CH215291A - Process for the production of a urea derivative. - Google Patents

Process for the production of a urea derivative.

Info

Publication number
CH215291A
CH215291A CH215291DA CH215291A CH 215291 A CH215291 A CH 215291A CH 215291D A CH215291D A CH 215291DA CH 215291 A CH215291 A CH 215291A
Authority
CH
Switzerland
Prior art keywords
urea derivative
production
derivative
acid
phosgene
Prior art date
Application number
Other languages
German (de)
Inventor
A-G J R Geigy
Original Assignee
Geigy Ag J R
Priority date (The priority date is an assumption and is not a legal conclusion. Google has not performed a legal analysis and makes no representation as to the accuracy of the date listed.)
Filing date
Publication date
Application filed by Geigy Ag J R filed Critical Geigy Ag J R
Publication of CH215291A publication Critical patent/CH215291A/en

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Classifications

    • CCHEMISTRY; METALLURGY
    • C07ORGANIC CHEMISTRY
    • C07CACYCLIC OR CARBOCYCLIC COMPOUNDS
    • C07C309/00Sulfonic acids; Halides, esters, or anhydrides thereof
    • C07C309/01Sulfonic acids
    • C07C309/28Sulfonic acids having sulfo groups bound to carbon atoms of six-membered aromatic rings of a carbon skeleton
    • C07C309/41Sulfonic acids having sulfo groups bound to carbon atoms of six-membered aromatic rings of a carbon skeleton containing singly-bound oxygen atoms bound to the carbon skeleton
    • C07C309/42Sulfonic acids having sulfo groups bound to carbon atoms of six-membered aromatic rings of a carbon skeleton containing singly-bound oxygen atoms bound to the carbon skeleton having the sulfo groups bound to carbon atoms of non-condensed six-membered aromatic rings

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  • Chemical & Material Sciences (AREA)
  • Organic Chemistry (AREA)
  • Organic Low-Molecular-Weight Compounds And Preparation Thereof (AREA)

Description

  

      Verfahren    zur Herstellung eines     Harnstoffderivates.            Gegenstand    des vorliegenden     Patentes    ist ein Verfahren zur     Herstellung    eines Harn  stoffderivates der Formel  
EMI0001.0006     
    dadurch gekennzeichnet,     dass    man     3,4,5-          Trichloranilin    mit     Phosgen    zu einem Derivat  der     3,4,5-Trichlorphenylearbaminsäure    und  dieses mit     2-Amino-4,4'-dichlor-1,1'-diphenyl-          äther-2'-sulfonsäure    umsetzt.

   Das neue Harn  stoffdemivat bildet als     Natriumsalz    ein     helles,     in heissem Wasser lösliches Pulver und eignet  sich als     Mattenschutzmittel.            Beispiel:            a:

  )    In 500 Teile Essigester, welche 135  Teile     Phosgen    enthalten, wird eine Lösung  von<B>196</B> Teilen     3,4,5-Trichloranilin    in 1000  Teilen Essigester langsam eingetropft, unter         gleichzeitigem    Durchleiten eines     Phosgen.          stromes.    Nach Beendigung der Reaktion wird  das     Lösungsmittel    in der Wärme     abdestil-          liert,    wobei das, gebildete     3,4,5-Trichlor-          phenylcarbaminsäurechlorid    unter Salzsäure  abspadtung in das.

       3,4,5-Trichlorphenyliso-          cyanat    übergeht.    b)     '/_o        Mol.    der     2-Amino-4;4'-dichlor-1,1'-          diphenyl@äth-er-2'-sulfonsiäure    wird in trocke  nem     Pyridin    gelöst und unter Rühren bei 10  bis<B>15'</B> C     portionenweise    mit     '/zu        Mol.        3,4,5-          Trichlorphenylisocyanat    versetzt. Dann wird  bei Raumtemperatur     weitergerührt,    bis keine  freie     Aminogruppe    mehr nachweisbar ist.

        Hierauf versetzt man mit     Sodalösung    bis zur  alkalischen Reaktion und bläst das     Pyridin     mit Wasserdampf ab. Den Rückstand löst  man in heissem Wasser, filtriert die Lösung,  fällt das     Reaktionsprodukt    durch Zugabe von  Kochsalz als graues Harz aus und erhält es    nach dem Abtrennen, Trocknen und Mahlen  als helles, in heissem Wasser ziemlich schwer  lösliches Pulver.



      Process for the production of a urea derivative. The subject of the present patent is a process for the preparation of a urea derivative of the formula
EMI0001.0006
    characterized in that 3,4,5-trichloroaniline with phosgene to a derivative of 3,4,5-trichlorophenylearbamic acid and this with 2-amino-4,4'-dichloro-1,1'-diphenyl ether-2 ' -sulfonic acid converts.

   As a sodium salt, the new urea derivative forms a light-colored powder that is soluble in hot water and is suitable as a mat protection agent. Example: a:

  A solution of 196 parts of 3,4,5-trichloroaniline in 1000 parts of ethyl acetate is slowly added dropwise to 500 parts of ethyl acetate, which contain 135 parts of phosgene, while phosgene is passed through at the same time. Stromes. After the reaction has ended, the solvent is distilled off in the heat, with the 3,4,5-trichlorophenylcarbamic acid chloride formed being sparged off under hydrochloric acid.

       3,4,5-trichlorophenyl isocyanate passes over. b) '/ _o mol. of the 2-amino-4; 4'-dichloro-1,1'-diphenyl @ ether-2'-sulfonic acid is dissolved in dry pyridine and stirred at 10 to 15 '</B> C added in portions with' / to mol. 3,4,5-trichlorophenyl isocyanate. Stirring is then continued at room temperature until free amino groups can no longer be detected.

        Soda solution is then added until an alkaline reaction occurs and the pyridine is blown off with steam. The residue is dissolved in hot water, the solution is filtered, the reaction product is precipitated as a gray resin by the addition of sodium chloride and obtained after separation, drying and grinding as a pale powder that is rather poorly soluble in hot water.

 

Claims (1)

PATENTANSPRUCH: Verfahren zur Herstellung eines Harn stoffderivates der Formel EMI0002.0004 dadurch gekennzeichnet, dass man 3,4,5-Tri- chloranilin mit Phosgen zu einem Derivat der 3,4,5-Trichlorphenylcarba-minsäure und die ses mit 2-Amino-4,4'-dichlor-1,1'-diphenyl- äther-2'-s@ulfonsäure umsetzt. Das neue Harn- stoffderivat bildet als Natriumsalz ein helles, in heissem Wasser lösliches Pulver und eignet sich als Mottenschutzmittel. PATENT CLAIM: Process for the production of a urea derivative of the formula EMI0002.0004 characterized in that 3,4,5-trichloroaniline with phosgene to a derivative of 3,4,5-trichlorophenylcarba-minic acid and this ses with 2-amino-4,4'-dichloro-1,1'-diphenyl - converts ether-2'-s @ ulfonic acid. As a sodium salt, the new urea derivative forms a light-colored powder that is soluble in hot water and is suitable as a moth repellent.
CH215291D 1938-06-16 1938-06-16 Process for the production of a urea derivative. CH215291A (en)

Applications Claiming Priority (2)

Application Number Priority Date Filing Date Title
CH212408T 1938-06-16
CH215291T 1938-06-16

Publications (1)

Publication Number Publication Date
CH215291A true CH215291A (en) 1941-06-15

Family

ID=25725171

Family Applications (1)

Application Number Title Priority Date Filing Date
CH215291D CH215291A (en) 1938-06-16 1938-06-16 Process for the production of a urea derivative.

Country Status (1)

Country Link
CH (1) CH215291A (en)

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