CH328660A - Process for the preparation of a disazo dye - Google Patents

Process for the preparation of a disazo dye

Info

Publication number
CH328660A
CH328660A CH328660DA CH328660A CH 328660 A CH328660 A CH 328660A CH 328660D A CH328660D A CH 328660DA CH 328660 A CH328660 A CH 328660A
Authority
CH
Switzerland
Prior art keywords
parts
disazo dye
oxy
preparation
amino
Prior art date
Application number
Other languages
German (de)
Inventor
Hans Dr Ischer
Lukas Dr Schneider
Original Assignee
Sandoz Ag
Priority date (The priority date is an assumption and is not a legal conclusion. Google has not performed a legal analysis and makes no representation as to the accuracy of the date listed.)
Filing date
Publication date
Application filed by Sandoz Ag filed Critical Sandoz Ag
Publication of CH328660A publication Critical patent/CH328660A/en

Links

Classifications

    • CCHEMISTRY; METALLURGY
    • C09DYES; PAINTS; POLISHES; NATURAL RESINS; ADHESIVES; COMPOSITIONS NOT OTHERWISE PROVIDED FOR; APPLICATIONS OF MATERIALS NOT OTHERWISE PROVIDED FOR
    • C09BORGANIC DYES OR CLOSELY-RELATED COMPOUNDS FOR PRODUCING DYES, e.g. PIGMENTS; MORDANTS; LAKES
    • C09B35/00Disazo and polyazo dyes of the type A<-D->B prepared by diazotising and coupling
    • C09B35/02Disazo dyes
    • C09B35/039Disazo dyes characterised by the tetrazo component
    • C09B35/28Disazo dyes characterised by the tetrazo component the tetrazo component containing two aryl nuclei linked by at least one of the groups —CON<, —SO2N<, —SO2—, or —SO2—O—
    • CCHEMISTRY; METALLURGY
    • C09DYES; PAINTS; POLISHES; NATURAL RESINS; ADHESIVES; COMPOSITIONS NOT OTHERWISE PROVIDED FOR; APPLICATIONS OF MATERIALS NOT OTHERWISE PROVIDED FOR
    • C09BORGANIC DYES OR CLOSELY-RELATED COMPOUNDS FOR PRODUCING DYES, e.g. PIGMENTS; MORDANTS; LAKES
    • C09B45/00Complex metal compounds of azo dyes
    • C09B45/02Preparation from dyes containing in o-position a hydroxy group and in o'-position hydroxy, alkoxy, carboxyl, amino or keto groups
    • C09B45/24Disazo or polyazo compounds
    • C09B45/28Disazo or polyazo compounds containing copper

Landscapes

  • Chemical & Material Sciences (AREA)
  • Organic Chemistry (AREA)
  • Coloring (AREA)

Description

  

  <B>Zusatzpatent</B> zum Hauptpatent Nr. 310831         Verfahren        zur    Herstellung     eines        Disazofarbstoffes       Gegenstand der vorliegenden     Erfindung     ist ein Verfahren     zur        Hersfellung    eines     Dis-          azofarbstoffes,    welches     darin    besteht, dass man  1     Mol    der durch Kuppeln von     tetrazotierter     1-     (4'-Amino-3'-methyl)

          -benzoylamino-4-amino-          benzol    - 3 -     carbonsäure    mit 5 -     Oxy-    7 -     sulfo-          naphthyl    (2)     -carbaminsäure-    (4' -     acetylamino-)        -          phenvjamid    erhältlichen     Diazomonoazoverbin-          dung    mit 1     Mol        1-(4'-Oxy-3'-carboxy)-phenyl-          5-pyrazolon-3-carbonsäureamid    kuppelt.  



  Im Beispiel bedeuten die Teile     Gewichts-          teile.     



  <I>Beispiel</I>  Eine     neutralgestellte,    8-10  kalte Suspen  sion der durch Kuppeln von 28,5 Teilen     tetra-          zotierter        1-(4'-Amino-3'-methyl)-benzoylamino-          4-aminobenzol-3-carbonsäure    mit 41,5 Teilen       5-Oxy-7-sulfonaphthyl(2)        -carbaminsäure-        (4'-          acetylamino)-phenylamid    erhältlichen     Diazo-          monoazozwischenverbindung    wird innerhalb  von einer Stunde in eine 30  warme Lösung  aus 26,3 Teilen     1-(4'-Oxy-3'-carboxy)

          phenyl-          5-pyrazolon-3-carbonsäureamid,    12 Teilen     Na-          triumcarbonat,    300 Teilen     Pyridin    und 500  Teilen Wasser gegeben. Der gebildete     Disazo-          farbstoff    wird nach zweistündigem Rühren  mittels Zusatz von     Natriumchlorid    abgeschie  den, anschliessend filtriert und getrocknet. Er  färbt Baumwolle und Fasern aus regenerier  ter     Cellulose    im     Nachkupferungsverfahren    in  roten Tönen von guter Licht- und Wasch  echtheit.  



  Die oben genannte Suspension der     Diazo-          monoazozwischenverhindung    erhält man, wenn  man 28,5 Teile     1-(4'-Amino-3'-methyl)-benzoy    1=         amino-4-aminobenzol-3-carbonsäiire    in 800 Tei  len Eiswasser anrührt und die     Aufschläm-          mung    mit 50 Teilen     301/oiger    Salzsäure und  hierauf bei 0  mit 46     Teilen*30'1/oiger    Natrium  nitritlösung versetzt.

   Der     Tetrazolösung        @lässt     man eine Lösung von 41,5 Teilen     5-Oxy-7-          sulfonaphthyl    (2) -     carbaminsäure    - (4' -     acetyl-          amino)-phenylamid    und 10 Teilen     Natrium-          carbonat    in 400 Teilen Wasser     zulaufen,    stellt  die Temperatur der Kupplungsmasse auf  8-10  und gibt ihr innerhalb von     einer     Stunde     portionenweise    ungefähr 20 Teile     Na-          triumbicarbonat    zu.

   Nachdem die Masse neu  tralgestellt worden ist, rührt man sie noch  2 Stunden lang bei 8-10  weiter. Dabei kup  pelt nur die am     Benzoylrest    sitzende     Diazo-          gruppe.    Die entstandene     Diazomonazozwischen-          verbindung    scheidet sich in roten Kristallen  aus.



  <B> Additional patent </B> to main patent No. 310831 Process for the production of a disazo dye The present invention relates to a process for the production of a disazo dye, which consists in that 1 mol of the 1- (4 ' -Amino-3'-methyl)

          -benzoylamino-4-amino-benzene-3-carboxylic acid with 5-oxy- 7-sulfonaphthyl (2) -carbamic acid- (4 '- acetylamino-) - phenvjamid available diazomonoazo compound with 1 mol 1- (4'- Oxy-3'-carboxy) -phenyl-5-pyrazolone-3-carboxamide couples.



  In the example, the parts mean parts by weight.



  <I> Example </I> A neutralized, 8-10 cold suspension of the tetrazotized 1- (4'-amino-3'-methyl) -benzoylamino-4-aminobenzene-3- by coupling 28.5 parts carboxylic acid with 41.5 parts of 5-oxy-7-sulfonaphthyl (2) carbamic acid (4'-acetylamino) phenylamide available diazo monoazo intermediate compound is in a 30 warm solution of 26.3 parts 1- (4 '-Oxy-3'-carboxy)

          phenyl-5-pyrazolone-3-carboxamide, 12 parts of sodium carbonate, 300 parts of pyridine and 500 parts of water. After stirring for two hours, the disazo dye formed is precipitated by adding sodium chloride, then filtered and dried. It dyes cotton and fibers from regenerated cellulose in red shades with good lightfastness and washfastness using the copper plating process.



  The abovementioned suspension of the diazo-monoazo intermediate compound is obtained when 28.5 parts of 1- (4'-amino-3'-methyl) -benzoy 1 = amino-4-aminobenzene-3-carboxylic acid are stirred in 800 parts of ice water and 50 parts of 301% hydrochloric acid were added to the suspension, followed by 46 parts of 30% sodium nitrite solution at 0.

   A solution of 41.5 parts of 5-oxy-7-sulfonaphthyl (2) -carbamic acid- (4'-acetyl-amino) -phenylamide and 10 parts of sodium carbonate in 400 parts of water is allowed to run into the tetrazo solution, and the temperature is set the coupling compound to 8-10 and add about 20 parts of sodium bicarbonate in portions within one hour.

   After the mass has been neutralized, it is stirred for a further 2 hours at 8-10. Only the diazo group on the benzoyl radical couples. The resulting diazomonazo intermediate compound separates out in red crystals.

 

Claims (1)

PATENTANSPRUCH Verfahren zur Herstellung eines Disazo- farbstoffes, dadurch gekennzeichnet, dass man 1 Mol der durch Kuppeln von tetrazotierter 1- (4'-Amino-3'-methyl) -benzoylamino-4-amino- benzol-3-carbonsäure mit 5-Oxy-7-sulfonaph thyl(2)-carbaminsäure-(4'-acetylaminö)-phenyl- amid erhältlichen Diazomonoazov erbindung mit 1 Mol 1-(4'-Oxy-3'-carboxy) PATENT CLAIM Process for the preparation of a disazo dye, characterized in that 1 mol of 1- (4'-amino-3'-methyl) -benzoylamino-4-aminobenzene-3-carboxylic acid with 5-oxy -7-sulfonaphthyl (2) -carbamic acid- (4'-acetylamino) -phenyl amide available diazomonoazov compound with 1 mole 1- (4'-oxy-3'-carboxy) -phenyl-5- pyrazolon-3-carbonsäureamid kuppelt. Der neue Disazofarbstoff färbt Baumwolle und Fasern aus regenerierter Cellulose im Nachkupferungsverfahren in roten Tönen von guter Licht- und Waschechtheit. -phenyl-5-pyrazolon-3-carboxamide couples. The new disazo dye dyes cotton and fibers from regenerated cellulose in red shades with good lightfastness and washfastness using the copper-plating process.
CH328660D 1954-05-11 1954-05-11 Process for the preparation of a disazo dye CH328660A (en)

Applications Claiming Priority (2)

Application Number Priority Date Filing Date Title
CH328660T 1954-05-11
CH310831T 1954-05-11

Publications (1)

Publication Number Publication Date
CH328660A true CH328660A (en) 1958-03-15

Family

ID=25735782

Family Applications (1)

Application Number Title Priority Date Filing Date
CH328660D CH328660A (en) 1954-05-11 1954-05-11 Process for the preparation of a disazo dye

Country Status (1)

Country Link
CH (1) CH328660A (en)

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