ES2637087T3 - Composiciones que contienen olefinas sustituidas con flúor - Google Patents

Composiciones que contienen olefinas sustituidas con flúor Download PDF

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Publication number
ES2637087T3
ES2637087T3 ES10011130.1T ES10011130T ES2637087T3 ES 2637087 T3 ES2637087 T3 ES 2637087T3 ES 10011130 T ES10011130 T ES 10011130T ES 2637087 T3 ES2637087 T3 ES 2637087T3
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Prior art keywords
composition
hfo
use according
propellant
atomized
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ES10011130.1T
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English (en)
Inventor
Hang T. Pham
Rajiv R. Singh
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Honeywell International Inc
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Honeywell International Inc
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    • C—CHEMISTRY; METALLURGY
    • C23—COATING METALLIC MATERIAL; COATING MATERIAL WITH METALLIC MATERIAL; CHEMICAL SURFACE TREATMENT; DIFFUSION TREATMENT OF METALLIC MATERIAL; COATING BY VACUUM EVAPORATION, BY SPUTTERING, BY ION IMPLANTATION OR BY CHEMICAL VAPOUR DEPOSITION, IN GENERAL; INHIBITING CORROSION OF METALLIC MATERIAL OR INCRUSTATION IN GENERAL
    • C23G—CLEANING OR DE-GREASING OF METALLIC MATERIAL BY CHEMICAL METHODS OTHER THAN ELECTROLYSIS
    • C23G5/00—Cleaning or de-greasing metallic material by other methods; Apparatus for cleaning or de-greasing metallic material with organic solvents
    • C23G5/02—Cleaning or de-greasing metallic material by other methods; Apparatus for cleaning or de-greasing metallic material with organic solvents using organic solvents
    • C23G5/028—Cleaning or de-greasing metallic material by other methods; Apparatus for cleaning or de-greasing metallic material with organic solvents using organic solvents containing halogenated hydrocarbons
    • C23G5/02803—Cleaning or de-greasing metallic material by other methods; Apparatus for cleaning or de-greasing metallic material with organic solvents using organic solvents containing halogenated hydrocarbons containing fluorine
    • C—CHEMISTRY; METALLURGY
    • C09—DYES; PAINTS; POLISHES; NATURAL RESINS; ADHESIVES; COMPOSITIONS NOT OTHERWISE PROVIDED FOR; APPLICATIONS OF MATERIALS NOT OTHERWISE PROVIDED FOR
    • C09K—MATERIALS FOR MISCELLANEOUS APPLICATIONS, NOT PROVIDED FOR ELSEWHERE
    • C09K5/00—Heat-transfer, heat-exchange or heat-storage materials, e.g. refrigerants; Materials for the production of heat or cold by chemical reactions other than by combustion
    • C—CHEMISTRY; METALLURGY
    • C09—DYES; PAINTS; POLISHES; NATURAL RESINS; ADHESIVES; COMPOSITIONS NOT OTHERWISE PROVIDED FOR; APPLICATIONS OF MATERIALS NOT OTHERWISE PROVIDED FOR
    • C09K—MATERIALS FOR MISCELLANEOUS APPLICATIONS, NOT PROVIDED FOR ELSEWHERE
    • C09K5/00—Heat-transfer, heat-exchange or heat-storage materials, e.g. refrigerants; Materials for the production of heat or cold by chemical reactions other than by combustion
    • C09K5/02—Materials undergoing a change of physical state when used
    • C09K5/04—Materials undergoing a change of physical state when used the change of state being from liquid to vapour or vice versa
    • C09K5/041—Materials undergoing a change of physical state when used the change of state being from liquid to vapour or vice versa for compression-type refrigeration systems
    • C09K5/044—Materials undergoing a change of physical state when used the change of state being from liquid to vapour or vice versa for compression-type refrigeration systems comprising halogenated compounds
    • C09K5/045—Materials undergoing a change of physical state when used the change of state being from liquid to vapour or vice versa for compression-type refrigeration systems comprising halogenated compounds containing only fluorine as halogen
    • A—HUMAN NECESSITIES
    • A01—AGRICULTURE; FORESTRY; ANIMAL HUSBANDRY; HUNTING; TRAPPING; FISHING
    • A01N—PRESERVATION OF BODIES OF HUMANS OR ANIMALS OR PLANTS OR PARTS THEREOF; BIOCIDES, e.g. AS DISINFECTANTS, AS PESTICIDES OR AS HERBICIDES; PEST REPELLANTS OR ATTRACTANTS; PLANT GROWTH REGULATORS
    • A01N29/00—Biocides, pest repellants or attractants, or plant growth regulators containing halogenated hydrocarbons
    • A01N29/02—Acyclic compounds or compounds containing halogen attached to an aliphatic side-chain of a cycloaliphatic ring system
    • A—HUMAN NECESSITIES
    • A61—MEDICAL OR VETERINARY SCIENCE; HYGIENE
    • A61P—SPECIFIC THERAPEUTIC ACTIVITY OF CHEMICAL COMPOUNDS OR MEDICINAL PREPARATIONS
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    • A—HUMAN NECESSITIES
    • A62—LIFE-SAVING; FIRE-FIGHTING
    • A62D—CHEMICAL MEANS FOR EXTINGUISHING FIRES OR FOR COMBATING OR PROTECTING AGAINST HARMFUL CHEMICAL AGENTS; CHEMICAL MATERIALS FOR USE IN BREATHING APPARATUS
    • A62D1/00—Fire-extinguishing compositions; Use of chemical substances in extinguishing fires
    • A62D1/0092—Gaseous extinguishing substances, e.g. liquefied gases, carbon dioxide snow
    • C—CHEMISTRY; METALLURGY
    • C07—ORGANIC CHEMISTRY
    • C07C—ACYCLIC OR CARBOCYCLIC COMPOUNDS
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    • C07C19/08—Acyclic saturated compounds containing halogen atoms containing fluorine
    • C—CHEMISTRY; METALLURGY
    • C07—ORGANIC CHEMISTRY
    • C07C—ACYCLIC OR CARBOCYCLIC COMPOUNDS
    • C07C21/00—Acyclic unsaturated compounds containing halogen atoms
    • C07C21/02—Acyclic unsaturated compounds containing halogen atoms containing carbon-to-carbon double bonds
    • C07C21/18—Acyclic unsaturated compounds containing halogen atoms containing carbon-to-carbon double bonds containing fluorine
    • C—CHEMISTRY; METALLURGY
    • C08—ORGANIC MACROMOLECULAR COMPOUNDS; THEIR PREPARATION OR CHEMICAL WORKING-UP; COMPOSITIONS BASED THEREON
    • C08J—WORKING-UP; GENERAL PROCESSES OF COMPOUNDING; AFTER-TREATMENT NOT COVERED BY SUBCLASSES C08B, C08C, C08F, C08G or C08H
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    • C08J—WORKING-UP; GENERAL PROCESSES OF COMPOUNDING; AFTER-TREATMENT NOT COVERED BY SUBCLASSES C08B, C08C, C08F, C08G or C08H
    • C08J9/00—Working-up of macromolecular substances to porous or cellular articles or materials; After-treatment thereof
    • C08J9/04—Working-up of macromolecular substances to porous or cellular articles or materials; After-treatment thereof using blowing gases generated by a previously added blowing agent
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    • C08J9/143—Halogen containing compounds
    • C08J9/144—Halogen containing compounds containing carbon, halogen and hydrogen only
    • C08J9/146—Halogen containing compounds containing carbon, halogen and hydrogen only only fluorine as halogen atoms
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    • C09—DYES; PAINTS; POLISHES; NATURAL RESINS; ADHESIVES; COMPOSITIONS NOT OTHERWISE PROVIDED FOR; APPLICATIONS OF MATERIALS NOT OTHERWISE PROVIDED FOR
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    • C09K21/00—Fireproofing materials
    • C09K21/06—Organic materials
    • C09K21/08—Organic materials containing halogen
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    • C09—DYES; PAINTS; POLISHES; NATURAL RESINS; ADHESIVES; COMPOSITIONS NOT OTHERWISE PROVIDED FOR; APPLICATIONS OF MATERIALS NOT OTHERWISE PROVIDED FOR
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    • C09K5/00—Heat-transfer, heat-exchange or heat-storage materials, e.g. refrigerants; Materials for the production of heat or cold by chemical reactions other than by combustion
    • C09K5/02—Materials undergoing a change of physical state when used
    • C09K5/04—Materials undergoing a change of physical state when used the change of state being from liquid to vapour or vice versa
    • C09K5/041—Materials undergoing a change of physical state when used the change of state being from liquid to vapour or vice versa for compression-type refrigeration systems
    • C09K5/044—Materials undergoing a change of physical state when used the change of state being from liquid to vapour or vice versa for compression-type refrigeration systems comprising halogenated compounds
    • C—CHEMISTRY; METALLURGY
    • C10—PETROLEUM, GAS OR COKE INDUSTRIES; TECHNICAL GASES CONTAINING CARBON MONOXIDE; FUELS; LUBRICANTS; PEAT
    • C10M—LUBRICATING COMPOSITIONS; USE OF CHEMICAL SUBSTANCES EITHER ALONE OR AS LUBRICATING INGREDIENTS IN A LUBRICATING COMPOSITION
    • C10M131/00—Lubricating compositions characterised by the additive being an organic non-macromolecular compound containing halogen
    • C10M131/02—Lubricating compositions characterised by the additive being an organic non-macromolecular compound containing halogen containing carbon, hydrogen and halogen only
    • C10M131/04—Lubricating compositions characterised by the additive being an organic non-macromolecular compound containing halogen containing carbon, hydrogen and halogen only aliphatic
    • C—CHEMISTRY; METALLURGY
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    • C10M141/04—Lubricating compositions characterised by the additive being a mixture of two or more compounds covered by more than one of the main groups C10M125/00 - C10M139/00, each of these compounds being essential at least one of them being an organic halogen-containing compound
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    • C11D—DETERGENT COMPOSITIONS; USE OF SINGLE SUBSTANCES AS DETERGENTS; SOAP OR SOAP-MAKING; RESIN SOAPS; RECOVERY OF GLYCEROL
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    • F25—REFRIGERATION OR COOLING; COMBINED HEATING AND REFRIGERATION SYSTEMS; HEAT PUMP SYSTEMS; MANUFACTURE OR STORAGE OF ICE; LIQUEFACTION SOLIDIFICATION OF GASES
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    • C—CHEMISTRY; METALLURGY
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    • C08J—WORKING-UP; GENERAL PROCESSES OF COMPOUNDING; AFTER-TREATMENT NOT COVERED BY SUBCLASSES C08B, C08C, C08F, C08G or C08H
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    • C11D7/22—Organic compounds
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Abstract

Una composición atomizable para su uso en medicina, comprendiendo dicha composición atomizable un propulsor que comprende HFO-1234ze y un material a ser atomizado, en donde dicho material a ser atomizado es un material medicinal

Description

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DESCRIPCION
Composiciones que contienen olefinas sustituidas con fluor
CAMPO DE LA INVENClON
Esta invencion se refiere a composiciones que tienen utilidad en calidad de un agente propulsor.
ANTECEDENTES DE LA INVENClON
Fluidos basados en fluorocarbonos han encontrado un uso generalizado en muchas aplicaciones comerciales e industriales. Por ejemplo, fluidos basados en fluorocarbonos se utilizan frecuentemente como un fluido de trabajo en sistemas tales como aplicaciones de acondicionamiento del aire, bomba de calor y de refrigeracion. El ciclo de la compresion de vapor es uno de los metodos tipo mas comunmente utilizados para conseguir la refrigeracion o el calentamiento en un sistema de refrigeracion. El ciclo de compresion de vapor implica habitualmente el cambio de fases del refrigerante desde la fase lfquida a la fase de vapor a traves de la absorcion de calor a una presion relativamente baja y luego desde la fase de vapor a la fase lfquida a traves de la eliminacion de calor a una presion y temperatura relativamente bajas, comprimir el vapor hasta una presion relativamente elevada, condensar el vapor a la fase lfquida a traves de la eliminacion de calor a esta presion y temperatura relativamente elevadas y luego reducir la presion para iniciar de nuevo el ciclo.
Mientras que el fin primario de la refrigeracion consiste en eliminar el calor de un objeto u otro fluido a una temperatura relativamente baja, el fin principal de una bomba de calor consiste en anadir calor a una temperatura mas elevada con respecto al entorno.
Determinados fluorocarbonos han sido un componente preferido en muchos fluidos de intercambio de calor tales como agentes refrigerantes, durante muchos anos en muchas aplicaciones. Por ejemplo, los fluoroalcanos tales como derivados de clorofluorometano y clorofluoroetano han adquirido un uso generalizado como agentes refrigerantes en aplicaciones que incluyen aplicaciones del acondicionamiento del aire y de la bomba de calor debido a su combinacion unica de propiedades qmmicas y ffsicas. Muchos de los agentes refrigerantes comunmente utilizados en sistemas de compresion de vapor son fluidos de un solo componente o mezclas azeotropicas.
En los ultimos anos ha crecido la preocupacion sobre el potencial dano a la atmosfera y clima de la Tierra y, a este respecto, se han identificado como particularmente problematicos determinados compuestos basados en cloro. El uso de composiciones con contenido en cloro (tales como clorofluorocarbonos (CFCs), hidrofluorocarbonos (HCFs) y similares) en calidad de agentes refrigerantes en sistemas de acondicionamiento del aire y de refrigeracion se ha visto desfavorecido debido a las propiedades de agotamiento del ozono asociadas con muchos compuestos de este tipo. Asf, ha existido una necesidad creciente de nuevos compuestos y composiciones de fluorocarbonos e hidrofluorocarbonos que ofrezcan alternativas para las aplicaciones de refrigeracion y de la bomba de calor. Por ejemplo, se ha vuelto deseable retro-ajustar los sistemas de refrigeracion con contenido en cloro reemplazando agentes refrigerantes con contenido en cloro por compuestos refrigerantes que no contengan cloro y que no agotaran la capa de ozono tales como hidrofluorocarbonos (HFCs).
La inflamabilidad es otra propiedad importante para muchas aplicaciones. Es decir, se considera importante o esencial en muchas aplicaciones, incluidas particularmente aplicaciones de transferencia de calor, utilizar composiciones que no sean inflamables. Asf, frecuentemente es beneficioso utilizar en composiciones de este tipo compuestos que no sean inflamables. Tal como se utiliza en esta memoria, la expresion “no inflamable” se refiere a compuestos o composiciones que se establece que son no inflamables segun se determina de acuerdo con la norma ASTM E-681 de fecha 2002, que se incorpora en esta memoria como referencia. Desgraciadamente, muchos HFCs que podnan ser de otro modo deseables para ser utilizados en composiciones refrigerantes, son inflamables. Por ejemplo, el fluoroalcano difluoroetano (HFC-152a) y el fluoroalqueno 1,1,1-trifluoropropeno (HFO- 1243zf) son cada uno de ellos inflamables y, por lo tanto, no son viables para uso en muchas aplicaciones.
Fluoroalquenos superiores, es decir, alquenos sustituidos con fluor que tengan al menos cinco atomos de carbono, han sido sugeridos para uso como agentes refrigerantes. La patente de EE.UU. n° 4.788.352 - Smutny se dirige a la produccion de compuestos C5 a Ca fluorados que tengan al menos un cierto grado de insaturacion. La patente de Smutny identifica a olefinas superiores de este tipo como conocidas por su utilidad como agentes refrigerantes, plaguicidas, fluidos dielectricos, fluidos de transferencia de calor, disolventes y compuestos intermedios en diversas reacciones qmmicas (vease la columna 1, lmeas 11-22).
Mientras que las olefinas fluoradas descritas en Smutny pueden tener un cierto nivel de eficacia en aplicaciones de
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transferencia de calor, se piensa que compuestos de este tipo tambien pueden tener determinados inconvenientes. Por ejemplo, algunos de estos compuestos pueden tender a atacar los sustratos, particularmente plasticos para fines generales tales como resinas acnlicas y resinas de ABS. Ademas de ello, los compuestos olefmicos superiores descritos en Smutny pueden tambien ser indeseables en determinadas aplicaciones, debido al potencial nivel de toxicidad de este tipo de compuestos que puede surgir como resultado de la actividad plaguicida senalada por Smutny. Tambien, compuestos de este tipo pueden tener un punto de ebullicion que sea demasiado elevado para hacerles utiles como un agente refrigerante en determinadas aplicaciones.
Derivados de bromofluorometano y bromoclorofluorometano, particularmente bromotrifluorometano (Halon 1301) y bromoclorodifluorometano (Halon 1211) han adquirido un uso generalizado como agentes para la extincion de incendios en zonas cerradas tales como cabinas de aviones y salas de ordenadores. Sin embargo, el uso de diversos halones esta siendo eliminado gradualmente debido a su elevado agotamiento del ozono. Ademas, dado que los halones se utilizan frecuentemente en zonas en las que estan presentes seres humanos, sustitutos adecuados deben ser tambien seguros para los seres humanos a las concentraciones necesarias para suprimir o extinguir el incendio.
El documento US-A-3723318 describe agentes propulsores de aerosol y agentes refrigerantes basados en trifluoropropeno (CF3CH=CH2).
El documento US-A-6300378 describe composiciones que comprenden bromo, que contienen aditivos halocarbonados que se utilizan para disminuir o eliminar la inflamabilidad de los propulsores de los aerosoles, refrigerantes, agentes de soplado de espumas, disolventes y esterilizantes.
El documento JP H04-110388 se refiere a la obtencion de fluidos novedosos para utilizar en la transferencia de calor que son adecuados para bombas de calor y maquinas termicas. La invencion descrita es un medio de transferencia de calor que comprende un compuesto organico que se puede representar mediante la formula molecular C3HmFn (en donde m esta comprendido entre 1 y 5, n esta comprendido entre 1 y 5, y m+n = 6) y que tiene un doble enlace en la estructura molecular.
La solicitante ha llegado pues a apreciar una necesidad de composiciones que sean potencialmente utiles en numerosas aplicaciones, al tiempo que eviten uno o mas de los inconvenientes arriba senalados.
SUMARIO
De acuerdo con la presente invencion, una composicion que comprende 1,3,3,3-tetrafluoropropeno (HFO-1234ze) es util como propulsor en una composicion atomizable para su uso en medicina o para su uso en el tratamiento del asma o la halitosis. La presente invencion tambien proporciona una composicion que comprende HFO-1234ze para utilizar como un propulsor en una composicion que comprende un material medico.
DESCRIPCION DETALLADA DE REALIZACIONES PREFERIDAS
En esta memoria se describen las clases de compuestos tetrafluoropropeno (HFO-1234) y pentafluoropropeno (HFO-1225).
El compuesto que es util en la presente invencion es el 1,3,3,3-tetrafluoropropeno (HFO-1234ze) y cualquiera de todos los estereoisomeros de este compuesto. La solicitante ha descubierto que este compuesto tiene un nivel de toxicidad aguda muy bajo segun se ha medido mediante la exposicion a la inhalacion de ratones y ratas.
Los compuestos descritos en esta memoria, concretamente HFO-1225 y HFO-1234, son materiales conocidos y estan registrados en las bases de datos de Chemical Abstracts.
Ademas de ello, generalmente en la bibliograffa de patentes se describen metodos para producir fluoroalquenos. Por ejemplo, la produccion de tetrafluoropropenos tal como CF3CH=CH2 mediante fluoracion en fase de vapor catalttica de diversos compuestos C3 con contenido en halogeno saturados e insaturados se describe en las patentes de EE.UU. n°s 2.889.379; 4.798.818 y 4.465.786. La patente de EE.UU. n° 5.532.419 describe un proceso catalttico en fase de vapor para la preparacion de fluoroalqueno utilizando un cloro- o bromo-halofluorocarbono y HF. El documento EP 974.571 describe la preparacion de 1,1,1,3-tetrafluoropropeno poniendo en contacto 1,1,1,3,3-pentafluoropropano (HFC-245fa) en la fase de vapor con un catalizador basado en cromo a temperatura elevada, o en la fase lfquida con una disolucion alcoholica de KOH, NaOH, Ca(OH)2 o Mg(OH)2. Ademas, metodos para producir compuestos divulgados en esta memoria se describen, en general, en relacion con la solicitud de patente de los Estados Unidos presentada al mismo tiempo, titulada “Procedimiento para producir fluoropropenos” con el numero de expediente del agente (H0003789 (26267)).
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Se piensa que las presentes composiciones poseen propiedades que son ventajosas por un cierto numero de razones importantes. Por ejemplo, la solicitante piensa, basado al menos en parte en un modelo matematico, que la fluoro-olefina que es util en la invencion no tendra efecto negativo sustancial alguno sobre la qmmica de la atmosfera, siendo un contribuyente despreciable al agotamiento del ozono en comparacion con algunas otras especies halogenadas. Las composiciones preferidas de la presente invencion tienen, asf, la ventaja de no contribuir esencialmente al agotamiento del ozono. Las composiciones preferidas tampoco contribuyen esencialmente al calentamiento global en comparacion con muchos de los hidrofluoroalcanos actualmente en uso.
Preferiblemente, las composiciones de la presente invencion tienen un potencial de calentamiento global (GWP - siglas en ingles) no mayor que 150, mas preferiblemente, no mayor que 100 e incluso mas preferiblemente, no mayor que 75. Tal como se utiliza en esta memoria, el “GWP” se mide con relacion al de dioxido de carbono y a lo largo de un horizonte en el tiempo de 100 anos, segun se define en “The Scientific Assessment of Ozone Depletion, 2002, A report of the World Meteorological Association's Global Ozone Research and Monitoring Project”.
Las presentes composiciones tienen tambien preferiblemente un potencial de agotamiento del ozono (ODP - siglas en ingles) no mayor que 0,05, mas preferiblemente no mayor que 0,02 e incluso mas preferiblemente, de aproximadamente cero. Tal como se utiliza en esta memoria, “ODP” es como se define en “The Scientific Assessment of Ozone Depletion, 2002, A report of the World Meteorological Association's Global Ozone Research and Monitoring Project”.
COMPOSICIONES DE AGENTES PROPULSORES
La presente invencion proporciona composiciones de agentes propulsores que comprenden o consisten esencialmente en HFO-1234ze, siendo dicha composicion de agente propulsor preferiblemente una composicion atomizable. Las composiciones de agente propulsor de la presente invencion comprenden preferiblemente un material a ser atomizado que es un material medicinal y un agente propulsor que comprende, consiste esencialmente o consiste en un HFO-1234ze. En la mezcla atomizable tambien pueden estar presentes ingredientes, disolventes y otros materiales inertes. Preferiblemente, la composicion atomizable es un aerosol. Materiales medicinales adecuados incluyen medicamentos anti-asma y anti-halitosis.

Claims (13)

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    REIVINDICACIONES
    1. - Una composicion atomizable para su uso en medicina, comprendiendo dicha composicion atomizable un propulsor que comprende HFO-1234ze y un material a ser atomizado, en donde dicho material a ser atomizado es un material medicinal.
  2. 2. - Una composicion atomizable para su uso en el tratamiento del asma, comprendiendo dicha composicion atomizable un propulsor que comprende HFO-1234ze y un material a ser atomizado, en donde dicho material a ser atomizado comprende un medicamento anti-asma.
  3. 3. - Una composicion atomizable para su uso en el tratamiento de la halitosis, comprendiendo dicha composicion atomizable un propulsor que comprende HFO-1234ze y un material a ser atomizado, en donde dicho material a ser atomizado comprende un medicamento anti-halitosis.
  4. 4. - La composicion para su uso de acuerdo con la cualquiera de las reivindicaciones 1 a 3, en donde la composicion es un aerosol.
  5. 5. - La composicion para su uso de acuerdo con cualquiera de las reivindicaciones 1 a 4, en donde la composicion tiene un Potencial del Calentamiento Global (GWP) no mayor que 150, mas preferiblemente no mayor que 100 e incluso mas preferiblemente no mayor que 75.
  6. 6. - La composicion para su uso de acuerdo con cualquiera de las reivindicaciones 1 a 5, en donde la composicion tiene un Potencial de Agotamiento del Ozono (ODP) no mayor que 0,05, mas preferiblemente no mayor que 0,02, e incluso mas preferiblemente de aproximadamente cero.
  7. 7. - La composicion para su uso de acuerdo con cualquiera de las reivindicaciones 1 a 6, en donde el propulsor consiste esencialmente en HFO-1234ze.
  8. 8. - El uso como propulsor de una composicion que comprende HFO-1234ze, en una composicion que comprende un material medicinal.
  9. 9. - El uso de acuerdo con la reivindicacion 8, en donde el propulsor consiste esencialmente en HFO-1234ze.
  10. 10. - El uso de acuerdo con la reivindicacion 8 o 9, en donde dicho material medicinal comprende medicamentos anti-asma o anti-halitosis.
  11. 11. - El uso de acuerdo con cualquiera las reivindicaciones 8 a 10, en donde la composicion es un aerosol.
  12. 12. - El uso de acuerdo con la cualquiera de las reivindicaciones 8 a 11, en donde la composicion tiene un Potencial del Calentamiento Global (GWP) no mayor que 150, mas preferiblemente no mayor que 100, e incluso mas preferiblemente no mayor que 75.
  13. 13. - El uso de acuerdo con cualquiera de las reivindicaciones 8 a 12, en donde la composicion tiene un Potencial de Agotamiento del Ozono (ODP) no mayor que 0,05, mas preferiblemente no mayor que 0,02, e incluso mas preferiblemente de aproximadamente cero.
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ES16204715T Expired - Lifetime ES2794405T3 (es) 2002-10-25 2003-10-27 Uso de composiciones que comprenden HFO-1234ze o HFO-1234yf como composición refrigerante
ES10011130.1T Expired - Lifetime ES2637087T3 (es) 2002-10-25 2003-10-27 Composiciones que contienen olefinas sustituidas con flúor
ES10011129.3T Expired - Lifetime ES2615857T3 (es) 2002-10-25 2003-10-27 Composiciones que contienen olefinas sustituidas con flúor
ES10011167.3T Expired - Lifetime ES2601879T3 (es) 2002-10-25 2003-10-27 Composiciones que contienen olefinas sustituidas con flúor
ES08020700.4T Expired - Lifetime ES2321796T5 (es) 2002-10-25 2003-10-27 Uso de una composición que comprende 1,3,3,3-tetrafluoropropeno (HFO 1234ze) en calidad de agente de soplado
ES03777896T Expired - Lifetime ES2382912T3 (es) 2002-10-25 2003-10-27 Composiciones que contienen olefinas sustituidas con flúor
ES10011164T Expired - Lifetime ES2728672T3 (es) 2002-10-25 2003-10-27 Composiciones que contienen olefinas sustituidas con flúor
ES10011131.9T Expired - Lifetime ES2645949T3 (es) 2002-10-25 2003-10-27 Método de esterilización que utiliza composiciones que contienen olefinas sustituidas con flúor

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ES10011167.3T Expired - Lifetime ES2601879T3 (es) 2002-10-25 2003-10-27 Composiciones que contienen olefinas sustituidas con flúor
ES08020700.4T Expired - Lifetime ES2321796T5 (es) 2002-10-25 2003-10-27 Uso de una composición que comprende 1,3,3,3-tetrafluoropropeno (HFO 1234ze) en calidad de agente de soplado
ES03777896T Expired - Lifetime ES2382912T3 (es) 2002-10-25 2003-10-27 Composiciones que contienen olefinas sustituidas con flúor
ES10011164T Expired - Lifetime ES2728672T3 (es) 2002-10-25 2003-10-27 Composiciones que contienen olefinas sustituidas con flúor
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