CH215327A - Process for the production of a urea derivative. - Google Patents

Process for the production of a urea derivative.

Info

Publication number
CH215327A
CH215327A CH215327DA CH215327A CH 215327 A CH215327 A CH 215327A CH 215327D A CH215327D A CH 215327DA CH 215327 A CH215327 A CH 215327A
Authority
CH
Switzerland
Prior art keywords
dichloro
urea derivative
production
derivative
phosgene
Prior art date
Application number
Other languages
German (de)
Inventor
A-G J R Geigy
Original Assignee
Geigy Ag J R
Priority date (The priority date is an assumption and is not a legal conclusion. Google has not performed a legal analysis and makes no representation as to the accuracy of the date listed.)
Filing date
Publication date
Application filed by Geigy Ag J R filed Critical Geigy Ag J R
Publication of CH215327A publication Critical patent/CH215327A/en

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Classifications

    • CCHEMISTRY; METALLURGY
    • C07ORGANIC CHEMISTRY
    • C07CACYCLIC OR CARBOCYCLIC COMPOUNDS
    • C07C309/00Sulfonic acids; Halides, esters, or anhydrides thereof
    • C07C309/01Sulfonic acids
    • C07C309/28Sulfonic acids having sulfo groups bound to carbon atoms of six-membered aromatic rings of a carbon skeleton
    • C07C309/41Sulfonic acids having sulfo groups bound to carbon atoms of six-membered aromatic rings of a carbon skeleton containing singly-bound oxygen atoms bound to the carbon skeleton
    • C07C309/42Sulfonic acids having sulfo groups bound to carbon atoms of six-membered aromatic rings of a carbon skeleton containing singly-bound oxygen atoms bound to the carbon skeleton having the sulfo groups bound to carbon atoms of non-condensed six-membered aromatic rings

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  • Chemical & Material Sciences (AREA)
  • Organic Chemistry (AREA)
  • Organic Low-Molecular-Weight Compounds And Preparation Thereof (AREA)

Description

  

  Verfahren zur Herstellung eines     Harnstoüderivates.       Gegenstand des vorliegenden     Patentes    ist ein Verfahren zur Herstellung eines Harn  stoffderivates der Formel  
EMI0001.0003     
    dadurch gekennzeichnet, dass man     3,5-Di-          chlor-2-phenetidin    mit     Phosgen    zu einem  Derivat der     3,5-Dichlor-2-äthogyphenylcarb-          aminsäure    und dieses mit     2-Amin.o-4,4'-di-!          chlor-1,1'-diphenyläther-2'-sulfonsäure    um  setzt.

       Das    neue     Harnstoffderivat    bildet als       Natriumsalz    ein helles, in Wasser lösliches  Pulver und eignet sich als Mottenschutz  mittel.  



       Beispiel:     a) In 500 Teile Essigester, welche 135  Teile     Phosgen    enthalten,     wirdeineLösung    von  207 Teilen     3,5-Dichlor-2-phenetidin    in<B>1000</B>  Teilen Essigester langsam     eingetropft        unter     gleichzeitigem Durchleiten eines Phosgen-         strames.    Nach Beendigung der     Reaktion     wird das     Lösungsmittel    in der     Wärme    ab  destilliert, wobei das gebildete     3,

  5-Dichlor-          2-äthogy-phenylcarbaminsäurechlflrid    unter       Salzsäureabspaltung    in das     3,5-Dichlor-2-          äthogyphenylisocyanat    vom     $p."    145   über  geht.  



  b)     'J")        Mol.    der     2-Amino-4,4'-dichlor-1,1'-          diphenyläther-2'-@sulfonsäure    wird in trocke  nem     Pyridin    gelöst und unter Rühren bei  10-15   C     portionenweise    mit     '/2o        Mol.        3,5-          Dichlor-    2 -     äthogyphenylisocyanat    versetzt.  Dann wird bei Raumtemperatur weiterge  rührt, bis keine freie     Aminogruppe    mehr  nachweisbar ist.

   Hierauf     versetzt    man mit           Sololösung    bis zur alkalischen Reaktion und  bläst das     Pyridin    mit Wasserdampf ab. Den  Rückstand löst man in heissem Wasser,  filtriert die Lösung, fällt das     Reaktions-          produkt    durch Zugabe von Kochsalz als  graues Harz aus und erhält es nach dem Ah-    trennen, Trocknen und Mahlen als helles, in  Wasser lösliches Pulver.



  Process for the production of a urinary derivative. The subject of the present patent is a process for the preparation of a urea derivative of the formula
EMI0001.0003
    characterized in that 3,5-dichloro-2-phenetidine with phosgene to a derivative of 3,5-dichloro-2-äthogyphenylcarb- aminsäure and this with 2-Amin.o-4,4'-di-! chlorine-1,1'-diphenylether-2'-sulfonic acid sets.

       The new urea derivative forms a pale, water-soluble powder as a sodium salt and is suitable as a moth repellent.



       Example: a) A solution of 207 parts of 3,5-dichloro-2-phenetidine in 1000 parts of ethyl acetate is slowly added dropwise to 500 parts of ethyl acetate containing 135 parts of phosgene while a phosgene stream is passed through at the same time. After the reaction has ended, the solvent is distilled off in the heat, whereby the 3 formed

  5-dichloro-2-ethogyphenylcarbamic acid chloride is converted into 3,5-dichloro-2-ethogyphenyl isocyanate from $ 145 with elimination of hydrochloric acid.



  b) 'J ") Mol. The 2-amino-4,4'-dichloro-1,1'-diphenylether-2' - @ sulfonic acid is dissolved in dry pyridine and stirred in portions at 10-15 C with '/ 20 moles of 3,5-dichloro-2-ethogyphenyl isocyanate are added, and stirring is continued at room temperature until free amino groups can no longer be detected.

   Solo solution is then added until an alkaline reaction is achieved and the pyridine is blown off with steam. The residue is dissolved in hot water, the solution is filtered, the reaction product precipitates as a gray resin by adding sodium chloride and, after separating, drying and grinding, it is obtained as a pale, water-soluble powder.

 

Claims (1)

PATENTANSPRUCH: Verfahren zur Herstellung eines Harn stoffderivates der Formel EMI0002.0007 dadurch gekennzeichnet, da.ss man 3,5-Di- chlor-?-phenetidin mit Phosgen zu einem Derivat der 3,5-Dichlor-2-äthoxyphenylcar-h- aminsäure und dieses mit 2-3mino-4,4'-di- chlor-1,1'-diphenyläther-\?'-sulfonsättre uni- setzt. PATENT CLAIM: Process for the production of a urea derivative of the formula EMI0002.0007 characterized in that 3,5-dichloro -? - phenetidine with phosgene to a derivative of 3,5-dichloro-2-ethoxyphenylcar-h-amic acid and this with 2-3mino-4,4'-di - chlorine-1,1'-diphenyl ether - \? '- sulfonic saturation uni- sets. Das neue Harnstoffderivat bildet als Natriumsalz ein helles, in Wasser lösliches Pulver und eignet sich als Mottenschutz mittel. The new urea derivative forms a pale, water-soluble powder as a sodium salt and is suitable as a moth repellent.
CH215327D 1938-06-16 1938-06-16 Process for the production of a urea derivative. CH215327A (en)

Applications Claiming Priority (2)

Application Number Priority Date Filing Date Title
CH215327T 1938-06-16
CH212408T 1938-06-16

Publications (1)

Publication Number Publication Date
CH215327A true CH215327A (en) 1941-06-15

Family

ID=25725207

Family Applications (1)

Application Number Title Priority Date Filing Date
CH215327D CH215327A (en) 1938-06-16 1938-06-16 Process for the production of a urea derivative.

Country Status (1)

Country Link
CH (1) CH215327A (en)

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