CH215329A - Process for the production of a urea derivative. - Google Patents

Process for the production of a urea derivative.

Info

Publication number
CH215329A
CH215329A CH215329DA CH215329A CH 215329 A CH215329 A CH 215329A CH 215329D A CH215329D A CH 215329DA CH 215329 A CH215329 A CH 215329A
Authority
CH
Switzerland
Prior art keywords
urea derivative
production
derivative
acid
trichlorophenylcarbamic
Prior art date
Application number
Other languages
German (de)
Inventor
A-G J R Geigy
Original Assignee
Geigy Ag J R
Priority date (The priority date is an assumption and is not a legal conclusion. Google has not performed a legal analysis and makes no representation as to the accuracy of the date listed.)
Filing date
Publication date
Application filed by Geigy Ag J R filed Critical Geigy Ag J R
Publication of CH215329A publication Critical patent/CH215329A/en

Links

Classifications

    • CCHEMISTRY; METALLURGY
    • C07ORGANIC CHEMISTRY
    • C07CACYCLIC OR CARBOCYCLIC COMPOUNDS
    • C07C309/00Sulfonic acids; Halides, esters, or anhydrides thereof
    • C07C309/01Sulfonic acids
    • C07C309/28Sulfonic acids having sulfo groups bound to carbon atoms of six-membered aromatic rings of a carbon skeleton
    • C07C309/41Sulfonic acids having sulfo groups bound to carbon atoms of six-membered aromatic rings of a carbon skeleton containing singly-bound oxygen atoms bound to the carbon skeleton
    • C07C309/42Sulfonic acids having sulfo groups bound to carbon atoms of six-membered aromatic rings of a carbon skeleton containing singly-bound oxygen atoms bound to the carbon skeleton having the sulfo groups bound to carbon atoms of non-condensed six-membered aromatic rings

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  • Chemical & Material Sciences (AREA)
  • Organic Chemistry (AREA)
  • Organic Low-Molecular-Weight Compounds And Preparation Thereof (AREA)

Description

  

  Verfahren zur Herstellung eines     Harnstoffderivates.       Gegenstand des vorliegenden     Patentes        ist    ein Verfahren zur Herstellung     eines        Harn-          stoffderivates    der Formel  
EMI0001.0007     
    dadurch gekennzeichnet, dass man     2,4,5-Tri-          chloranilin    mit     Phosgen    zu einem Derivat der       2,4,5-Trichlorphenylcarbaminsäure    und dieses  mit     2-Amino-4,4'-dichlor-1,1'-diphenyläther-          2'-sulfonsäure    umsetzt.

   Das neue Harnstoff  derivat bildet als     Natriumsalz    ein helles, in  heissem Wasser lösliches Pulver und eignet  sich als Mottenschutzmittel.  



  <I>Beispiel:</I>  a) In 500 Teile Essigester, welche 135  Teile     Phosgen    enthalten, wird     eine    Lösung  von 196 Teilen     2,4,5-Trichloranilin    in 1000  Teilen Essigester langsam eingetropft unter    gleichzeitigem Durchleiten     eines.        Phosgen-          stromes..    Nach Beendigung der Reaktion wird  das Lösungsmittel in der Wärme     abd@estil-          liert,    wobei das gebildete     2,4,5-Trichlor-          phenylcarbaminsäurechlorid    unter Salzsäure  abspaltung in das     2,4,

  5-Trichlorphenyliso-          cyanat    übergeht.  



  b)     '/2o        Mol.    der     2-Amino-4,4'-dichlor-1,1'-          diphenyläth-er-2'-.sulfonsäure    wird in trocke  nem     Pyridin    gelöst und     unter    Rühren bei  l0-15   C     portionenweise        mit1/zo        Mol.        2,4,5-          Trichlorphenylisocyanat    versetzt. Dann wird  bei Raumtemperatur weitergerührt, bis keine  freie     Aminogruppe    mehr nachweisbar ist.

        hierauf versetzt man mit     Soda-lösung    bis zur  alkalischen Reaktion und bläst das     Pyridin     mit Wasserdampf ab. Den     Rückstand    löst  man in heissem Wasser, filtriert die Lösung,  fällt das Reaktionsprodukt durch Zugabe  von Kochsalz als graues Harz aus und er-    hält es nach dem Abtrennen, Trocknen und  Mahlen als helles, in heissem Wasser lösliches  Pulver.



  Process for the production of a urea derivative. The present patent relates to a process for the preparation of a urea derivative of the formula
EMI0001.0007
    characterized in that 2,4,5-trichloroaniline with phosgene to a derivative of 2,4,5-trichlorophenylcarbamic acid and this with 2-amino-4,4'-dichloro-1,1'-diphenyl ether- 2 ' -sulfonic acid converts.

   As a sodium salt, the new urea derivative forms a light-colored powder that is soluble in hot water and is suitable as a moth repellent.



  <I> Example: </I> a) A solution of 196 parts of 2,4,5-trichloroaniline in 1000 parts of ethyl acetate is slowly added dropwise to 500 parts of ethyl acetate which contain 135 parts of phosgene, while a solution is simultaneously passed through. Phosgene stream .. After the reaction has ended, the solvent is removed in the heat, the 2,4,5-trichlorophenylcarbamic acid chloride formed being split off into the 2,4,5-trichlorophenylcarbamic acid chloride with hydrochloric acid

  5-trichlorophenyl isocyanate passes over.



  b) '/ 2o mol. of the 2-amino-4,4'-dichloro-1,1'-diphenylether-2' -. sulfonic acid is dissolved in dry pyridine and stirred in portions at 10-15 ° C with 1 / zo mol. 2,4,5-trichlorophenyl isocyanate added. Stirring is then continued at room temperature until free amino groups can no longer be detected.

        Soda solution is then added to an alkaline reaction and the pyridine is blown off with steam. The residue is dissolved in hot water, the solution is filtered, the reaction product is precipitated as a gray resin by the addition of sodium chloride and obtained after separation, drying and grinding as a pale powder which is soluble in hot water.

 

Claims (1)

PATENTANSPRUCH: Verfahren zur Herstellung eines Harn stoffderivates der Formel EMI0002.0006 dadurch gekennzeichnet, dass man 2,4,5-Tri- chloranilin mit. Phosgen zu einem Derivat der ?,4,5-Trichlorphenylcarbaminsäure und dieses mit. 2-Amino-4,4'-dichlor-1,1'-diphenyläther- 2'-sulfonsäure umsetzt. Das neue Ha.rnstoff- derivat bildet als Natriumsalz ein helles, in heissem Wasser lösliches Pulver und eignet sich als Mottensehutzmittel. PATENT CLAIM: Process for the production of a urea derivative of the formula EMI0002.0006 characterized in that 2,4,5-trichloroaniline with. Phosgene to a derivative of?, 4,5-trichlorophenylcarbamic acid and this with. 2-Amino-4,4'-dichloro-1,1'-diphenylether-2'-sulfonic acid is converted. As a sodium salt, the new urea derivative forms a light-colored powder that is soluble in hot water and is suitable as a moth repellent.
CH215329D 1938-06-16 1938-06-16 Process for the production of a urea derivative. CH215329A (en)

Applications Claiming Priority (2)

Application Number Priority Date Filing Date Title
CH215329T 1938-06-16
CH212408T 1938-06-16

Publications (1)

Publication Number Publication Date
CH215329A true CH215329A (en) 1941-06-15

Family

ID=25725209

Family Applications (1)

Application Number Title Priority Date Filing Date
CH215329D CH215329A (en) 1938-06-16 1938-06-16 Process for the production of a urea derivative.

Country Status (1)

Country Link
CH (1) CH215329A (en)

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