CH313108A - Process for the preparation of a copper-containing polyazo dye of the stilbene series - Google Patents

Process for the preparation of a copper-containing polyazo dye of the stilbene series

Info

Publication number
CH313108A
CH313108A CH313108DA CH313108A CH 313108 A CH313108 A CH 313108A CH 313108D A CH313108D A CH 313108DA CH 313108 A CH313108 A CH 313108A
Authority
CH
Switzerland
Prior art keywords
copper
polyazo dye
stilbene series
parts
dye
Prior art date
Application number
Other languages
German (de)
Inventor
Kappeler Markus Dipl-Ing Che H
Schweizer August
Original Assignee
Sandoz Ag
Priority date (The priority date is an assumption and is not a legal conclusion. Google has not performed a legal analysis and makes no representation as to the accuracy of the date listed.)
Filing date
Publication date
Application filed by Sandoz Ag filed Critical Sandoz Ag
Publication of CH313108A publication Critical patent/CH313108A/en

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Classifications

    • CCHEMISTRY; METALLURGY
    • C09DYES; PAINTS; POLISHES; NATURAL RESINS; ADHESIVES; COMPOSITIONS NOT OTHERWISE PROVIDED FOR; APPLICATIONS OF MATERIALS NOT OTHERWISE PROVIDED FOR
    • C09BORGANIC DYES OR CLOSELY-RELATED COMPOUNDS FOR PRODUCING DYES, e.g. PIGMENTS; MORDANTS; LAKES
    • C09B45/00Complex metal compounds of azo dyes
    • C09B45/02Preparation from dyes containing in o-position a hydroxy group and in o'-position hydroxy, alkoxy, carboxyl, amino or keto groups
    • C09B45/24Disazo or polyazo compounds
    • C09B45/28Disazo or polyazo compounds containing copper

Landscapes

  • Chemical & Material Sciences (AREA)
  • Organic Chemistry (AREA)
  • Paper (AREA)
  • Inks, Pencil-Leads, Or Crayons (AREA)
  • Coloring (AREA)

Description

  

  <B>Zusatzpatent</B> zum Hauptpatent Nr. 312189    verfahren zur Herstellung     eines    kupferhaltigen     Polyazofarbstoffes    der     Stilbenreihe       Gegenstand des vorliegenden Patentes ist  ein Verfahren zur Herstellung eines kupfer  haltigen     Polyazofarbstoffes    der     Stilbenreihe,       welches darin besteht, dass man 1     Mol    der       Aminotrisazoverbindung    der     Zusammenset-          zung     
EMI0001.0010     
         diazotiert,        den:

          Diazokörper    mit 1     Mol        2,2',4'-          Trioxy-1,1'-azobenzol-5-sulfonsäure        kuppelt     und den erhaltenen     Polyazofarbstoff    mit kup  ferabgebenden Mitteln derart behandelt, dass  unter Aufspaltung der     Methoxygruppe    ein  kupferhaltiger     Polyazofarbstoff    entsteht, der  auf ein     F'arbstoffmolekül    zwei Atome Kupfer  komplex gebunden enthält.

      Der neue, kupferhaltige     Polyazofarbstoff     der     Stilbenreihe    ist ein schwarzes Pulver,  welches sich in Wasser mit     dunkelbrauner     Farbe löst und     Chromvelourleder    in schwarz  braunen, schleifechten Tönen färbt.  



  Im nachfolgenden Beispiel bedeuten die  Teile Gewichtsteile, und die Prozente sind in  Gewichtsprozenten angegeben.    <I>Beispiel</I>  79,1 Teile der     Aminotrisazoverbindung    der Zusammensetzung  
EMI0001.0027     
    werden in Form des     Natriumsalzes    in 1000  Teilen Wasser gelöst und durch Zugabe einer  Lösung von 7 Teilen     Natriumnitrit    in 20 Tei  len Wasser und 30 Teilen     30 /oiger    Salzsäure  bei 1.5      diazotiert.    Die     Diazosuspension    lässt  man     ztt    einer eisgekühlten Lösung von 31 Tei-         len        2,2',4'-Trioxy-7.,

  1'-azobenzol-5-sulfonsäure     und 40 Teilen     Natriumcarbonat    in 600 Teilen  Wasser fliessen. Nach beendigter Kupplung  wird der erhaltene     Polyazofarbstoff    durch  Zugabe von     Natriumehlorid    zur Lösung ab  geschieden und hierauf     abfiltriert.         Zur     überführung    des Farbstoffes in eine       Kupferkomplexverbindung,    welche auf ein  Molekül.

   des     Polyazofarbstoffes    zwei Atome  Kupfer komplex gebunden enthält, wird die  ser in 2500 Teilen heissem Wasser gelöst und  nach Zusatz von 100 Teilen     25 /oiger        Ammo-          niaklösung    und nach Zugabe einer Lösung  von 50 Teilen kristallisiertem Kupfersulfat in  200 Teilen Wasser     während.    9 Stunden bei 90    bis 95  gerührt. Der entstandene kupferhal  tige     Polyazofarbstoff    wird mittels Natrium  chlorid aus der Lösung abgeschieden,     abfil-          triert    und getrocknet.

   Er stellt ein schwar  zes Pulver dar, welches sich in Wasser mit  dunkelbrauner Farbe löst und     Chromvelour-          leder    in schwarzbraunen, schleifechten Tönen  färbt.



  <B> Additional patent </B> to main patent No. 312189 Process for the production of a copper-containing polyazo dye of the stilbene series The subject of the present patent is a process for the production of a copper-containing polyazo dye of the stilbene series, which consists in adding 1 mol of the aminotrisazo compound of the composition tongue
EMI0001.0010
         diazotized, the:

          Diazo bodies with 1 mol of 2,2 ', 4'-trioxy-1,1'-azobenzene-5-sulfonic acid and the resulting polyazo dye is treated with copper-releasing agents in such a way that, with splitting of the methoxy group, a copper-containing polyazo dye is formed which is based on an F. 'Dye molecule contains two atoms of copper in a complex bond.

      The new, copper-containing polyazo dye from the stilbene series is a black powder that dissolves in water with a dark brown color and dyes chrome suede in black-brown, abrasion-resistant tones.



  In the example below, parts are parts by weight and percentages are percentages by weight. <I> Example </I> 79.1 parts of the aminotrisazo compound of the composition
EMI0001.0027
    are dissolved in 1000 parts of water in the form of the sodium salt and diazotized at 1.5 by adding a solution of 7 parts of sodium nitrite in 20 parts of water and 30 parts of 30% hydrochloric acid. The diazo suspension is left in an ice-cooled solution of 31 parts of 2,2 ', 4'-trioxy-7.,

  1'-azobenzene-5-sulfonic acid and 40 parts of sodium carbonate flow in 600 parts of water. When the coupling is complete, the polyazo dye obtained is separated off by adding sodium chloride to the solution and then filtered off. To convert the dye into a copper complex compound, which is attached to a molecule.

   of the polyazo dye contains two atoms of copper in a complex bond, this water is dissolved in 2500 parts of hot water and after adding 100 parts of 25% ammonia solution and after adding a solution of 50 parts of crystallized copper sulfate in 200 parts of water. Stirred at 90-95 for 9 hours. The resulting copper-containing polyazo dye is precipitated from the solution using sodium chloride, filtered off and dried.

   It is a black powder that dissolves in water with a dark brown color and dyes chrome suede in black-brown, abrasion-resistant tones.

 

Claims (1)

PATENTANSPRUCH Zierfahren zur Herstellung eines kupfer haltigen Polyazofarbstoffes der Stilbenreihe, dadurch gekennzeichnet, dass man 1 Mol der Aminotrisazov erbindung der Zusammenset zung EMI0002.0019 diazotiert, den Diazokörper mit 1 Mol 2,2',4'- Trioxy-1,1'-azobenzol-5-sulfonsäure kuppelt und den erhaltenen Polyazofarbstoff mit kup ferabgebenden Mitteln derart behandelt, PATENT CLAIM Decorative process for the production of a copper-containing polyazo dye of the stilbene series, characterized in that one mole of the aminotrisazov compound of the composition EMI0002.0019 diazotized, coupling the diazo body with 1 mol of 2,2 ', 4'-trioxy-1,1'-azobenzene-5-sulfonic acid and treating the resulting polyazo dye with copper-releasing agents in this way, dass unter Aufspaltung der Methoxygruppe ein kupferhaltiger Polyazofarbstoff entsteht, der auf ein Parbstoffmolekül zwei Atome Kupfer komplex gebunden enthält. Der neue, kupferhaltige Polyazofarbstoff der Stilbenreihe ist ein schwarzes Pulver, wel ches sich in Wasser mit dunkelbrauner Farbe löst und Chromvelourleder in schwarzbrau nen, schleifeehten Tönen färbt. that by splitting the methoxy group, a copper-containing polyazo dye is formed, which contains two atoms of copper in a complex bonded to a paraffin molecule. The new, copper-containing polyazo dye from the stilbene series is a black powder which dissolves in water with a dark brown color and dyes chrome suede in black-brown, ribbon-like tones.
CH313108D 1952-12-24 1952-12-24 Process for the preparation of a copper-containing polyazo dye of the stilbene series CH313108A (en)

Applications Claiming Priority (2)

Application Number Priority Date Filing Date Title
CH313108T 1952-12-24
CH312189T 1952-12-24

Publications (1)

Publication Number Publication Date
CH313108A true CH313108A (en) 1956-03-15

Family

ID=25735887

Family Applications (1)

Application Number Title Priority Date Filing Date
CH313108D CH313108A (en) 1952-12-24 1952-12-24 Process for the preparation of a copper-containing polyazo dye of the stilbene series

Country Status (1)

Country Link
CH (1) CH313108A (en)

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