ES2129969T3 - Interpolimeros elastomericos de isomonoolefinas c{sub,4} c{sub,7} y para - alquilestireno con funcionalidad ester - Google Patents

Interpolimeros elastomericos de isomonoolefinas c{sub,4} c{sub,7} y para - alquilestireno con funcionalidad ester

Info

Publication number
ES2129969T3
ES2129969T3 ES96916853T ES96916853T ES2129969T3 ES 2129969 T3 ES2129969 T3 ES 2129969T3 ES 96916853 T ES96916853 T ES 96916853T ES 96916853 T ES96916853 T ES 96916853T ES 2129969 T3 ES2129969 T3 ES 2129969T3
Authority
ES
Spain
Prior art keywords
sub
free
estirene
isomonoolefins
alkyl
Prior art date
Legal status (The legal status is an assumption and is not a legal conclusion. Google has not performed a legal analysis and makes no representation as to the accuracy of the status listed.)
Expired - Lifetime
Application number
ES96916853T
Other languages
English (en)
Inventor
Bernard Jean Costemalle
James Vincent Fusco
Pierre Therese Hous
Hsien-Chang Wang
Current Assignee (The listed assignees may be inaccurate. Google has not performed a legal analysis and makes no representation or warranty as to the accuracy of the list.)
ExxonMobil Chemical Patents Inc
Original Assignee
Exxon Chemical Patents Inc
Priority date (The priority date is an assumption and is not a legal conclusion. Google has not performed a legal analysis and makes no representation as to the accuracy of the date listed.)
Filing date
Publication date
Application filed by Exxon Chemical Patents Inc filed Critical Exxon Chemical Patents Inc
Application granted granted Critical
Publication of ES2129969T3 publication Critical patent/ES2129969T3/es
Anticipated expiration legal-status Critical
Expired - Lifetime legal-status Critical Current

Links

Classifications

    • B—PERFORMING OPERATIONS; TRANSPORTING
    • B60—VEHICLES IN GENERAL
    • B60C—VEHICLE TYRES; TYRE INFLATION; TYRE CHANGING; CONNECTING VALVES TO INFLATABLE ELASTIC BODIES IN GENERAL; DEVICES OR ARRANGEMENTS RELATED TO TYRES
    • B60C1/00—Tyres characterised by the chemical composition or the physical arrangement or mixture of the composition
    • B60C1/0008—Compositions of the inner liner
    • C—CHEMISTRY; METALLURGY
    • C08—ORGANIC MACROMOLECULAR COMPOUNDS; THEIR PREPARATION OR CHEMICAL WORKING-UP; COMPOSITIONS BASED THEREON
    • C08F—MACROMOLECULAR COMPOUNDS OBTAINED BY REACTIONS ONLY INVOLVING CARBON-TO-CARBON UNSATURATED BONDS
    • C08F212/00—Copolymers of compounds having one or more unsaturated aliphatic radicals, each having only one carbon-to-carbon double bond, and at least one being terminated by an aromatic carbocyclic ring
    • C08F212/02—Monomers containing only one unsaturated aliphatic radical
    • C08F212/04—Monomers containing only one unsaturated aliphatic radical containing one ring
    • C08F212/06—Hydrocarbons
    • C08F212/12—Monomers containing a branched unsaturated aliphatic radical or a ring substituted by an alkyl radical
    • C—CHEMISTRY; METALLURGY
    • C08—ORGANIC MACROMOLECULAR COMPOUNDS; THEIR PREPARATION OR CHEMICAL WORKING-UP; COMPOSITIONS BASED THEREON
    • C08F—MACROMOLECULAR COMPOUNDS OBTAINED BY REACTIONS ONLY INVOLVING CARBON-TO-CARBON UNSATURATED BONDS
    • C08F210/00—Copolymers of unsaturated aliphatic hydrocarbons having only one carbon-to-carbon double bond
    • C08F210/04—Monomers containing three or four carbon atoms
    • C08F210/08—Butenes
    • C08F210/10—Isobutene
    • C—CHEMISTRY; METALLURGY
    • C08—ORGANIC MACROMOLECULAR COMPOUNDS; THEIR PREPARATION OR CHEMICAL WORKING-UP; COMPOSITIONS BASED THEREON
    • C08K—Use of inorganic or non-macromolecular organic substances as compounding ingredients
    • C08K3/00—Use of inorganic substances as compounding ingredients
    • C08K3/01—Use of inorganic substances as compounding ingredients characterized by their specific function
    • C08K3/011—Crosslinking or vulcanising agents, e.g. accelerators
    • C—CHEMISTRY; METALLURGY
    • C08—ORGANIC MACROMOLECULAR COMPOUNDS; THEIR PREPARATION OR CHEMICAL WORKING-UP; COMPOSITIONS BASED THEREON
    • C08K—Use of inorganic or non-macromolecular organic substances as compounding ingredients
    • C08K3/00—Use of inorganic substances as compounding ingredients
    • C08K3/01—Use of inorganic substances as compounding ingredients characterized by their specific function
    • C08K3/013—Fillers, pigments or reinforcing additives
    • C—CHEMISTRY; METALLURGY
    • C08—ORGANIC MACROMOLECULAR COMPOUNDS; THEIR PREPARATION OR CHEMICAL WORKING-UP; COMPOSITIONS BASED THEREON
    • C08K—Use of inorganic or non-macromolecular organic substances as compounding ingredients
    • C08K3/00—Use of inorganic substances as compounding ingredients
    • C08K3/02—Elements
    • C08K3/04—Carbon
    • C—CHEMISTRY; METALLURGY
    • C08—ORGANIC MACROMOLECULAR COMPOUNDS; THEIR PREPARATION OR CHEMICAL WORKING-UP; COMPOSITIONS BASED THEREON
    • C08K—Use of inorganic or non-macromolecular organic substances as compounding ingredients
    • C08K3/00—Use of inorganic substances as compounding ingredients
    • C08K3/02—Elements
    • C08K3/06—Sulfur
    • C—CHEMISTRY; METALLURGY
    • C08—ORGANIC MACROMOLECULAR COMPOUNDS; THEIR PREPARATION OR CHEMICAL WORKING-UP; COMPOSITIONS BASED THEREON
    • C08K—Use of inorganic or non-macromolecular organic substances as compounding ingredients
    • C08K5/00—Use of organic ingredients
    • C08K5/0008—Organic ingredients according to more than one of the "one dot" groups of C08K5/01 - C08K5/59
    • C08K5/0016—Plasticisers
    • C—CHEMISTRY; METALLURGY
    • C08—ORGANIC MACROMOLECULAR COMPOUNDS; THEIR PREPARATION OR CHEMICAL WORKING-UP; COMPOSITIONS BASED THEREON
    • C08K—Use of inorganic or non-macromolecular organic substances as compounding ingredients
    • C08K5/00—Use of organic ingredients
    • C08K5/0008—Organic ingredients according to more than one of the "one dot" groups of C08K5/01 - C08K5/59
    • C08K5/0025—Crosslinking or vulcanising agents; including accelerators
    • C—CHEMISTRY; METALLURGY
    • C08—ORGANIC MACROMOLECULAR COMPOUNDS; THEIR PREPARATION OR CHEMICAL WORKING-UP; COMPOSITIONS BASED THEREON
    • C08K—Use of inorganic or non-macromolecular organic substances as compounding ingredients
    • C08K5/00—Use of organic ingredients
    • C08K5/01—Hydrocarbons
    • C—CHEMISTRY; METALLURGY
    • C08—ORGANIC MACROMOLECULAR COMPOUNDS; THEIR PREPARATION OR CHEMICAL WORKING-UP; COMPOSITIONS BASED THEREON
    • C08K—Use of inorganic or non-macromolecular organic substances as compounding ingredients
    • C08K5/00—Use of organic ingredients
    • C08K5/04—Oxygen-containing compounds
    • C08K5/14—Peroxides
    • C—CHEMISTRY; METALLURGY
    • C08—ORGANIC MACROMOLECULAR COMPOUNDS; THEIR PREPARATION OR CHEMICAL WORKING-UP; COMPOSITIONS BASED THEREON
    • C08L—COMPOSITIONS OF MACROMOLECULAR COMPOUNDS
    • C08L21/00—Compositions of unspecified rubbers
    • C—CHEMISTRY; METALLURGY
    • C08—ORGANIC MACROMOLECULAR COMPOUNDS; THEIR PREPARATION OR CHEMICAL WORKING-UP; COMPOSITIONS BASED THEREON
    • C08L—COMPOSITIONS OF MACROMOLECULAR COMPOUNDS
    • C08L23/00—Compositions of homopolymers or copolymers of unsaturated aliphatic hydrocarbons having only one carbon-to-carbon double bond; Compositions of derivatives of such polymers
    • C08L23/02—Compositions of homopolymers or copolymers of unsaturated aliphatic hydrocarbons having only one carbon-to-carbon double bond; Compositions of derivatives of such polymers not modified by chemical after-treatment
    • C08L23/18—Homopolymers or copolymers of hydrocarbons having four or more carbon atoms
    • C08L23/20—Homopolymers or copolymers of hydrocarbons having four or more carbon atoms having four to nine carbon atoms
    • C08L23/22—Copolymers of isobutene; Butyl rubber; Homopolymers or copolymers of other iso-olefins
    • C—CHEMISTRY; METALLURGY
    • C08—ORGANIC MACROMOLECULAR COMPOUNDS; THEIR PREPARATION OR CHEMICAL WORKING-UP; COMPOSITIONS BASED THEREON
    • C08L—COMPOSITIONS OF MACROMOLECULAR COMPOUNDS
    • C08L23/00—Compositions of homopolymers or copolymers of unsaturated aliphatic hydrocarbons having only one carbon-to-carbon double bond; Compositions of derivatives of such polymers
    • C08L23/26—Compositions of homopolymers or copolymers of unsaturated aliphatic hydrocarbons having only one carbon-to-carbon double bond; Compositions of derivatives of such polymers modified by chemical after-treatment
    • C—CHEMISTRY; METALLURGY
    • C08—ORGANIC MACROMOLECULAR COMPOUNDS; THEIR PREPARATION OR CHEMICAL WORKING-UP; COMPOSITIONS BASED THEREON
    • C08L—COMPOSITIONS OF MACROMOLECULAR COMPOUNDS
    • C08L23/00—Compositions of homopolymers or copolymers of unsaturated aliphatic hydrocarbons having only one carbon-to-carbon double bond; Compositions of derivatives of such polymers
    • C08L23/26—Compositions of homopolymers or copolymers of unsaturated aliphatic hydrocarbons having only one carbon-to-carbon double bond; Compositions of derivatives of such polymers modified by chemical after-treatment
    • C08L23/28—Compositions of homopolymers or copolymers of unsaturated aliphatic hydrocarbons having only one carbon-to-carbon double bond; Compositions of derivatives of such polymers modified by chemical after-treatment by reaction with halogens or halogen-containing compounds
    • C08L23/283—Iso-olefin halogenated homopolymers or copolymers
    • C—CHEMISTRY; METALLURGY
    • C08—ORGANIC MACROMOLECULAR COMPOUNDS; THEIR PREPARATION OR CHEMICAL WORKING-UP; COMPOSITIONS BASED THEREON
    • C08L—COMPOSITIONS OF MACROMOLECULAR COMPOUNDS
    • C08L25/00—Compositions of, homopolymers or copolymers of compounds having one or more unsaturated aliphatic radicals, each having only one carbon-to-carbon double bond, and at least one being terminated by an aromatic carbocyclic ring; Compositions of derivatives of such polymers
    • C08L25/02—Homopolymers or copolymers of hydrocarbons
    • C08L25/16—Homopolymers or copolymers of alkyl-substituted styrenes
    • C—CHEMISTRY; METALLURGY
    • C08—ORGANIC MACROMOLECULAR COMPOUNDS; THEIR PREPARATION OR CHEMICAL WORKING-UP; COMPOSITIONS BASED THEREON
    • C08L—COMPOSITIONS OF MACROMOLECULAR COMPOUNDS
    • C08L7/00—Compositions of natural rubber
    • C—CHEMISTRY; METALLURGY
    • C08—ORGANIC MACROMOLECULAR COMPOUNDS; THEIR PREPARATION OR CHEMICAL WORKING-UP; COMPOSITIONS BASED THEREON
    • C08L—COMPOSITIONS OF MACROMOLECULAR COMPOUNDS
    • C08L9/00—Compositions of homopolymers or copolymers of conjugated diene hydrocarbons
    • C08L9/02—Copolymers with acrylonitrile
    • C—CHEMISTRY; METALLURGY
    • C08—ORGANIC MACROMOLECULAR COMPOUNDS; THEIR PREPARATION OR CHEMICAL WORKING-UP; COMPOSITIONS BASED THEREON
    • C08L—COMPOSITIONS OF MACROMOLECULAR COMPOUNDS
    • C08L9/00—Compositions of homopolymers or copolymers of conjugated diene hydrocarbons
    • C08L9/06—Copolymers with styrene
    • C—CHEMISTRY; METALLURGY
    • C08—ORGANIC MACROMOLECULAR COMPOUNDS; THEIR PREPARATION OR CHEMICAL WORKING-UP; COMPOSITIONS BASED THEREON
    • C08K—Use of inorganic or non-macromolecular organic substances as compounding ingredients
    • C08K3/00—Use of inorganic substances as compounding ingredients
    • C08K3/18—Oxygen-containing compounds, e.g. metal carbonyls
    • C08K3/20—Oxides; Hydroxides
    • C08K3/22—Oxides; Hydroxides of metals
    • C08K2003/2296—Oxides; Hydroxides of metals of zinc
    • Y—GENERAL TAGGING OF NEW TECHNOLOGICAL DEVELOPMENTS; GENERAL TAGGING OF CROSS-SECTIONAL TECHNOLOGIES SPANNING OVER SEVERAL SECTIONS OF THE IPC; TECHNICAL SUBJECTS COVERED BY FORMER USPC CROSS-REFERENCE ART COLLECTIONS [XRACs] AND DIGESTS
    • Y10—TECHNICAL SUBJECTS COVERED BY FORMER USPC
    • Y10S—TECHNICAL SUBJECTS COVERED BY FORMER USPC CROSS-REFERENCE ART COLLECTIONS [XRACs] AND DIGESTS
    • Y10S525/00—Synthetic resins or natural rubbers -- part of the class 520 series
    • Y10S525/912—Polymer from nonethylenic monomers only, having pendant unsaturated group
    • Y—GENERAL TAGGING OF NEW TECHNOLOGICAL DEVELOPMENTS; GENERAL TAGGING OF CROSS-SECTIONAL TECHNOLOGIES SPANNING OVER SEVERAL SECTIONS OF THE IPC; TECHNICAL SUBJECTS COVERED BY FORMER USPC CROSS-REFERENCE ART COLLECTIONS [XRACs] AND DIGESTS
    • Y10—TECHNICAL SUBJECTS COVERED BY FORMER USPC
    • Y10T—TECHNICAL SUBJECTS COVERED BY FORMER US CLASSIFICATION
    • Y10T152/00—Resilient tires and wheels
    • Y10T152/10—Tires, resilient
    • Y10T152/10495—Pneumatic tire or inner tube

Landscapes

  • Chemical & Material Sciences (AREA)
  • Health & Medical Sciences (AREA)
  • Chemical Kinetics & Catalysis (AREA)
  • Medicinal Chemistry (AREA)
  • Polymers & Plastics (AREA)
  • Organic Chemistry (AREA)
  • General Chemical & Material Sciences (AREA)
  • Engineering & Computer Science (AREA)
  • Mechanical Engineering (AREA)
  • Compositions Of Macromolecular Compounds (AREA)
  • Tires In General (AREA)
  • Processes Of Treating Macromolecular Substances (AREA)
  • Moulds For Moulding Plastics Or The Like (AREA)
  • Heating, Cooling, Or Curing Plastics Or The Like In General (AREA)
  • Paints Or Removers (AREA)

Abstract

SE DESCRIBEN COMPOSICIONES VULCANIZABLES PARA EL REVESTIMIENTO INTERIOR DE NEUMATICOS QUE ESTAN ESENCIALMENTE LIBRES DE ATOMOS DE HALOGENOS O PRESENTAN UN CONTENIDO EN HALOGENOS REDUCIDO. LOS REVESTIMIENTOS CONTIENEN UN INTERPOLIMERO ELASTOMERICO SATURADO DE UNA ISOMONOOLEFINA C4 -C7, P.EJ: ISOBUTILENO Y UN PARA NO, QUE CONTIENE FUNCIONALIDAD ESTER BENCILICA DE ESTRUCTURA (I), DONDE R2 Y R3 SON SELECCIONADOS INDEPENDIENTEMENTE DE ENTRE HIDROGENO O ALQUILOS C1 A C6, Y R4 ES SELECCIONADO DE ENTRE HIDROGENO, ALQUILOS C1 A C28, ARILOS O ALQUENILOS C2 A C28. LOS REVESTIMIENTOS DE LA INVENCION PROPORCIONAN EXCELENTE IMPERMEABILIDAD AL AIRE, PROPIEDADES DE DEGRADACION TERMICA Y BUENA ADHESION AL MATERIAL DE LA CARCASA DEL NEUMATICO COMO SE REQUIRE DE LOS REVESTIMIENTOS INTERIORES PARA NEUMATICOS, Y ESTAN TAMBIEN ESENCIALMENTE LIBRES DE HALOGENOS O PRESENTAN BAJO CONTENIDO EN HALOGENOS REDUCIENDO DE ESE MODO EL POTENCIAL IMPACTO AMBIENTAL DE LA INCINERACION DE NEUMATICOS USADOS.
ES96916853T 1995-06-07 1996-05-31 Interpolimeros elastomericos de isomonoolefinas c{sub,4} c{sub,7} y para - alquilestireno con funcionalidad ester Expired - Lifetime ES2129969T3 (es)

Applications Claiming Priority (1)

Application Number Priority Date Filing Date Title
US08/472,373 US5631316A (en) 1993-09-30 1995-06-07 Tire innerliner comprising ester-functionalized elastomeric interpolymers of C4-C7 isomonoolefin and para-alkylstyrene

Publications (1)

Publication Number Publication Date
ES2129969T3 true ES2129969T3 (es) 1999-06-16

Family

ID=23875262

Family Applications (1)

Application Number Title Priority Date Filing Date
ES96916853T Expired - Lifetime ES2129969T3 (es) 1995-06-07 1996-05-31 Interpolimeros elastomericos de isomonoolefinas c{sub,4} c{sub,7} y para - alquilestireno con funcionalidad ester

Country Status (16)

Country Link
US (1) US5631316A (es)
EP (1) EP0830387B1 (es)
JP (1) JP3278680B2 (es)
KR (1) KR19990022616A (es)
CN (1) CN1190975A (es)
BR (1) BR9608727A (es)
CA (1) CA2221650A1 (es)
CZ (1) CZ385197A3 (es)
DE (1) DE69601936T2 (es)
EA (1) EA000430B1 (es)
ES (1) ES2129969T3 (es)
HU (1) HUP9900875A3 (es)
MX (1) MX9709601A (es)
PL (1) PL323739A1 (es)
TW (1) TW368511B (es)
WO (1) WO1996040801A1 (es)

Families Citing this family (30)

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US6060549A (en) * 1997-05-20 2000-05-09 Exxon Chemical Patents, Inc. Rubber toughened thermoplastic resin nano composites
US6203855B1 (en) 1999-08-13 2001-03-20 Xerox Corporation Process for preparing nonbleeding fluorinated carbon and zinc oxide filler layer for bias charging member
US6620476B2 (en) 1999-08-13 2003-09-16 Xerox Corporation Nonbleeding fluorinated carbon and zinc oxide filled layer for bias charging member
US6710116B1 (en) 2000-10-18 2004-03-23 Exxonmobil Chemical Patents Inc. Abrasion resistant transparent and colorable elastomeric compositions
MXPA03003383A (es) * 2000-10-18 2004-05-21 Exxonmobil Chem Patents Inc Composicion elastomerica.
US7425591B2 (en) * 2001-10-16 2008-09-16 Exxonmobil Chemical Patents Inc Elastomeric composition
DE60231306D1 (de) * 2001-06-08 2009-04-09 Exxonmobil Chem Patents Inc Nanoverbundwerkstoffe mit geringer permeabilität
US6939921B2 (en) * 2001-10-16 2005-09-06 Exxonmobil Chemical Patents Inc. Colorable elastomeric composition
US20040030036A1 (en) * 2001-10-16 2004-02-12 Waddell Walter H. Elastomeric composition
KR20030094907A (ko) * 2002-06-10 2003-12-18 한국타이어 주식회사 튜브리스형 트럭,버스용 래디얼 공기입 타이어의인너라이너 고무 조성물
US7294664B2 (en) * 2002-11-07 2007-11-13 Exxonmobil Chemical Patents Inc. Elastomeric blend for air barriers comprising grafted resin components
WO2004044051A1 (en) * 2002-11-07 2004-05-27 Exxonmobil Chemical Patents Inc. Elastomeric blend for air barriers comprising low glass transition temperature petroleum hydrocarbon resins
US20050027062A1 (en) * 2003-08-01 2005-02-03 Waddell Walter Harvey Elastomeric composition
RU2369620C2 (ru) * 2004-10-22 2009-10-10 Сосьете Де Текноложи Мишлен Барьерный слой для эластомерных изделий
FR2877348B1 (fr) 2004-10-28 2007-01-12 Michelin Soc Tech Systeme plastifiant pour composition de caoutchouc
US8247496B2 (en) * 2005-12-05 2012-08-21 Exxonmobil Chemical Patents Inc. Processing aids for elastomeric compositions
CA2632734C (en) * 2005-12-16 2011-07-05 Exxonmobil Chemical Patents Inc. Processing aids for elastomeric compositions
ATE463516T1 (de) * 2005-12-16 2010-04-15 Exxonmobil Chem Patents Inc Verfahrenshilfsmittel für elastomerzusammensetzungen
EP2102018B1 (en) * 2006-12-29 2010-11-03 Bridgestone Americas Tire Operations, LLC Tire innerliner
US7923491B2 (en) * 2008-08-08 2011-04-12 Exxonmobil Chemical Patents Inc. Graphite nanocomposites
EP2323856A4 (en) * 2008-08-31 2011-12-21 Michelin Soc Tech GAS BARRIER WITH AN ALIPHATIC RESIN
FR2954336B1 (fr) * 2009-12-23 2013-01-04 Michelin Soc Tech Objet pneumatique pourvu d'une couche etanche aux gaz a base d'un elastomere thermoplastique styrenique et d'un polyphenylene ether
WO2012044317A1 (en) * 2010-09-30 2012-04-05 Michelin Recherche Et Technique S.A. Barrier layer for inflatable articles
JP2016128553A (ja) * 2015-01-09 2016-07-14 株式会社ブリヂストン ゴム組成物の製造方法、その製造方法で得られたゴム組成物及びそれを用いたタイヤ
CN107614555B (zh) 2015-05-26 2020-03-20 株式会社钟化 热塑性弹性体的制造方法及热塑性弹性体
CA2997048C (en) * 2015-09-02 2023-05-23 Threebond Co., Ltd. Photocurable resin composition, fuel cell, and sealing method
ITUB20160382A1 (it) * 2016-01-28 2017-07-28 Bridgestone Corp Mescola in gomma per la preparazione di uno strato di innerliner
CN107778565A (zh) * 2016-08-24 2018-03-09 中国石油天然气股份有限公司 一种溴化异丁烯/烷基苯乙烯聚合物与溶聚丁苯橡胶的复合材料及其制备方法
CN107778566A (zh) * 2016-08-24 2018-03-09 中国石油天然气股份有限公司 一种异丁烯/烷基苯乙烯聚合物与乳聚丁苯橡胶的复合材料及其制备方法
CN113736148B (zh) * 2020-05-29 2024-08-13 中国石油化工股份有限公司 一种全钢载重轮胎子午线轮胎胎面胶料及其制备方法

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US2943664A (en) * 1956-07-09 1960-07-05 Exxon Research Engineering Co Pneumatic tire
US5162445A (en) * 1988-05-27 1992-11-10 Exxon Chemical Patents Inc. Para-alkylstyrene/isoolefin copolymers and functionalized copolymers thereof
NL8902414A (nl) * 1989-09-28 1991-04-16 Stichting Centr Diergeneeskund Oligopeptiden/expressieprodukten van het aujeszky's disease virus en daarvoor coderende recombinante polynucleotiden.
BR9106657A (pt) * 1990-07-18 1993-06-08 Exxon Chemical Patents Inc Composicao de revestimento interno de pneu,e,pneu vulcanizado compreendendo um revestimento interno
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Also Published As

Publication number Publication date
CZ385197A3 (cs) 1998-04-15
EP0830387B1 (en) 1999-03-31
KR19990022616A (ko) 1999-03-25
TW368511B (en) 1999-09-01
BR9608727A (pt) 1999-05-04
JP3278680B2 (ja) 2002-04-30
DE69601936D1 (de) 1999-05-06
MX9709601A (es) 1998-04-30
DE69601936T2 (de) 1999-10-14
WO1996040801A1 (en) 1996-12-19
JP2000504358A (ja) 2000-04-11
CN1190975A (zh) 1998-08-19
CA2221650A1 (en) 1996-12-19
EA199800021A1 (ru) 1998-08-27
EP0830387A1 (en) 1998-03-25
PL323739A1 (en) 1998-04-14
EA000430B1 (ru) 1999-08-26
US5631316A (en) 1997-05-20
HUP9900875A3 (en) 1999-11-29
HUP9900875A2 (hu) 1999-07-28

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