titanate coupling agent TMC-TTS, the 3-4% of the nano-carbon powder be equivalent to its weight 5-8%, 3-4%, the calcium stearate of 3-4%, mix, stirred 30-50 minute oven dry, pulverize at 60-70 ℃ of lower 3500-4000 rev/min;
Described modified alta-mud prepares by the following method:
(1) bentonite is used 10-15% salt acid soak 3-4 hour, and the deionized water washing was soaked 3-4 hour with the 10-12% sodium hydroxide solution again, and is extremely neutral with the deionized water washing again, oven dry;
(2) add the sldium lauryl sulfate of the sodium phosphate trimer be equivalent to its weight 3-5%, 3-5% aluminium hydroxide, 2-3% in the oven dry bentonite, 60-70 ℃ of lower the stirring 40-50 minute, dry, be ground into powder.
The manufacture method of described attapulgite modified polyvinyl chloride synthetic leather is characterized in that adopting release liners knife coating technique:
(1), stir after the surface layer raw material mixed, mixing speed is 1200-1500 rev/min, and mixing time is 1-2 hour, filters to get surface layer slurry,
(2), then release liners is preheated to 60-70 ℃, with surface layer slurry with 150-200g/m 2The blade coating amount be coated with and scrape the release liners surface, 160-165 ℃ of lower plasticizing film forming;
(3), stir after will the foaming layer slurry mixing, mixing speed is 1200-1500 rev/min, filters to get the foaming layer slurry;
(4), the foaming layer slurry is coated on the surface layer, under 160-180 ℃, foam;
(5), re-use the aqueous polyurethane slurry and as adhesive linkage foaming layer and nylon loop fitted, binding temperature is 120-130 ℃, peels off at last rolling.
Beneficial effect of the present invention:
(1), the present invention is by prescription and process modification, increased the pliability of synthetic leather, have to be similar to the naturally comfortable feel that natural leather has; 3-5 is not easy breakage or tears damage.
(2), adopt aqueous polyurethane coating, can keep permanent and higher firmness.
(3), attapulgite modified, modified Nano bentonite has preferably thoroughly vapour moisture absorption conductibility, so that synthetic leather of the present invention is realized the needs of good ventilative moisture absorbing.
(4), synthetic leather of the present invention, all surpass the standard of similar environment-friendly type artificial leather on the market in feel, outward appearance and comfort level, reach respective standard in physics, chemical property, also can be by various strict environmental protection barriers tests.
The specific embodiment
A kind of attapulgite modified polyvinyl chloride synthetic leather comprises surface layer, foaming layer and adhesive linkage, nylon loop,
Described surface layer is made into slurry and is made by following weight portion (kilogram) raw material:
SG-2 type polyvinyl chloride resin 70, SG-5 type polyvinyl chloride resin 30, triethyl citrate 15, epoxyoleic acid butyl ester 30, n-BMA 25, PVC color 6, dibasic lead phosphite 2, lead sulfate tribasic 1, modification infusorial earth 5, aluminium oxide 35, nano-calcium carbonate Ca45, extrude carbon black N660 25, titanate coupling agent TMC-TTS 1, irgasfos 168 1, N-2-(aminoethyl soon)-3-aminopropyl trimethoxysilane 1, Silane coupling agent KH550 2, protein powder 3;
Described foaming layer is made into slurry and is made by following weight portion (kilogram) raw material:
SG-4 type polyvinyl chloride resin 40, SG-6 type polyvinyl chloride resin 80, adipic acid propanediol polyester 35, n-BMA 25, decanedioic acid propanediol polyester 20, n-BMA 25, unifor 2, blowing agent (461DU40) 2, sodium sulfate of polyethenoxy ether of fatty alcohol 1, Imarcaptoacetate dioctyltin 1, calcium stearate 1, dimethyl dimercapto 2-ethyl hexyl ethanoate tin 1, attapulgite modified 10, carbon black N220 40, precipitated silica 30, antioxidant 1010 2,3-aminopropyl trimethoxysilane 2, crosslinking agent TAC 1;
Described attapulgite modified by the following method preparation:
With attapulgite at 780-800 ℃ of lower roasting 4-5 hour, after put into 12% hydrochloric acid solution and soak after 3 hours, pull out, dry to moisture 2-3%, add and be equivalent to the nano-carbon powder of its weight 5%, 4% titanate coupling agent TMC-TTS, 3% dibutyl maleate, 4% calcium stearate, mix, stirred 30-40 minute oven dry, pulverize at 60-70 ℃ of lower 3500-4000 rev/min;
Described modified alta-mud prepares by the following method:
(1) bentonite was with 12% salt acid soak 3 hours, and the deionized water washing was soaked 3 hours with 10% sodium hydroxide solution again, again with the deionized water washing to neutral, dry;
(2) add the sodium phosphate trimer be equivalent to its weight 5%, 3% aluminium hydroxide, 2% sldium lauryl sulfate in the oven dry bentonite, 60-70 ℃ of lower the stirring 40-50 minute, dry, be ground into powder.
The described gloves manufacture method of polyvinyl chloride synthetic leather, adopt release liners knife coating technique:
(1), stir after the surface layer raw material mixed, mixing speed is 1200-1500 rev/min, and mixing time is 1-2 hour, filters to get surface layer slurry,
(2), then release liners is preheated to 60-70 ℃, with surface layer slurry with 180g/m 2The blade coating amount be coated with and scrape the release liners surface, 160-165 ℃ of lower plasticizing film forming;
(3), stir after will the foaming layer slurry mixing, mixing speed is 1200-1500 rev/min, filters to get the foaming layer slurry;
(4), the foaming layer slurry is coated on the surface layer, under 175-180 ℃, foam;
(5), re-use the aqueous polyurethane slurry and as adhesive linkage foaming layer and nylon loop fitted, binding temperature is 120-130 ℃, peels off at last rolling.
Synthetic leather physical and chemical performance of the present invention is as follows:
Stretch breaking strength/broadwise stretch breaking strength radially〉350N/3CM, directly/and filling-tear resistance〉25N ,-10 ℃ of low temperature flexibility can reach anti-tortuous 30,000 times, and degradation does not ftracture, and has ventilative and hygroscopicity; Harmful element is detected, can pass through REACH46 item environmental protection test.

Claims (2)

1. an attapulgite modified polyvinyl chloride synthetic leather comprises surface layer, foaming layer and adhesive linkage, nylon loop, it is characterized in that:
Described surface layer is made into slurry by following raw materials in part by weight and makes:
SG-2 type polyvinyl chloride resin 70-80, SG-5 type polyvinyl chloride resin 30-40, triethyl citrate 10-15, epoxyoleic acid butyl ester 30-35, n-BMA 20-25, PVC color 5-6, dibasic lead phosphite 1-2, lead sulfate tribasic 1-2, modification infusorial earth 5-10, aluminium oxide 30-35, nano-calcium carbonate 40-45, the fast carbon black N660 20-25 that extrudes, titanate coupling agent TMC-TTS 1-2, irgasfos 168 1-2, the N-2-(aminoethyl)-3-aminopropyl trimethoxysilane 1-2, Silane coupling agent KH550 1-2, protein powder 3-4;
Described foaming layer is made into slurry by following raw materials in part by weight and makes:
SG-4 type polyvinyl chloride resin 40-50, SG-6 type polyvinyl chloride resin 70-80, adipic acid propanediol polyester 30-35, n-BMA 25-30, decanedioic acid propanediol polyester 15-20, n-BMA 20-25, unifor 1-2, blowing agent (461DU40) 1-2, sodium sulfate of polyethenoxy ether of fatty alcohol 1-2, Imarcaptoacetate dioctyltin 1-2, calcium stearate 1-2, dimethyl dimercapto 2-ethyl hexyl ethanoate tin 1-2, attapulgite modified 5-10, carbon black N220 40-45, precipitated silica 30-35, antioxidant 1010 1-2,3-aminopropyl trimethoxysilane 2-3, crosslinking agent TAC 1-2;
Described attapulgite modified by the following method preparation:
With attapulgite at 750-800 ℃ of lower roasting 4-5 hour, after put into the 10-15% hydrochloric acid solution and soak after 3-4 hour, pull out, dry to moisture 2-3%, add the dibutyl maleate of titanate coupling agent TMC-TTS, the 3-4% of the nano-carbon powder be equivalent to its weight 5-8%, 3-4%, the calcium stearate of 3-4%, mix, stirred 30-50 minute oven dry, pulverize at 60-70 ℃ of lower 3500-4000 rev/min;
Described modified alta-mud prepares by the following method:
(1) bentonite is used 10-15% salt acid soak 3-4 hour, and the deionized water washing was soaked 3-4 hour with the 10-12% sodium hydroxide solution again, and is extremely neutral with the deionized water washing again, oven dry;
(2) add the sldium lauryl sulfate of the sodium phosphate trimer be equivalent to its weight 3-5%, 3-5% aluminium hydroxide, 2-3% in the oven dry bentonite, 60-70 ℃ of lower the stirring 40-50 minute, dry, be ground into powder.
2. the manufacture method of attapulgite modified polyvinyl chloride synthetic leather according to claim 1 is characterized in that adopting release liners knife coating technique:
(1), stir after the surface layer raw material mixed, mixing speed is 1200-1500 rev/min, and mixing time is 1-2 hour, filters to get surface layer slurry,
(2), then release liners is preheated to 60-70 ℃, with surface layer slurry with 150-200g/m 2The blade coating amount be coated with and scrape the release liners surface, 160-165 ℃ of lower plasticizing film forming;
(3), stir after will the foaming layer slurry mixing, mixing speed is 1200-1500 rev/min, filters to get the foaming layer slurry;
(4), the foaming layer slurry is coated on the surface layer, under 160-180 ℃, foam;
(5), re-use the aqueous polyurethane slurry and as adhesive linkage foaming layer and nylon loop fitted, binding temperature is 120-130 ℃, peels off at last rolling.
CN201210406489.3A 2012-10-23 2012-10-23 Attapulgite-modified polyvinyl chloride synthetic leather and manufacturing method thereof Expired - Fee Related CN102995446B (en)

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Cited By (17)

* Cited by examiner, † Cited by third party
Publication number Priority date Publication date Assignee Title
CN103352372A (en) * 2013-07-03 2013-10-16 六安三希皮革制品有限公司 PVC synthetic leather for cases and preparation method thereof
CN103352376A (en) * 2013-07-03 2013-10-16 六安三希皮革制品有限公司 PVC synthetic leather for shoe vamps of high-grade sports shoes and production method thereof
CN103642094A (en) * 2013-11-15 2014-03-19 蚌埠赛英电子科技发展有限公司 Rubber gasket material used for valves, and preparation method thereof
CN103694513A (en) * 2013-11-29 2014-04-02 马鞍山市中澜橡塑制品有限公司 Modified rubber composite sealing gasket material and preparation method thereof
CN103694512A (en) * 2013-11-29 2014-04-02 马鞍山市中澜橡塑制品有限公司 Butadiene-acrylonitrile rubber and fluororubber composite sealing gasket material and preparation method thereof
CN103694510A (en) * 2013-11-29 2014-04-02 马鞍山市中澜橡塑制品有限公司 Attapulgite-modified nitrile rubber sealing pad material and preparation method thereof
CN103694511A (en) * 2013-11-29 2014-04-02 马鞍山市中澜橡塑制品有限公司 Modified nitrile rubber gasket material and preparation method thereof
CN103694515A (en) * 2013-11-29 2014-04-02 马鞍山市中澜橡塑制品有限公司 Butadiene-acrylonitrile rubber sealing gasket material modified by adding attapulgite and preparation method thereof
CN103709471A (en) * 2013-11-29 2014-04-09 马鞍山市中澜橡塑制品有限公司 Safe and non-toxic rubber sealing gasket material and its preparation method
CN104098933A (en) * 2014-07-15 2014-10-15 淮阴工学院 Preparation method for attapulgite clay/calcium carbonate composite filling for polyurethane leather
CN104213428A (en) * 2014-09-23 2014-12-17 安徽登克尔旅游用品有限公司 Polyvinyl chloride (PVC) synthetic leather and production method thereof for bags and suitcases
CN104312090A (en) * 2014-10-25 2015-01-28 合肥市安山涂层织物有限公司 Anti-aging synthetic leather slurry and preparation method thereof
CN106192447A (en) * 2015-05-04 2016-12-07 蒋华 A kind of method that attapulgite clay produces Synthetic Leather as filler
CN106589787A (en) * 2016-12-07 2017-04-26 合肥市安山涂层织物有限公司 Weather-fastness synthetic leather slurry and preparation method thereof
CN108486905A (en) * 2018-05-07 2018-09-04 安徽索亚装饰材料有限公司 A kind of artificial leather synthetic method for skin carving Soft Roll
CN108755173A (en) * 2018-05-07 2018-11-06 安徽索亚装饰材料有限公司 A kind of skin carving artificial leather treatment process
CN108998988A (en) * 2018-06-22 2018-12-14 安徽索亚装饰材料有限公司 A kind of degradable PVC decorative artificial leather of Environment-friendlywear-resistant wear-resistant

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CN101349013A (en) * 2008-08-29 2009-01-21 黄成源 A kind of manufacturing method and automatic assembly line of ecological artificial leather or similar leather
CN102505513A (en) * 2011-11-05 2012-06-20 合肥市安山涂层织物有限公司 Gas-permeable moisture-absorption type environmentally-friendly polyvinyl chloride synthetic leather and manufacturing method thereof

Patent Citations (5)

* Cited by examiner, † Cited by third party
Publication number Priority date Publication date Assignee Title
US4575471A (en) * 1983-11-28 1986-03-11 Wong Winston W Structure of dual-face artificial leather and method of manufacture thereof
JPH05311581A (en) * 1992-04-30 1993-11-22 Kanto Leather Cloth Co Ltd Method for manufacturing sheet material
KR100873655B1 (en) * 2007-07-27 2008-12-12 (주)아이앤에스 Flame retardant FISH foam artificial leather and its manufacturing method
CN101349013A (en) * 2008-08-29 2009-01-21 黄成源 A kind of manufacturing method and automatic assembly line of ecological artificial leather or similar leather
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Cited By (21)

* Cited by examiner, † Cited by third party
Publication number Priority date Publication date Assignee Title
CN103352372B (en) * 2013-07-03 2015-12-23 六安三希皮革制品有限公司 Case and bag PVC synthetic leather and preparation method thereof
CN103352376A (en) * 2013-07-03 2013-10-16 六安三希皮革制品有限公司 PVC synthetic leather for shoe vamps of high-grade sports shoes and production method thereof
CN103352372A (en) * 2013-07-03 2013-10-16 六安三希皮革制品有限公司 PVC synthetic leather for cases and preparation method thereof
CN103352376B (en) * 2013-07-03 2015-12-23 六安三希皮革制品有限公司 Vamp PVC synthetic leather of high-grade sport footwear and preparation method thereof
CN103642094A (en) * 2013-11-15 2014-03-19 蚌埠赛英电子科技发展有限公司 Rubber gasket material used for valves, and preparation method thereof
CN103642094B (en) * 2013-11-15 2016-03-30 蚌埠赛英电子科技发展有限公司 A kind of valve Rubber gasket material and preparation method thereof
CN103694513A (en) * 2013-11-29 2014-04-02 马鞍山市中澜橡塑制品有限公司 Modified rubber composite sealing gasket material and preparation method thereof
CN103694512A (en) * 2013-11-29 2014-04-02 马鞍山市中澜橡塑制品有限公司 Butadiene-acrylonitrile rubber and fluororubber composite sealing gasket material and preparation method thereof
CN103694510A (en) * 2013-11-29 2014-04-02 马鞍山市中澜橡塑制品有限公司 Attapulgite-modified nitrile rubber sealing pad material and preparation method thereof
CN103694511A (en) * 2013-11-29 2014-04-02 马鞍山市中澜橡塑制品有限公司 Modified nitrile rubber gasket material and preparation method thereof
CN103694515A (en) * 2013-11-29 2014-04-02 马鞍山市中澜橡塑制品有限公司 Butadiene-acrylonitrile rubber sealing gasket material modified by adding attapulgite and preparation method thereof
CN103709471A (en) * 2013-11-29 2014-04-09 马鞍山市中澜橡塑制品有限公司 Safe and non-toxic rubber sealing gasket material and its preparation method
CN104098933B (en) * 2014-07-15 2016-04-13 淮阴工学院 For the recessed soil/Calcium Carbonate Composite Fillers preparation method of polyurethane leather
CN104098933A (en) * 2014-07-15 2014-10-15 淮阴工学院 Preparation method for attapulgite clay/calcium carbonate composite filling for polyurethane leather
CN104213428A (en) * 2014-09-23 2014-12-17 安徽登克尔旅游用品有限公司 Polyvinyl chloride (PVC) synthetic leather and production method thereof for bags and suitcases
CN104312090A (en) * 2014-10-25 2015-01-28 合肥市安山涂层织物有限公司 Anti-aging synthetic leather slurry and preparation method thereof
CN106192447A (en) * 2015-05-04 2016-12-07 蒋华 A kind of method that attapulgite clay produces Synthetic Leather as filler
CN106589787A (en) * 2016-12-07 2017-04-26 合肥市安山涂层织物有限公司 Weather-fastness synthetic leather slurry and preparation method thereof
CN108486905A (en) * 2018-05-07 2018-09-04 安徽索亚装饰材料有限公司 A kind of artificial leather synthetic method for skin carving Soft Roll
CN108755173A (en) * 2018-05-07 2018-11-06 安徽索亚装饰材料有限公司 A kind of skin carving artificial leather treatment process
CN108998988A (en) * 2018-06-22 2018-12-14 安徽索亚装饰材料有限公司 A kind of degradable PVC decorative artificial leather of Environment-friendlywear-resistant wear-resistant

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