PL399306A1 - Proton cation ionic liquids 1-(2-chloroethyl)pyrrolidinyl and a process for their preparation - Google Patents

Proton cation ionic liquids 1-(2-chloroethyl)pyrrolidinyl and a process for their preparation

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Publication number
PL399306A1
PL399306A1 PL399306A PL39930612A PL399306A1 PL 399306 A1 PL399306 A1 PL 399306A1 PL 399306 A PL399306 A PL 399306A PL 39930612 A PL39930612 A PL 39930612A PL 399306 A1 PL399306 A1 PL 399306A1
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PL
Poland
Prior art keywords
chloroethyl
chain
alkyl
ionic liquids
pyrrolidinium
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Application number
PL399306A
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Polish (pl)
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PL225664B1 (en
Inventor
Juliusz Pernak
Barbara Górska
Francois Beguin
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Politechnika Poznanska
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Priority to PL399306A priority Critical patent/PL225664B1/en
Publication of PL399306A1 publication Critical patent/PL399306A1/en
Publication of PL225664B1 publication Critical patent/PL225664B1/en

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Abstract

Przedmiotem wynalazku sa protonowe ciecze jonowe z kationem 1-(2-chloroetylo)pirolidyniowym oraz sposób ich otrzymywania majace zastosowanie jako ekstrahent jonów miedzi z roztworów wodnych. Protonowe ciecze jonowe z kationem 1-(2-chloroetylo)pirolidyniowym o wzorze ogólnym 2, w którym, A- oznacza anion organiczny alkilokarboksylowy lancuchowy lub rozgaleziony o dlugosci lancucha alkilowego od 1 do 10 atomów wegla, bis(trifluorometylosulfonylo)imidkowy lub nieorganiczny z grupy: azotanów(III) lub azotanów(V) lub wodorosiarczanów(IV) lub wodorosiarczanów(VI) lub siarczanów(IV), siarczanów(VI) lub tetrafluoroboranów lub heksafluorofosforanów. Sposób polega na tym, ze chlorowodorek 1-(2-chloroetylo)pirolidyniowy, rozpuszcza sie w krótkolancuchowym alkoholu alifatycznym, korzystnie w metanolu, miesza sie z alkoholanowym roztworem soli sodowej lub potasowej, lub litowej, lub amonowej kwasu alkilokarboksylowego lancuchowego lub rozgalezionego o dlugosci lancucha alkilowego od 1 do 10 atomów wegla, w stosunku molowym chlorowodorku 1-(2-chloroetylo)pirolidyniowym do soli kwasu organicznego od 1:1 do 1:1,05, korzystnie 1:1, w temperaturze od 293 do 363 K, korzystnie 293 K, w czasie co najmniej 2 minut, nastepnie odsacza sie nieorganiczny produkt uboczny, po czym z przesaczu usuwa sie rozpuszczalnik.The subject of the invention are proton ionic liquids with a 1- (2-chloroethyl) pyrrolidinium cation and a method for their preparation which is used as an extractant of copper ions from aqueous solutions. Protic ionic liquids with a 1- (2-chloroethyl) pyrrolidinium cation of general formula 2, wherein, A- is an organic chain or alkyl branched alkyl carboxylic anion with an alkyl chain length of from 1 to 10 carbon atoms, bis (trifluoromethylsulfonyl) imide or inorganic group : nitrates (III) or nitrates (V) or bisulphates (IV) or bisulphates (VI) or sulphates (IV), sulphates (VI) or tetrafluoroborates or hexafluorophosphates. The method consists in the fact that 1- (2-chloroethyl) pyrrolidinium hydrochloride is dissolved in a short-chain aliphatic alcohol, preferably in methanol, mixed with an alcoholate solution of sodium or potassium or lithium or ammonium chain or branched chain alkyl carboxylic acid alkyl from 1 to 10 carbon atoms, in a molar ratio of 1- (2-chloroethyl) pyrrolidinium hydrochloride to the organic acid salt from 1: 1 to 1: 1.05, preferably 1: 1, at a temperature from 293 to 363 K, preferably 293 K, for at least 2 minutes, the inorganic by-product is filtered off, then the solvent is removed from the filtrate.

PL399306A 2012-05-25 2012-05-25 Proton cation ionic liquids 1-(2-chloroethyl)pyrrolidinyl and a process for their preparation PL225664B1 (en)

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PL399306A PL225664B1 (en) 2012-05-25 2012-05-25 Proton cation ionic liquids 1-(2-chloroethyl)pyrrolidinyl and a process for their preparation

Applications Claiming Priority (1)

Application Number Priority Date Filing Date Title
PL399306A PL225664B1 (en) 2012-05-25 2012-05-25 Proton cation ionic liquids 1-(2-chloroethyl)pyrrolidinyl and a process for their preparation

Publications (2)

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PL399306A1 true PL399306A1 (en) 2013-12-09
PL225664B1 PL225664B1 (en) 2017-05-31

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