CH215319A - Process for the production of a urea derivative. - Google Patents

Process for the production of a urea derivative.

Info

Publication number
CH215319A
CH215319A CH215319DA CH215319A CH 215319 A CH215319 A CH 215319A CH 215319D A CH215319D A CH 215319DA CH 215319 A CH215319 A CH 215319A
Authority
CH
Switzerland
Prior art keywords
production
urea derivative
derivative
hot water
phosgene
Prior art date
Application number
Other languages
German (de)
Inventor
A-G J R Geigy
Original Assignee
Geigy Ag J R
Priority date (The priority date is an assumption and is not a legal conclusion. Google has not performed a legal analysis and makes no representation as to the accuracy of the date listed.)
Filing date
Publication date
Application filed by Geigy Ag J R filed Critical Geigy Ag J R
Publication of CH215319A publication Critical patent/CH215319A/en

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Classifications

    • CCHEMISTRY; METALLURGY
    • C07ORGANIC CHEMISTRY
    • C07CACYCLIC OR CARBOCYCLIC COMPOUNDS
    • C07C309/00Sulfonic acids; Halides, esters, or anhydrides thereof
    • C07C309/01Sulfonic acids
    • C07C309/28Sulfonic acids having sulfo groups bound to carbon atoms of six-membered aromatic rings of a carbon skeleton
    • C07C309/45Sulfonic acids having sulfo groups bound to carbon atoms of six-membered aromatic rings of a carbon skeleton containing nitrogen atoms, not being part of nitro or nitroso groups, bound to the carbon skeleton
    • C07C309/51Sulfonic acids having sulfo groups bound to carbon atoms of six-membered aromatic rings of a carbon skeleton containing nitrogen atoms, not being part of nitro or nitroso groups, bound to the carbon skeleton at least one of the nitrogen atoms being part of any of the groups, X being a hetero atom, Y being any atom

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  • Chemical & Material Sciences (AREA)
  • Organic Chemistry (AREA)
  • Organic Low-Molecular-Weight Compounds And Preparation Thereof (AREA)

Description

  

  Verfahren zur Herstellung eines     HarnstofFderivates.       Gegenstand des. vorliegenden Patentes ist ein       stoffderivates    der     Formel     
EMI0001.0004     
    dadurch gekennzeichnet,     dass    man     3,4-Di-          chloranilin    mit     Phosgen    zu einem Derivat der       3,4-Dichlorphenylcarbaminsäure    und dieses  mit     4-Amino-2',5'-dichlor-1,1'-diphenyläther-          2-sulfonsäure    umsetzt.

   Das neue Harnstoff  derivat bildet     als,        Natriumsalz    ein helles, in  heissem Wasser lösliches Pulver und eignet  sich als Mottenschutzmittel.  



       Beispiel:          a)    In 500 Teile     Essigester,    welche 135  Teile     Phosgen    enthalten, wird eine     Lösung     von 162 Teilen     3,4-Dichloranilin    in 1000 Tei  len Essigester langsam eingetropft, unter    Verfahren zur Herstellung eines Harn-         gleichzeitigem    Durchleiten eines     Phosgen-          stromes.    Nach Beendigung der     Reaktion    wird       dasLösungsmittel        in,derWärme        abdestilliert,     wobei das gebildete     3,

  4-Dichlorphenylcarb-          a-minsäurechlorid    unter     Salzsäureabspaltung     in das     3,4-Dichlorphenylisocyanat    übergeht.  



  b)     112p        Mol.    der     4-Amino-2',5'-@dichlor-          1,1'-diphenyläther-2-sulfonsäurewird        in        trok-          kenem        Pyridin    gelöst und unter Rühren bei  10 bis<B>15'</B> C     portionenweise    mit     1/"    Mal-,       3,4-Dichlorphenylisocyanat    versetzt. Dann  wird bei Raumtemperatur weitergerührt, bis  keine freie     Aminogruppe    mehr nachweisbar  ist.

   Hierauf versetzt man mit     Sodalösung    bis      zur alkalischen Reaktion und bläst das     Pyri-          din    mit Wasserdampf ab. Den Rückstand  löst man in     heissem    Wasser, filtriert die Lö  sung, fällt das Reaktionsprodukt durch Zu  gabe von Kochsalz als graues Harz aus und  
EMI0002.0004     
    dadurch gekennzeichnet,     da.ss    man     3,4-Di-          chloranilin    mit     Phosgen    zu einem Derivat der       3,4-Dichlorphenylcarbaminsäure    und dieses  mit     4-Amino-2',5'-dichlor-1,1'-diphenyläther-          2-sulfonsäure    umsetzt.

   Das neue Harnstoff-    erhält es nach dem Abtrennen, Trocknen und  Mahlen als helles, in heissem Wasser lösliches  Pulver.



  Process for the production of a urea derivative. The subject of the present patent is a substance derivative of the formula
EMI0001.0004
    characterized in that 3,4-dichloroaniline is reacted with phosgene to give a derivative of 3,4-dichlorophenylcarbamic acid and this with 4-amino-2 ', 5'-dichloro-1,1'-diphenylether-2-sulfonic acid.

   As a sodium salt, the new urea derivative forms a pale powder that is soluble in hot water and is suitable as a moth repellent.



       Example: a) A solution of 162 parts of 3,4-dichloroaniline in 1000 parts of ethyl acetate is slowly added dropwise to 500 parts of ethyl acetate which contain 135 parts of phosgene, using a method for producing urine while a phosgene stream is passed through. After the reaction has ended, the solvent is distilled off in the heat, whereby the 3,

  4-dichlorophenylcarb-a-minic acid chloride passes into the 3,4-dichlorophenyl isocyanate with elimination of hydrochloric acid.



  b) 112p mol. of the 4-amino-2 ', 5' - @ dichloro-1,1'-diphenyl ether-2-sulfonic acid is dissolved in dry pyridine and stirred at 10 to 15 ' 1 / ″ Mal-, 3,4-dichlorophenyl isocyanate are added to C in portions. Stirring is then continued at room temperature until free amino groups can no longer be detected.

   Soda solution is then added until an alkaline reaction occurs, and the pyridine is blown off with steam. The residue is dissolved in hot water, the solution is filtered, the reaction product is precipitated as a gray resin by adding sodium chloride and
EMI0002.0004
    characterized in that 3,4-dichloroaniline is combined with phosgene to form a derivative of 3,4-dichlorophenylcarbamic acid and this with 4-amino-2 ', 5'-dichloro-1,1'-diphenyl ether-2-sulfonic acid implements.

   The new urea is obtained after separation, drying and grinding as a pale powder that is soluble in hot water.

 

Claims (1)

PATENTANSPRUCH: Verfahren zur Herstellung eines Harn- stoffderivates der Formel derivat bildet als Natriumsalz ein helles, in heissem Wasser lösliches Pulver und eignet sich als Mottenschutzmittel. PATENT CLAIM: Process for the production of a urea derivative of the formula derivat, as a sodium salt, forms a light-colored powder that is soluble in hot water and is suitable as a moth repellent.
CH215319D 1938-06-16 1938-06-16 Process for the production of a urea derivative. CH215319A (en)

Applications Claiming Priority (2)

Application Number Priority Date Filing Date Title
CH212408T 1938-06-16
CH215319T 1938-06-16

Publications (1)

Publication Number Publication Date
CH215319A true CH215319A (en) 1941-06-15

Family

ID=25725199

Family Applications (1)

Application Number Title Priority Date Filing Date
CH215319D CH215319A (en) 1938-06-16 1938-06-16 Process for the production of a urea derivative.

Country Status (1)

Country Link
CH (1) CH215319A (en)

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